The spin Hall effect is a spin–orbit coupling phenomenon, which enables electric generation and detection of spin currents. This relativistic effect provides a way for realizing efficient spintronic devices based on electric manipulation of magnetization through spin torque. However, it has been believed that heavy metals are indispensable for the spin–torque generation. Here we show that the spin Hall effect in Cu, a light metal with weak spin–orbit coupling, is significantly enhanced through natural oxidation. We demonstrate that the spin–torque generation efficiency of a Cu/Ni81Fe19 bilayer is enhanced by over two orders of magnitude by tuning the surface oxidation, reaching the efficiency of Pt/ferromagnetic metal bilayers. This finding illustrates a crucial role of oxidation in the spin Hall effect, opening a route for engineering the spin–torque generator by oxygen control and manipulating magnetization without using heavy metals.
We report the observation of the intrinsic dampinglike spin-orbit torque (SOT) arising from the Berry curvature in metallic-magnet/CuO_{x} heterostructures. We show that a robust dampinglike SOT, an order of magnitude larger than a fieldlike SOT, is generated in the heterostructure despite the absence of the bulk spin-orbit effect in the CuO_{x} layer. Furthermore, by tuning the interfacial oxidation level, we demonstrate that the fieldlike SOT changes drastically and even switches its sign, which originates from oxygen-modulated spin-dependent disorder. These results provide important information for a fundamental understanding of the physics of the SOTs.
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