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The measurement of SO 2 flux from volcanoes is of major importance for monitoring and hazard assessment purposes, and for evaluation of the environmental impact of volcanic emissions. We propose here a novel technique for accurate and high time resolution estimations of the gas flux. We use two wide field of view UV spectrometers capable of collecting, instantaneously, light from thin parallel cross sections of the whole gas plume, obviating the need for either traversing, scanning or imaging. It enables tracking of inhomogeneities in the gas cloud from which accurate evaluation of the plume velocity can be made by correlation analysis. The method has been successfully applied on Mt. Erebus volcano (Antarctica). It yields estimations of the plume velocity and gas flux at unprecedented time resolution (1 Hz) and high accuracy (uncertainty of 33%). During a ∼2 h experiment on 26 December 2006, SO 2 flux varied between 0.17 and 0.89 ± 0.2 kg s −1 with a vertical plume velocity varying between 1 and 2.5 ± 0.1 m s −1. These

Eruptive activity shapes volcanic edifices. The formation of broad caldera depressions is often associated with major collapse events, emplacing conspicuous pyroclastic deposits. However, caldera subsidence may also proceed silently by magma withdrawal at depth, more difficult to detect. Ambrym, a basaltic volcanic island, hosts a 12-km wide caldera and several intensely-degassing lava lakes confined to intra-caldera cones. Using satellite remote sensing of deformation, gas emissions and thermal anomalies, combined with seismicity and ground observations, we show that in December 2018 an intra-caldera eruption at Ambrym preceded normal faulting with >2 m of associated uplift along the eastern rift zone and 2.5 m of caldera-wide subsidence. Deformation was caused by lateral migration of >0.4 cubic kilometers of magma into the rift zone, extinguishing the lava lakes, and feeding a submarine eruption in the rift edge. Recurring rifting episodes, favored by stress induced by the D’Entrecasteaux Ridge collision against the New Hebrides arc, lead to progressive subsidence of Ambrym’s caldera and concurrent draining of the lava lakes. Although counterintuitive, convergent margin systems can induce rift zone volcanism and subsequent caldera subsidence.

The underwater Hunga Tonga-Hunga Ha-apai volcano erupted in the early hours of 15th January 2022, and injected volcanic gases and aerosols to over 50 km altitude. Here we synthesise satellite, ground-based, in situ and radiosonde observations of the eruption to investigate the strength of the stratospheric aerosol and water vapour perturbations in the initial weeks after the eruption and we quantify the net radiative impact across the two species using offline radiative transfer modelling. We find that the Hunga Tonga-Hunga Ha-apai eruption produced the largest global perturbation of stratospheric aerosols since the Pinatubo eruption in 1991 and the largest perturbation of stratospheric water vapour observed in the satellite era. Immediately after the eruption, water vapour radiative cooling dominated the local stratospheric heating/cooling rates, while at the top-of-the-atmosphere and surface, volcanic aerosol cooling dominated the radiative forcing. However, after two weeks, due to dispersion/dilution, water vapour heating started to dominate the top-of-the-atmosphere radiative forcing, leading to a net warming of the climate system.

Abstract. Depending on the magnitude of their eruptions, volcanoes impact the atmosphere at various temporal and spatial scales. The volcanic source remains a major unknown to rigorously assess these impacts. At the scale of an eruption, the limited knowledge of source parameters, including time variations of erupted mass flux and emission profile, currently represents the greatest issue that limits the reliability of volcanic cloud forecasts. Today, a growing number of satellite and remote sensing observations of distant plumes are becoming available, bringing indirect information on these source terms. Here, we develop an inverse modelling approach combining satellite observations of the volcanic plume with an Eulerian regional chemistry-transport model (CHIMERE) to characterise the volcanic SO2 emissions during an eruptive crisis. The May 2010 eruption of Eyjafjallajökull is a perfect case study to apply this method as the volcano emitted substantial amounts of SO2 during more than a month. We take advantage of the SO2 column amounts provided by a vast set of IASI (Infrared Atmospheric Sounding Interferometer) satellite images to reconstruct retrospectively the time series of the mid-tropospheric SO2 flux emitted by the volcano with a temporal resolution of ~2 h, spanning the period from 1 to 12 May 2010. We show that no a priori knowledge on the SO2 flux is required for this reconstruction. The initialisation of chemistry-transport modelling with this reconstructed source allows for reliable simulation of the evolution of the long-lived tropospheric SO2 cloud over thousands of kilometres. Heterogeneities within the plume, which mainly result from the temporal variability of the emissions, are correctly tracked over a timescale of a week. The robustness of our approach is also demonstrated by the broad similarities between the SO2 flux history determined by this study and the ash discharge behaviour estimated by other means during the phases of high explosive activity at Eyjafjallajökull in May 2010. Finally, we show how a sequential IASI data assimilation allows for a substantial improvement in the forecasts of the location and concentration of the plume compared to an approach assuming constant flux at the source. As the SO2 flux is an important indicator of the volcanic activity, this approach is also of interest to monitor poorly instrumented volcanoes from space.

Abstract. In this paper we combine SO 2 and ash plume dispersion modelling with satellite and surface remote sensing observations to study the regional influence of a relatively weak volcanic eruption from Mount Etna on the optical and micro-physical properties of Mediterranean aerosols. We analyse the Mount Etna eruption episode of 25-27 October 2013. The evolution of the plume along the trajectory is investigated by means of the FLEXible PARTicle Lagrangian dispersion (FLEXPART) model. The satellite data set includes true colour images, retrieved values of volcanic SO 2 and ash, estimates of SO 2 and ash emission rates derived from MODIS (MODerate resolution Imaging Spectroradiometer) observations and estimates of cloud top pressure from SEVIRI (Spinning Enhanced Visible and InfraRed Imager). Surface remote sensing measurements of aerosol and SO 2 made at the ENEA Station for Climate Observations (35.52 • N, 12.63 • E; 50 m a.s.l.) on the island of Lampedusa are used in the analysis. The combination of these different data sets suggests that SO 2 and ash, despite the initial injection at about 7.0 km altitude, reached altitudes around 10-12 km and influenced the column average aerosol particle size distribution at a distance of more than 350 km downwind. This study indicates that even a relatively weak volcanic eruption may produce an observable effect on the aerosol properties at the regional scale. The impact of secondary sulfate particles on the aerosol size distribution at Lampedusa is discussed and estimates of the clear-sky direct aerosol radiative forcing are derived. Daily shortwave radiative forcing efficiencies, i.e. radiative forcing per unit AOD (aerosol optical depth), are calculated with the LibRadtran model. They are estimated between −39 and −48 W m −2 AOD −1 at the top of the atmosphere and between −66 and −49 W m −2 AOD −1 at the surface, with the variability in the estimates mainly depending on the aerosol single scattering albedo. These results suggest that sulfate particles played a large role in the transported plume composition and radiative forcing, while the contribution by ash particles was small in the volcanic plume arriving at Lampedusa during this event.

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