Ilmenite-hematite (IH) [(1-x)FeTiO 3 ·xFe 2 O 3 ] solid solutions are unique classes of materials showing both magnetic and semiconducting properties, which make them potential candidates for novel applications in microelectronics and spintronics. This paper focuses on their varistor behavior before and after exposure to 40 MeV and 10 MeV proton radiations up to a fluence of 5 ϫ 10 10 p/cm 2 . The IH films are tolerant to these irradiations with little significant change to the nonlinear current-voltage characteristics. The switching voltage of the devices is in the regime of practical applications, and the radiation tolerance makes these materials suitable for aerospace applications.Radiation-induced damage has become an important field of study and continues to gain importance because of the need to protect electronic components, devices, and microelectronic circuits from the potentially catastrophic effects of radiation on their performance. 1 Space systems often require electronics that can operate in a high-radiation environment. This radiation may result from particles trapped in planetary magnetic fields, galactic cosmic rays, or high-energy protons from solar events. Exposure to high energetic particles can degrade device performance and ultimately lead to component failure. The primary effects of natural space radiation on spacecraft electronics are total ionizing dose effects, displacement damage, and single event upsets. 2 Radiation can alter the characteristics of electronic materials and the performance of electronic devices made from these materials by the mechanisms of ionization and atomic displacement. The displacement damage takes place by nuclear interactions and the ionization damage by atomic interactions in which energy deposited by the ionizing radiations creates electron-hole pairs. Semiconductor-based sensors, such as varistors and other current sensitive sensors, have applications in aerospace and other hostile environments for power and other applications. The radiation effects on device performance are important in these applications because the elevated radiation levels associated with these environments can produce both ionization and displacement damage.