[1] A new method is proposed for the computation of CO 2 Net Ecosystem Exchange (NEE) and its components in a forest ecosystem. Advective flux is estimated by taking into account the air mass conservation principle. For this purpose, wind and dry air density values on the surface of the control volume are first corrected and then the advective flux is estimated on the surface of the control volume. Turbulent flux is also computed along the surface of the control volume while storage flux is computed inside the volume. Additional characteristics of this method are that incompressibility of the mean flow is not assumed a priori, and that vertical and horizontal advective fluxes are not treated separately, but their sum is estimated directly. The methodology is applied to experimental data collected with a three-dimensional scheme at the alpine site of Renon during the Advex project (July 2005). The advection flux was found to be prevailing positive at night and negative during the day, as was found in previous studies on advection for the same site, but showed a lower scatter in half-hour calculated values. We tested the effect of its summation on turbulent and storage fluxes to produce half-hourly values of NEE. Nighttime NEE values were used in functional relations with soil temperature, daytime values with PPFD. The effect of addition of the advection component was an increase in the values of parameters indicating ecosystem respiration, quantum yield, and photosynthetic capacity. The coefficient of correlation between NEE and environmental drivers increased.
The contribution of main PM pollution sources and their geographic origin in three urban sites of the Danube macro-region (Zagreb, Budapest and Sofia) were determined by combining receptor and Lagrangian models. The source contribution estimates were obtained with the Positive Matrix Factorization (PMF) receptor model and the results were further examined using local wind data and backward trajectories obtained with FLEXPART. Potential Source Contribution Function (PSCF) analysis was applied to identify the geographical source areas for the PM sources subject to long-range transport. Gas-to-particle transformation processes and primary emissions from biomass burning are the most important contributors to PM in the studied sites followed by re-suspension of soil (crustal material) and traffic. These four sources can be considered typical of the Danube macro-region because they were identified in all the studied locations. Long-range transport was observed of: a) sulphate-enriched aged aerosols, deriving from SO2 emissions in combustion processes in the Balkans and Eastern Europe and b) dust from the Saharan and Karakum deserts. The study highlights that PM pollution in the studied urban areas of the Danube macro-region is the result of both local sources and long-range transport from both EU and no-EU areas.
h i g h l i g h t s• The model inter-comparison initiative AQMEII is outlined.• The NIMH's WRF-CMAQ model system as designed for AQMEII-2 exercise is described. • Simulations for 2010 over Europe as prepared for the ENSEMBLE tool are described. • O3, NO2 and PM model results are analyzed against surface measurements in ENSEMBLE.
a b s t r a c tThe air quality modeling system WRF-CMAQ was applied to the European domain for the year 2010 in the frame of the Air Quality Model Evaluation International Initiative (AQMEII), Phase 2. The model system was set up for a domain of 5000 × 5000 km 2 size with horizontal resolution of 25km. The emissions at European level were available through AQMEII and further processed in a way to feed the chemistry transport model CMAQ. The meso-meteorological model WRF was driven by NCEP GFS data with 1°×1°resolution. The chemical boundary conditions were extracted from MACC global simulation data. Model performance was investigated by means of AQMEII-2 web based evaluation platform and the monitoring data gathered for this activity. A preliminary model evaluation for ozone, nitrogen dioxide and particulate matter was conducted. The statistical analysis was based on comparison between simulated and observed concentrations at different type of surface stations in the EU wide domain (rural, urban, suburban), as well as for selected four cities. Model performance was characterized by overestimation for ozone and underestimation for the other pollutants. The relative statistical indicators were discussed also in view of recently published performance criteria.
In spite of recent progress in the prognostic numerical simulation of the atmospheric boundary layer, the explicit simulation of turbulent flows in actual complex terrain is generally still very complicated and time consuming for many environmental applications.In an attempt to develop simpler and more efficient application oriented techniques, although less refined, we propose a multi-step procedure for simulating wind fields. Once obtained the necessary meteorological input, the mass-consistent modelling technique is used to perform high-resolution mean wind flow simulations taking into account recent developments in the atmospheric boundary-layer theory. Besides, a procedure based on a generalisation of the local logarithmic law-of-the-wall over complex terrain is used to estimate the effective parameters characterising the simulated wind profiles. Turbulence intensities and spectral properties are then calculated through the estimated effective parameters, in particular through the effective friction velocity parameter. Finally, time series of the instantaneous velocity field are simulated by the Monte Carlo technique. Two applications of the proposed approach are discussed briefly: the first one is related to a coastal area in southern Italy (the Messina Straits), where the construction of the world's longest central span bridge is being planned; the second one corresponds to the flow in a mountainous area in northern Italy (the Albenga Airport).
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