HIGHLIGHTS Low LCOE is achieved due to extreme low cost of perovskites in tandem PVs Further improving tandem module lifetime and efficiency reduces LCOE LCOE decrease rates are used to measure the research efforts
Long-term stability is an essential requirement for perovskite solar cells (PSCs) to be commercially viable. Heterojunctions built by low-dimensional and three-dimensional perovskites (1D/3D or 2D/3D) help to improve the stability...
Understanding interfacial loss and the ways to improving interfacial property is critical to fabricate highly efficient and reproducible perovskite solar cells (PSCs). In SnO2‐based PSCs, nonradiative recombination sites at the SnO2–perovskite interface lead to a large potential loss and performance variation in the resulting photovoltaic devices. Here, a novel SnO2‐in‐polymer matrix (i.e., polyethylene glycol) is devised as the electron transporting layer to improve the film quality of the SnO2 electron transporting layer. The SnO2‐in‐polymer matrix is fabricated through spin‐coating a polymer‐incorporated SnO2 colloidal ink. The polymer is uniformly dispersed in SnO2 colloidal ink and promotes the nanoparticle disaggregation in the ink. Owing to polymer incorporation, the compactness and wetting property of SnO2 layer is significantly ameliorated. Finally, photovoltaic devices based on Cs0.05FA0.81MA0.14PbI2.55Br0.45 perovskite sandwiched between SnO2 and Spiro‐OMeTAD layer are fabricated. Compared with the averaging power conversion efficiency of 16.2% with 1.2% deviation for control devices, the optimized devices exhibit an improved averaging efficiency of 19.5% with 0.25% deviation. The conception of polymer incorporation in the electron transporting layer paves a way to further increase the performance of planar perovskite solar cells.
Paper-based transparent flexible thin film supercapacitors were fabricated using CNF-[RGO]n hybrid paper as an electrode material and charge collector. Owing to the self-anti-stacking of distorted RGO nanosheets and internal electrolyte nanoscale-reservoirs, the device exhibited good electrochemical performance (about 1.73 mF cm(-2)), and a transmittance of about 56% (at 550 nm).
In scaffold based bone tissue engineering, both the pore size and the mechanical properties of the scaffold are of great importance. However, an increase in pore size is generally accompanied by a decrease in mechanical properties. In order to achieve both suitable mechanical properties and porosity, a multilayer scaffold is designed to mimic the structure of cancellous bone and cortical bone. A porous nano-hydroxyapatite-chitosan composite scaffold with a multilayer structure is fabricated and encased in a smooth compact chitosan membrane layer to prevent fibrous tissue ingrowth. The exterior tube is shown to have a small pore size (15-40 microm in diameter) for the enhancement of mechanical properties, while the core of the multilayer scaffold has a large pore size (predominantly 70-150 microm in diameter) for nutrition supply and bone formation. Compared with the uniform porous scaffold, the multilayer scaffold with the same size shows an enhanced mechanical strength and larger pore size in the center. More cells are shown to grow into the center of the multilayer scaffold in vitro than into the uniform porous scaffold under the same seeding condition. Finally, the scaffolds are implanted into a rabbit fibula defect to evaluate the osteoconductivity of the scaffold and the efficacy of the scaffold as a barrier to fibrous tissue ingrowth. At 12 weeks post operation, affluent blood vessels and bone formation are found in the center of the scaffold and little fibrous tissue is noted in the defect site.
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