A low background gamma spectrometer with an Etruscan, 2500 years old lead shield and a muon veto detector were applied to study 22Na and 7Be activity concentration in ground level air aerosol samples collected weekly over the years 2003–2006 in Kraków. Each sample was formed with ca 100 000 m3 of passed air, collected with two parallel ASS-500 high volume air samplers. The results for 40K and 137Cs are also presented for reference and comparison. Presented frequency distributions for activity concentration and correlation between the obtained results are discussed. The activity concentration results confirmed seasonal variation of activity to be different for all the investigated radionuclides. Moreover, the seasonal variation in nucleus activity ratio was also noticed for 22Na and 7Be. Cosmogenic radionuclides being mainly of stratospheric origin, are subsequently attached to fine aerosols, via which they are transported to the ground level air. The mean aerosol transport time within the troposphere was estimated as equal to 7.5 days on average, reaching even 50 days in warm seasons. Limitations of the applied model were identified.
The appearance of plutonium isotopes in the environment was connected with the human activity, mainly: nuclear weapon tests (global fallout), nuclear accident in Chernobyl (1986), disintegration of satellite SNAP 9 (1963) and releases from nuclear reprocessing factories. At present, the concentration of plutonium in the atmosphere is very small but still observable.The aim of the study is to report and to discuss the results of plutonium alpha-emitters determination from sampling aerosols in air (Krakow 1990–1998, 2001–2002 and Bialystok 1996–1998, 2001) and in precipitation (Krakow 2005–2006). Plutonium activity concentration in air samples (in Krakow and Bialystok) varied in range: 0.22±0.04 nBq/mOne of the mechanisms responsible for the airborne plutonium is resuspension but on the other hand the main source of plutonium in the air seems to be marines aerosols from North See. This new hypothesis will be checked during the future research. The most interesting finding is the seasonal variation of plutonium air concentration. The conclusion from calculated ratio of plutonium isotopes (
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