We have developed a technique for defect reduction in GaN epitaxial films grown on sapphire substrates. This technique relies on the generation of high densities of embedded microvoids (∼108/cm2), a few microns long and less than a micron in diameter. These voids are located near the sapphire substrate, where high densities of dislocations are present. Network of embedded voids offer free surfaces that act as dislocation sinks or termination sites for the dislocations generated at the GaN/sapphire interface. Both transmission electron and atomic force microscopy results confirm the uniform reduction of the dislocation density by two orders of magnitude.
Gamma‐rays (γ‐rays), wherever present, e.g., in medicine, nuclear environment, or homeland security, due to their strong impact on biological matter, should be closely monitored. There is a need for simple, sensitive γ‐ray detectors at affordable prices. Here, it is shown that γ‐ray detectors based on crystals of methylammonium lead tribromide (MAPbBr3) ideally meet these requirements. Specifically, the γ‐rays incident on a MAPbBr3 crystal generates photocarriers with a high mobility‐lifetime product, allowing radiation detection by photocurrent measurements at room temperatures. Moreover, the MAPbBr3 crystal‐based detectors, equipped with improved carbon electrodes, can operate at low bias (≈1.0 V), hence being suitable for applications in energy‐sparse environments, including space. The γ‐ray detectors reported herein are exposed to radiation from a 60Co source at dose rates up to 2.3 Gy h−1 under ambient conditions for over 100 h, without any sign of degradation. The excellent radiation tolerance stems from the intrinsic structural plasticity of the organic–inorganic halide perovskites, which can be attributed to a defect‐healing process by fast ion migration at the nanoscale level. The sensitivity of the γ‐ray detection upon volume is tested for MAPbBr3 crystals reaching up to 1000 cm3 (3.3 kg in weight) grown by a unique crystal growth technique.
We report on the electrical field control of ferromagnetism ͑FM͒ at room temperature in III-N dilute magnetic semiconductor ͑DMS͒ films. A GaMnN layer was grown on top of an n-GaN substrate and found to be almost always paramagnetic. However, when grown on a p-type GaN layer, a strong saturation magnetization ͑M s ͒ was observed. This FM in GaMnN can be controlled by depletion of the holes in the GaMnN/p-GaN/n-GaN multilayer structures. We have demonstrated the dependence of the FM on the thickness of the p-GaN in this heterostructure and on the applied bias to the GaN p-n junction. The M s was measured by an alternating gradient magnetometer ͑AGM͒ and a strong correlation between the hole concentration near the GaMnN/p-GaN interface and the magnetic properties of the DMS was observed. At room temperature an anomalous Hall effect was measured for zero bias and an ordinary Hall effect for reverse bias in a fully depleted p-GaN layer. This is in close agreement with the AGM measurement results.
Abstract-The present article is an overview of developments and results regarding neutron noise measurements in current mode at the CROCUS zero power facility. Neutron noise measurements offer a non-invasive method to determine kinetic reactor parameters such as the prompt decay constant at criticality α = βeff / Λ, the effective delayed neutron fraction βeff, and the mean generation time Λ for code validation efforts. At higher detection rates, i.e. above 2×10 4 cps in the used configuration at 0.1 W, the previously employed pulse charge amplification electronics with BF3 detectors yielded erroneous results due to dead time effects. Future experimental needs call for higher sensitivity in detectors, higher detection rates or higher reactor powers, and thus a generally more versatile measurement system. We, therefore, explored detectors operated with current mode acquisition electronics to accommodate the need. We approached the matter in two ways: 1) By using the two compensated , also within 1σ agreement. The improvements to previous neutron noise measurements include shorter measurement durations that can achieve comparable statistical uncertainties and measurements at higher detection rates.
An advanced neutron detection system for highly localized measurements in nuclear reactor cores was developed and tested in the Laboratory for Reactor Physics and System Behaviour (LRS) at the École polytechnique fédérale de Lausanne (EPFL), Switzerland, in close collaboration with the Detector group of the Laboratory for Particle Physics (LTP) at the Paul Scherrer Institute (PSI), Switzerland. The miniature-size detector is based on the coupling of a ZnS:6LiF scintillator/converter screen of 1 mm2 and 0.2 mm thickness with a 10-m optical fiber, the latter being connected to a silicon photomultiplier (SiPM). In this development version, the output signal is processed via analog read-out electronics. The present work documents the characterization of a detection system prototype in the mixedradiation fields o f t he C ARROUSEL f acility a nd i ts t esting in the CROCUS zero-power reactor operated at LRS. The fibercoupled scintillator shows a linear response with the reactor power increase up to 6.5 W (i.e. around 108 cm-2s-1 total neutron flux), with a s ubsequent l oss o f l inearity d ue t o e lectronic dead time of the analog system. Nevertheless, the detector shows excellent neutron counting capabilities whether compared to other localized detection systems available at LRS, e.g. miniature fission chambers and an sCVD diamond detector.
Interest in fast and easy detection of high-energy radiation (x-, γ-rays and neutrons) is closely related to numerous practical applications ranging from biomedicine and industry to homeland security issues. In this regard, crystals of hybrid halide perovskite have proven to be excellent detectors of x- and γ-rays, offering exceptionally high sensitivities in parallel to the ease of design and handling. Here, we demonstrate that by assembling a methylammonium lead tri-bromide perovskite single crystal (CH3NH3PbBr3 SC) with a Gadolinium (Gd) foil, one can very efficiently detect a flux of thermal neutrons. The neutrons absorbed by the Gd foil turn into γ-rays, which photo-generate charge carriers in the CH3NH3PbBr3 SC. The induced photo-carriers contribute to the electric current, which can easily be measured, providing information on the radiation intensity of thermal neutrons. The dependence on the beam size, bias voltage and the converting distance is investigated. To ensure stable and efficient charge extraction, the perovskite SCs were equipped with carbon electrodes. Furthermore, other types of conversion layers were also tested, including borated polyethylene sheets as well as Gd grains and Gd2O3 pellets directly engulfed into the SCs. Monte Carlo N-Particle (MCNP) radiation transport code calculations quantitatively confirmed the detection mechanism herein proposed.
The present article describes the preliminary design studies for PETALE (Programme d’Etude en Transmission de l’Acier Lourd et ses Eléments), an oncoming experimental program in the CROCUS reactor. Within the framework of the Venus-Eole-Proteus collaboration, PETALE continues the nuclear data validation efforts required for modeling GEN-III pressurized water reactors with heavy steel reflectors. The inelastic scattering cross sections at around 1 MeV of iron-56, as well as nickel and chromium isotopes, will be studied separately. The water reflector will be replaced successively by sheets of stainless steel alloy and pure metals—iron, nickel, and chromium. Data will be extracted from two sources: the measured neutron flux attenuation using adequate dosimetry and possibly fission chambers in the metal reflector and from the criticality effects of these reflectors. PETALE will also be used with nuclear data adjustment methods because, as a separated and elemental integral experiment, it allows the limiting of compensation effects in the nuclear data adjustments. A parametric study has been carried out with MCNPX for assessing the optimal configuration and the feasibility of the experiments. This study is the first step toward optimizing the global sensitivity of the experiments to the reactions in the energy range of interest, thus assessing the measurements’ target uncertainties and preparing further use of the program results.
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