Pt/Ca x Sr 1−x Bi 2 Ta 2 O 9 (CSBT)/Hf-Al-O(HAO)/Si ferroelectric-gate field-effect transistors (FeFETs) with x = 0, 0.1, 0.2, 0.5 and 1 were fabricated and characterized. As-deposited layer thicknesses of the CSBT and HAO were fixed at 200 nm and 7 nm. The memory window (V w ) values of the FeFETs with the CSBTs of x = 0, 0.1, 0.2 and 0.5 were 0.75 V, 0.89 V, 0.84 V and 0.43 V, respectively, when the gate voltage V g was scanned from −4 to 6 V. The V w values of the FeFETs with x = 0.1 and 0.2 were 19% and 12% larger than those of the FeFET with pure SrBi 2 Ta 2 O 9 (x = 0). The V w of the FeFET with pure CaBi 2 Ta 2 O 9 (x = 1) was almost zero. The Bi-layered perovskite crystalline structure of the CSBTs in the Pt/CSBT/HAO/Si stacks was confirmed by x-ray diffraction pattern characterization. The FeFETs with the CSBTs of x = 0.1 and 0.2 showed good retention characteristics measured for at least 4.6 days and high endurance performance over 10 8 cycles.