New experimental and theoretical results for the material parameter reconstruction using terahertz (THz) pulsed spectroscopy (TPS) are presented. The material parameter reconstruction algorithm was realized and experimentally implemented to study the test sample. In order to both verify the algorithm and to estimate the reconstruction accuracy, test sample material parameters obtained with the TPS were compared with the results of the same sample studying by the use of the backward-wave oscillator (BWO) spectroscopy. Thus, high reconstruction accuracy was demonstrated for the spectral range, corresponding to the BWO sensitivity and located between 0.2 and 1.2 THz. The numerical simulations were applied for determining the material parameter reconstruction stability in the presence of white Gaussian noise in TPS waveforms as well as fluctuations in the femtosecond (FS) optical pulse duration. We report a strong dependence of the inverse problem solution stability on these factors. We found that the instability of the FS optical pulse duration used for THz pulses generation and detection limits the material parameter reconstruction with TPS.

Mid‐infrared materials antireflection is in high demand for high‐powered or ultra‐broadband coherent light sources, where conventional antireflection coatings cannot be reliably applied. This work provides a critical review of the recent advances in microstructure fabrication technology for mid‐infrared antireflection applications. Several techniques are reviewed, including direct imprinting, wet and reactive ion etching using conventional photoresist masking, novel colloid crystal masks, and maskless etching, laser‐induced periodic structure formation, and multiple laser ablation method modifications, including femtosecond laser direct writing, direct laser interference ablation, and single pulse ablation. The advantages and drawbacks of the different approaches are discussed in detail to highlight the most promising techniques for the fabrication of antireflection microstructures capable of achieving 99% transmittance in the 2–16 μm range.

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We report a study on the switching of the generation regimes in a high-powered thulium-doped all-fiber ring oscillator that is passively mode-locked with nonlinear polarization evolution technique with different pumping rates and cavity dispersion values. In one experimental setup, switching was observed between the noise-like pulse and the multi-soliton (in the forms of soliton bunches and soliton rain) regimes by the adjustment of the intracavity polarization controllers. We attributed this to the crucial influence of the nonlinear polarization evolution strength determined by such key parameters as saturation (over-rotation) power, linear phase bias, and nonlinear losses on the pulse evolution and stability. So the soliton collapse effect (leading to noise-like pulse generation) or the peak power clamping effect (generating a bunch of loosely-bound solitons) may determine pulse dynamics. Both the spectrum bandwidth and coherence time were studied for noise-like pulses by varying the cavity length and pump power, as well as the duration of solitons composing bunches. As a result, both noise-like pulses (with spectrum as broad as 32 nm bandwidth) and multi-soliton formations (with individual pulse-widths ranging from 748 to 1273 fs with a cavity length increase from 12 to 53 m) with up to 730 mW average power were generated at a wavelength of around 1.9 μm. The results are important for the realization of the broadband and smooth supercontinuum which can be used as a source for mid-IR vibrational spectroscopy of gas samples for breath analysis and environmental sensing.

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We report for the first time to the best of our knowledge on the ultra-short pulse (USP) generation in the dispersion-managed erbium-doped all-fiber ring laser hybridly mode-locked with boron nitride-doped single-walled carbon nanotubes in the co-action with a nonlinear polarization evolution in the ring cavity with a distributed polarizer. Stable 92.6 fs dechirped pulses were obtained via precise polarization state adjustment at a central wavelength of 1560 nm with 11.2 mW average output power, corresponding to the 2.9 kW maximum peak power. We have also observed the laser switching from a USP generation regime to a chirped pulse one with a corresponding pulse-width of 7.1 ps at the same intracavity dispersion.

Ultrafast Tm-doped fibre lasers have been actively studied for the last decade due to their potential applications in precise mid-IR spectroscopy, LIDARs, material processing and more. The majority of research papers is devoted to the comparison between a numerical modelling and experimental results; however, little attention is being paid to the comprehensive description of the mathematical models and parameters of the active and passive components forming cavities of Tm-doped all-fibre lasers. Thus, here we report a numerical model of a stretched-pulsed Tm-doped fibre laser with hybrid mode-locking and compare it with experimental results. The key feature of the developed numerical model is employment of the experimentally measured dispersion coefficients and optimisation of some model parameters, such as the bandwidth of the spectral filter spectral filtering and the saturation power of the active fibre, for a conformity with the experiment. The developed laser emits 331.7 fs pulses with a 23.8 MHz repetition rate, 6 mW of average power, 0.25 nJ of pulse energy, and a 21.66 nm spectral bandwidth at a peak wavelength of 1899.5 nm. The numerical model characteristics coincide with experimentally achieved spectral width, pulse duration, and average power with inaccuracy of 4.7%, 5.4%, and 22.9%, respectively. Moreover, in the discussion of the work the main possible reasons influencing this inaccuracy are highlighted. Elimination of those factors might allow to increase accuracy even more. We show that numerical model has a good agreement with the experiment and can be used for development of ultrafast Tm-doped fibre laser systems.

We report on a comprehensive characterization of Cr 2+-doped CdSe single crystal as an efficient active material for tunable laser applications in the mid-infrared spectral region. Optical gain, thermo-optical behavior, power efficiency, scalability and wavelength tunability have been thoroughly investigated. Using an antireflection-coated crystal pumped by a Tmfiber laser at at 1.94 μm, 1-W CW output power and 50% slope efficiency at 2.65 μm emission wavelength have been obtained in a diffraction-limited output beam. An output peak power of 2.5 W has been achieved without significant beam distortion in a quasi-CW regime. Exploiting an intra-cavity diffraction grating in a Littrow configuration, a maximum tuning range of 900 nm from 2.22 to 3.12 μm, limited by the finite bandwidth of resonator components, has been demonstrated with an uncoated crystal.