Two-dimensional (2D) graphene (GRA) and polyaniline (C 3 N) monolayers are attracting growing research interest due to their excellent electrical and thermal properties. In this work, in-plane and out-of-plane phonon thermal conduction of GRA-C 3 N heterobilayer are systematically investigated by using classical molecular dynamics simulations. Effects of system size, temperature and interlayer coupling strength on the in-plane thermal conductivity (k) and out-of-plane interfacial thermal resistance (R) are evaluated. Firstly, a monotonic increasing trend of k with increasing system size is observed, while a negative correlation between thermal conductivity and temperature is revealed. The interlayer coupling strength is found to have a weak effect on the in-plane thermal conductivity of the heterobilayer. Secondly, at T=300 K and χ=1, the predicted R of GRA→C 3 N and C 3 N→GRA are 1.29×10 −7 K m 2 W −1 and 1.35×10 −7 K m 2 W −1 , respectively, which indicates that there is no significant thermal rectification phenomenon. It can also be observed that R decreases monotonically with increasing temperature and coupling strength due to the enhanced Umklapp phonon scattering and the phonon transmission probability across the interface. Phonon density of states, phonon dispersions and participation ratios are evaluated to reveal the mechanism of heat conduction in the heterobilayer. This work contributes the valuable thermal information to modulate the phonon behaviors in 2D heterobilayer based nanoelectronics.
The complex [(PNHP)Fe(H)(CO)(HBH)] (PNHP = HN(CHCHPi-Pr)) serves as a catalyst precursor for the selective dehydrocoupling of methylamine borane at room temperature, tentatively via an off-metal polymerisation pathway.
Visible-light-responsive reversible color-switching systems are attractive to many applications because visible light has superior penetration and causes far less damage to organic molecules than UV. Herein, we report that self-doping of SnO nanocrystals with Sn red-shifts their absorption to the visible region and simultaneously produces oxygen vacancies, which can effectively scavenge photogenerated holes and thus enable the color switching of redox dyes using visible light. Wavelength-selective switching can also be achieved by coupling the photocatalytic activity of the SnO NCs with the color-switching kinetics of different redox dyes. The fast light response enables the further fabrication of a solid film that can be repeatedly written on using a visible laser pen or projection printing through a photomask. This discovery represents a big step forward towards practical applications, especially in areas in which safety issues and photodamage by UV light are of concern.
An integration of an electric motor and a drive with wide-bandgap (WBG) devices possesses numerous attractive features for electrified and decentralized actuation systems. The WBG devices can operate at a high-junction temperature (>170°C) with improved efficiency due to fast switching speed and low on-state resistance. It also leads to better performance and higher power density electro-hydrostatic actuators (EHAs) than the traditional solutions, which are being widely adopted in industrial applications such as aerospace, robotics, automobiles, manufacturing, wind turbine, and off-road vehicles. This paper introduces and investigates the benefits of the integrated motor drive with the WBG-based power electronics for the EHA systems.
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