Gamma‐rays (γ‐rays), wherever present, e.g., in medicine, nuclear environment, or homeland security, due to their strong impact on biological matter, should be closely monitored. There is a need for simple, sensitive γ‐ray detectors at affordable prices. Here, it is shown that γ‐ray detectors based on crystals of methylammonium lead tribromide (MAPbBr3) ideally meet these requirements. Specifically, the γ‐rays incident on a MAPbBr3 crystal generates photocarriers with a high mobility‐lifetime product, allowing radiation detection by photocurrent measurements at room temperatures. Moreover, the MAPbBr3 crystal‐based detectors, equipped with improved carbon electrodes, can operate at low bias (≈1.0 V), hence being suitable for applications in energy‐sparse environments, including space. The γ‐ray detectors reported herein are exposed to radiation from a 60Co source at dose rates up to 2.3 Gy h−1 under ambient conditions for over 100 h, without any sign of degradation. The excellent radiation tolerance stems from the intrinsic structural plasticity of the organic–inorganic halide perovskites, which can be attributed to a defect‐healing process by fast ion migration at the nanoscale level. The sensitivity of the γ‐ray detection upon volume is tested for MAPbBr3 crystals reaching up to 1000 cm3 (3.3 kg in weight) grown by a unique crystal growth technique.
An advanced neutron detection system for highly localized measurements in nuclear reactor cores was developed and tested in the Laboratory for Reactor Physics and System Behaviour (LRS) at the École polytechnique fédérale de Lausanne (EPFL), Switzerland, in close collaboration with the Detector group of the Laboratory for Particle Physics (LTP) at the Paul Scherrer Institute (PSI), Switzerland. The miniature-size detector is based on the coupling of a ZnS:6LiF scintillator/converter screen of 1 mm2 and 0.2 mm thickness with a 10-m optical fiber, the latter being connected to a silicon photomultiplier (SiPM). In this development version, the output signal is processed via analog read-out electronics. The present work documents the characterization of a detection system prototype in the mixedradiation fields o f t he C ARROUSEL f acility a nd i ts t esting in the CROCUS zero-power reactor operated at LRS. The fibercoupled scintillator shows a linear response with the reactor power increase up to 6.5 W (i.e. around 108 cm-2s-1 total neutron flux), with a s ubsequent l oss o f l inearity d ue t o e lectronic dead time of the analog system. Nevertheless, the detector shows excellent neutron counting capabilities whether compared to other localized detection systems available at LRS, e.g. miniature fission chambers and an sCVD diamond detector.
The present article presents the mechanical characterization of the fuel rods oscillator developed for the purposes of the COLIBRI experimental program in CROCUS. COLIBRI aims at investigating the radiation noise related to fuel vibrations. The main motivation is the increased amplitudes in the neutron noise distributions recorded in ex- and in-core detectors that have been observed in recent years in Siemens pre-Konvoi type of pressurized water reactors. Several potential explanations have been put forward, but no definitive conclusions could yet be drawn. Among others, changes in fuel assembly or pin vibration patterns, due to recent modifications of assembly structural designs, were pointed out as a possible cause. Computational dynamic tools are currently developed within the Horizon 2020 European project CORTEX, to help with understanding the additional noise amplitude. The COLIBRI program is used for their validation. An in-core device was designed, tested, and licensed between 2015 and 2019 for fuel rods oscillation in CROCUS, in successive steps from out-of-pile tests with dummy fuel rods to critical in-core tests. The characterization of its mechanical behavior is presented, in air and in water, and as a function of the load, for safety and experimental purposes. The device allows simultaneously oscillating up to 18 fuel rods. The maximum oscillation amplitude is 5 mm, while the maximum allowed frequency is 2 Hz, i.e. in the frequency range in which the induced neutron flux fluctuations are most pronounced in nuclear power plants.
Abstract-The present article is an overview of developments and results regarding neutron noise measurements in current mode at the CROCUS zero power facility. Neutron noise measurements offer a non-invasive method to determine kinetic reactor parameters such as the prompt decay constant at criticality α = βeff / Λ, the effective delayed neutron fraction βeff, and the mean generation time Λ for code validation efforts. At higher detection rates, i.e. above 2×10 4 cps in the used configuration at 0.1 W, the previously employed pulse charge amplification electronics with BF3 detectors yielded erroneous results due to dead time effects. Future experimental needs call for higher sensitivity in detectors, higher detection rates or higher reactor powers, and thus a generally more versatile measurement system. We, therefore, explored detectors operated with current mode acquisition electronics to accommodate the need. We approached the matter in two ways: 1) By using the two compensated , also within 1σ agreement. The improvements to previous neutron noise measurements include shorter measurement durations that can achieve comparable statistical uncertainties and measurements at higher detection rates.
The present article describes the preliminary design studies for PETALE (Programme d’Etude en Transmission de l’Acier Lourd et ses Eléments), an oncoming experimental program in the CROCUS reactor. Within the framework of the Venus-Eole-Proteus collaboration, PETALE continues the nuclear data validation efforts required for modeling GEN-III pressurized water reactors with heavy steel reflectors. The inelastic scattering cross sections at around 1 MeV of iron-56, as well as nickel and chromium isotopes, will be studied separately. The water reflector will be replaced successively by sheets of stainless steel alloy and pure metals—iron, nickel, and chromium. Data will be extracted from two sources: the measured neutron flux attenuation using adequate dosimetry and possibly fission chambers in the metal reflector and from the criticality effects of these reflectors. PETALE will also be used with nuclear data adjustment methods because, as a separated and elemental integral experiment, it allows the limiting of compensation effects in the nuclear data adjustments. A parametric study has been carried out with MCNPX for assessing the optimal configuration and the feasibility of the experiments. This study is the first step toward optimizing the global sensitivity of the experiments to the reactions in the energy range of interest, thus assessing the measurements’ target uncertainties and preparing further use of the program results.
The present article gives an overview of the first experimental campaigns carried out in the AKR-2 and CROCUS reactors within the framework of the Horizon 2020 European project CORTEX. CORTEX aims at developing innovative core monitoring techniques that allow detecting anomalies in nuclear reactors, e.g. excessive vibrations of core internals. The technique will be mainly based on using the fluctuations in neutron flux, i.e. noise analysis. The project will result in a deepened understanding of the physical processes involved. This will allow utilities to detect operational problems at a very early stage, and to take proper actions before such problems have any adverse effect on plant safety and reliability. The purpose of the experimental campaigns in the AKR-2 and CROCUS reactors is to produce noise-specific experimental data for the validation of the neutron noise computational models developed within this framework. The first campaigns at both facilities consisted in measurements at reference static states, and with the addition of mechanical perturbations. In the AKR-2 reactor, perturbations were induced by two devices: a rotating absorber and a vibrating absorber, both sets in experimental channels close to the core. In CROCUS, the project benefited from the COLIBRI experimental program: 18 periphery fuel rods were oscillated at a maximum of ±2 mm around their central position in the Hz range. The present article documents the experimental setups and measurements for each facility and perturbation type.
The PETALE experimental programme in the CROCUS reactor intends to provide integral measurements to constrain stainless steel nuclear data. This article presents the tools and the methodology developed to design and optimize the experiments, and its operating principle. Two acceleration techniques have been implemented in the Serpent2 code to perform a Total Monte Carlo uncertainty propagation using variance reduction and correlated sampling technique. Their application to the estimation of the expected reaction rates in dosimeters is also discussed, together with the estimation of the impact of the nuisance parameters of aluminium used in the experiment structures. This is an Open Access article distributed under the terms of the Creative Commons Attribution License (http://creativecommons.org/licenses/by/4.0), which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited. ,
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