This study investigates heat waves in Taiwan and their maintenance mechanism, based upon observations and dynamically downscaled simulations. A 95th percentile threshold is used for identifying hot extremes over a period of consecutive days. Heat waves are forecast to become more severe in the future projection. Daily minimum temperatures are generally high and diurnal temperature ranges (DTR) are relatively large. The daily minimum temperature serves as the primary control in the variation in DTR during heat waves. An apparent increase in the daily minimum temperature suggests elevated heat stress at nighttime during future heat waves. Heat waves in Taiwan are associated with abnormal warming and drying atmospheric conditions under the control of an enhanced western North Pacific subtropical high. The surrounding waters serve as a vast moisture source to suppress the drying magnitude in the surface layer as the temperature rises, thereby ensuring a high humidity level during the hot spell. The subsidence and adiabatic warming above can trap the warm and humid air in the surface layer, leading to positive feedback to the abnormally hot surface condition. The associated warming and drying atmospheric conditions cover certain spatial extents, suggesting that the extreme situation identified here is not confined to just an island-wide hot spell; the abnormal hot weather can take place across a broad geographical area.

This study examined the climate variability of heat wave (HW) according to air temperature and relative humidity to determine trends of variation and stress threshold in three major cities of Taiwan, Taipei (TP), Taichung (TC), and Kaohsiung (KH), in the past four decades . According to the data availability, the wet-bulb globe temperature (WBGT) heat stress for the three studied cities was also calculated for the past (2003)(2004)(2005)(2006)(2007)(2008)(2009)(2010)(2011)(2012) and simulated under the future warming scenario for the end of this century (2075-2099) using ECHAM5/MPIOM-WRF (ECW) dynamic downscaling 5-km resolution. Analysis showed that past decade (2001-2010) saw increase not only in the number of HW days in all three cities but also in the duration of each HW event in TP and KH. Simulation results revealed that ECW well captures the characteristics of data distribution in these three cities during [2003][2004][2005][2006][2007][2008][2009][2010][2011][2012]. Under the A1B projection, ECW yielded higher WBGT in all three cities for 2075-2099. The WBGT in TP indicated that the heat stress for 50% of the days in July and August by 2075-2099 will be at danger level (WBGT ≥ 31°C). Even the median of WBGT in TC and KH (30.91 and 30.88°C, respectively) are close to 31°C. Hence, the heat stress in all three cities will either exceed or approach the danger level by the end of this century. Such projection under the global warming trend would necessitate adaptation and mitigation, and the huge impact of dangerous heat stress on public health merits urgent attention for Taiwan.

Abstract. Air pollution is typically at its lowest in Taiwan during summer. The mean concentrations of PM10, PM2.5, and daytime ozone (08:00–17:00 LST) during summer (June–August) over central Taiwan were 35–40 µg m−3, 18–22 µg m−3, and 30–42 ppb, respectively, between 2004 and 2019. Sampling analysis revealed that the contribution of organic carbon (OC) to PM2.5 could have exceeded 30 % in urban and inland mountain sites during July in 2017 and 2018. Frequent episodes of air quality deterioration occur over the western plains of Taiwan when an easterly typhoon circulation interacts with the complex topographic structure of the island. We explored an episode of air quality deterioration that was associated with a typhoon between 15 and 17 July 2018 using the Weather Research Forecasting with Chemistry (WRF-Chem) model. The results indicated that the continual formation of low-pressure systems or typhoons in the area between Taiwan and Luzon island in the Philippines provided a strong easterly ambient flow, which lasted for an extended period between 15 and 17 July. The interaction between the easterly flow and Taiwan's Central Mountain Range (CMR) resulted in stable weather conditions and weak wind speed in western Taiwan during the study period. Numerical modeling also indicated that a lee side vortex easily formed, and the wind direction could have changed from southwesterly to northwesterly over central Taiwan because of the interaction between the typhoon circulation and the CMR. The northwesterly wind coupled with a sea breeze was conducive to the transport of air pollutants from the coastal upstream industrial and urban areas to the inland area. The dynamic process for the wind direction changed given a reasonable explanation for why the observed SO42- became the major contributor to PM2.5 during the episode. SO42- contribution proportions (%) to PM2.5 at the coastal, urban, and mountain sites were 9.4 µg m−3 (30.5 %), 12.1 µg m−3 (29.9 %), and 11.6 µg m−3 (29.7 %), respectively. Moreover, the variation of the boundary layer height had a strong effect on the concentration level of both PM2.5 and ozone. The lee vortex and land–sea breeze, as well as the boundary layer development, were the key mechanisms in air pollutant accumulation and transport. As typhoons frequently occur around Taiwan during summer and fall, their effect on the island's air quality merits further research attention.

Abstract. The Indochina biomass burning (BB) season in springtime has a substantial environmental impact on the surrounding areas in Asia. In this study, we evaluated the environmental impact of a major long-range BB transport event on 19 March 2018 (a flight of the HALO research aircraft, flight F0319) preceded by a minor event on 17 March 2018 (flight F0317). Aircraft data obtained during the campaign in Asia of the Effect of Megacities on the transport and transformation of pollutants on the Regional to Global scales (EMeRGe) were available between 12 March and 7 April 2018. In the F0319, results of 1-min mean carbon monoxide (CO), ozone (O3), acetone (ACE), acetonitrile (ACN), organic aerosol (OA) and black carbon aerosol (BC) concentrations were up to 312.0 ppb, 79.0 ppb, 3.0 ppb, 0.6 ppb, 6.4 µg m−3, 2.5 µg m−3 respectively, during the flight, which passed through the BB plume transport layer (BPTL) between the elevation of 2000–4000 m over the East China Sea (ECS). During F0319, CO, O3, ACE, ACN, OA and BC maximum of the 1 minute average concentrations were higher in the BPTL by 109.0 ppb, 8.0 ppb, 1.0 ppb, 0.3 ppb, 3.0 µg m−3 and 1.3 µg m−3 compared to flight F0317, respectively. Sulfate aerosol, rather than OA, showed the highest concentration at low altitudes (<1000 m) in both flights F0317 and F0319 resulting from the continental outflow in the ECS. The transport of BB aerosols from Indochina and its impacts on the downstream area was evaluated using a WRF-Chem model. Over the ECS, the simulated BB contribution demonstrated an increasing trend from the lowest values on 17 March 2018 to the highest values on 18 and 19 March 2018 for CO, fine particulate matter (PM2.5), OA, BC, hydroxyl radicals (OH), nitrogen oxides (NOx), total reactive nitrogen (NOy), and O3; by contrast, the variation of J(O1D) decreased as the BB plume’s contribution increased over the ECS. In the low boundary layer (<1000 m), the BB plume’s contribution to most species in the remote downstream areas was <20 %. However, at the BPTL, the contribution of the long-range transported BB plume was as high as 30–80 % for most of the species (NOy, NOx, PM2.5, BC, OH, O3, and CO) over South China (SC), Taiwan, and the ECS. BB aerosols were identified as a potential source of cloud condensation nuclei, and the simulation results indicated that the transported BB plume had an effect on cloud water formation over SC and the ECS on 19 March 2018. The combination of BB aerosol enhancement with cloud water resulted in a reduction of incoming shortwave radiation at the surface in SC and the ECS which potentially has significant regional climate implications.

Abstract. The Indochina biomass burning (BB) season in springtime has a substantial environmental impact on the surrounding areas in Asia. In this study, we evaluated the environmental impact of a major long-range BB transport event on 19 March 2018 (a flight of the High Altitude and Long Range Research Aircraft (HALO; https://www.halo-spp.de, last access: 14 February 2023) research aircraft, flight F0319) preceded by a minor event on 17 March 2018 (flight F0317). Aircraft data obtained during the campaign in Asia of the Effect of Megacities on the transport and transformation of pollutants on the Regional to Global scales (EMeRGe) were available between 12 March and 7 April 2018. In F0319, results of 1 min mean carbon monoxide (CO), ozone (O3), acetone (ACE), acetonitrile (ACN), organic aerosol (OA), and black carbon aerosol (BC) concentrations were up to 312.0, 79.0, 3.0, and 0.6 ppb and 6.4 and 2.5 µg m−3, respectively, during the flight, which passed through the BB plume transport layer (BPTL) between the elevation of 2000–4000 m over the East China Sea (ECS). During F0319, the CO, O3, ACE, ACN, OA, and BC maximum of the 1 min average concentrations were higher in the BPTL by 109.0, 8.0, 1.0, and 0.3 ppb and 3.0 and 1.3 µg m−3 compared to flight F0317, respectively. Sulfate aerosol, rather than OA, showed the highest concentration at low altitudes (<1000 m) in both flights F0317 and F0319 resulting from the continental outflow in the ECS. The transport of BB aerosols from Indochina and its impacts on the downstream area were evaluated using a Weather Research Forecasting with Chemistry (WRF-Chem) model. The modeling results tended to overestimate the concentration of the species, with examples being CO (64 ppb), OA (0.3 µg m−3), BC (0.2 µg m−3), and O3 (12.5 ppb) in the BPTL. Over the ECS, the simulated BB contribution demonstrated an increasing trend from the lowest values on 17 March 2018 to the highest values on 18 and 19 March 2018 for CO, fine particulate matter (PM2.5), OA, BC, hydroxyl radicals (OH), nitrogen oxides (NOx), total reactive nitrogen (NOy), and O3; by contrast, the variation of J(O1D) decreased as the BB plume's contribution increased over the ECS. In the lower boundary layer (<1000 m), the BB plume's contribution to most species in the remote downstream areas was <20 %. However, at the BPTL, the contribution of the long-range transported BB plume was as high as 30 %–80 % for most of the species (NOy, NOx, PM2.5, BC, OH, O3, and CO) over southern China (SC), Taiwan, and the ECS. BB aerosols were identified as a potential source of cloud condensation nuclei, and the simulation results indicated that the transported BB plume had an effect on cloud water formation over SC and the ECS on 19 March 2018. The combination of BB aerosol enhancement with cloud water resulted in a reduction of incoming shortwave radiation at the surface in SC and the ECS by 5 %–7 % and 2 %–4 %, respectively, which potentially has significant regional climate implications.

Understanding temporal coherence in particulate matter (PM) pollution across East Asian outflow regions is crucial for collaborative efforts in addressing air pollution challenges. In this study, we analyze daily PM exceedance patterns using ground-based measurements over the past two decades, focusing on the influence of El Niño-Southern Oscillation (ENSO) and Asian dust activity. ENSO-related coherent PM exceedance shows lower occurrence during El Niño compared to La Niña in spring, due to weakened continental outflows and increased precipitation. Temporal distribution of dust-related coherent PM exceedance closely mirrors springtime dust activity in source regions, indicating significant dust emission impact on outflow regions. Furthermore, COVID-19 restrictions likely contributed to decreased PM levels in the spring of 2020. Our findings have implications for climate variability and the assessment of multi-decade model simulations.

No abstract

&lt;p&gt;&amp;#160;Air pollution is typically at its lowest in Taiwan during summer. The mean concentrations of PM&lt;sub&gt;10&lt;/sub&gt;, PM&lt;sub&gt;2.5&lt;/sub&gt;, and daytime ozone (08:00&amp;#8211;17:00 LST) during summer (June&amp;#8211;August) over central Taiwan are 35&amp;#8211;40 &amp;#181;g m&lt;sup&gt;-3&lt;/sup&gt;, 18&amp;#8211;22 &amp;#181;g m&lt;sup&gt;-3&lt;/sup&gt;, and 30&amp;#8211;42 ppb, respectively, between 2004 and 2019. Sampling analysis revealed that the contribution of organic carbon (OC) in PM&lt;sub&gt;2.5&lt;/sub&gt; could exceed 30% in urban and inland mountain sites during July in 2017 and 2018. Frequent episodes of air quality deterioration occur over the western plains of Taiwan when an easterly typhoon circulation interacts with the complex topographic structure of the island. We explored an episode of air quality deterioration that was associated with a typhoon between 15 and 17 July 2018, using the Weather Research Forecasting with Chemistry (WRF-Chem) model. The results indicated that the continual formation of low-pressure systems or typhoons in the area between Taiwan and Luzon island in the Philippines provided a strong easterly ambient flow, which lasted for an extended period between 15 and 17 July. The interaction between the easterly flow and Taiwan&amp;#8217;s Central Mountain Range (CMR) resulted in stable weather conditions and weak wind speed in western Taiwan during the study period. Numerical modeling also indicated that a lee side vortex easily formation and the wind direction could be changed from southwesterly to northwesterly over central Taiwan because of the interaction between the typhoon circulation and the CMR. The northwesterly wind coupled with a sea breeze was conducive to the transport of air pollutants, from the coastal upstream industrial and urban areas to the inland area. The dynamic process for the wind direction changed given a reasonable explanation why the observed SO&lt;sub&gt;4&lt;/sub&gt;&lt;sup&gt;2-&lt;/sup&gt; became the major contributor to PM&lt;sub&gt;2.5&lt;/sub&gt; during the episode. SO&lt;sub&gt;4&lt;/sub&gt;&lt;sup&gt;2-&lt;/sup&gt; contribution proportions (%) to PM&lt;sub&gt;2.5&lt;/sub&gt; at the coastal, urban, and mountain sites were 9.4 &amp;#181;g m&lt;sup&gt;-3&lt;/sup&gt; (30.5%), 12.1 &amp;#181;g m&lt;sup&gt;-3&lt;/sup&gt; (29.9%), and 11.6 &amp;#181;g m&lt;sup&gt;-3&lt;/sup&gt; (29.7%), respectively. Moreover, the variation of the boundary layer height had a strong effect on the concentration level of both PM&lt;sub&gt;2.5&lt;/sub&gt; and ozone. The combination of the lee vortex and land-sea breeze, as well as the boundary layer development, were the key mechanisms in air pollutants accumulation and transport. As typhoons frequently occur around Taiwan during summer and fall, and their effect on the island&amp;#8217;s air quality merits further research attention.&lt;/p&gt;