Simulation of stratospheric tracers using an improved empirically based two‐dimensional model transport formulation

Abstract

Abstract. We have developed a new empirically based transport formulation for use in our Goddard Space Flight Center (GSFC) two-dimensional chemistry and transport model. In this formulation, we consider much of the information about atmospheric transport processes available from existing data sets. This includes zonal mean temperature, zonal wind, net heating rates, and Eliassen-Palm flux diagnostics for planetary and synoptic-scale waves. We also account for the effects of gravity waves and equatorial Kelvin waves by utilizing previously developed parameterizations in which the zonal mean flow is constrained to observations. This scheme utilizes significantly more information compared to our previous formulation and results in simulations that are in substantially better agreement with observations. The new model transport captures much of the qualitative structure and seasonal variability observed in stratospheric long lived tracers, such as isolation of the tropics and the southern hemisphere winter polar vortex, the well-mixed surf-zone region of the winter subtropics and midlatitudes, and the latitudinal and seasonal variations of total ozone. Model simulations of carbon 14 and strontium 90 are in good agreement with observations, capturing the peak in mixing ratio at 20-25 km and the decrease with altitude in mixing ratio above 25 kin. We also find mostly good agreement between modeled and observed age of air determined from SFc outside of the northern hemisphere polar vortex. However, inside the vortex, the model simulates significantly younger air compared to observations. This is consistent with the model deficiencies in simulating CH4 in this region and illustrates the limitations of the current climatological zonal mean model formulation. The model correctly propagates the phase of the lower stratospheric seasonal cycles in 2CH4+H20 and CO2. The model also qualitatively captures the observed decrease in the amplitude of the stratospheric COe seasonal cycle between the tropics and midlatitudes. However, the simulated seasonal amplitudes were attenuated too rapidly with altitude in the tropics. The generally good model-measurement agreement of these tracer simulations demonstrate that a successful formulation of zonal mean transport processes can be constructed from currently available atmospheric data sets.

Methane as a diagnostic tracer of changes in the Brewer–Dobson circulation of the stratosphere

“…CH 4 , exhibit distributions that are well correlated and vary seasonally in response to changes in the BDC (Plumb and Ko, 1992;Holton, 1986). Figure 2 is an example of the zonally averaged distribution of CH 4 for January from a NASA/Goddard, two-dimensional chemistry and transport model simulation (Fleming et al, 1999). The white arrows show the effects of the stratospheric BDC, which is strong in the winter hemisphere (longer arrows) and weak in the summer stratosphere.…”

Middle atmospheric changes caused by the January and March 2012 solar proton events

“…This model was first discussed over 20 yr ago (Douglass et al, 1989;Jackman et al, 1990) and has undergone extensive improvements over the years (e.g., Considine et al, 1994;Jackman et al, 1996;Fleming et al, 1999Fleming et al, , 2007Fleming et al, , 2011. The vertical range of the model, equally spaced in log pressure, is from the ground to approximately 92 km (0.0024 hPa) with a 1 km grid spacing.…”

Solar geoengineering using solid aerosol in the stratosphere

“…3.5. The model's 2-D transport is prescribed based on calculations by Fleming et al (1999) for each year from 1978 to 2004, employing observed temperature, ozone, water vapor, zonal wind, and planetary waves. Different phases of the quasi-biennial oscillation (QBO) are included in the observational data employed.…”