Energetic charged particles have been measured in the bombardment of 150-keV deuterons on deuterated Ti. Protons and α particles were observed with energies up to ~17 and ~6.5 MeV, respectively, which can never be attained in the D+D reaction. A bump structure at around 14 MeV seen in the proton spectrum can be well explained as emitted in the sequential reaction involving three deuterons. However, protons and α particles distributed continuously up to the maximum energies can never be understood as products of the conceivable nuclear reactions.KEYWORDS: D+D reaction in Ti, high energy proton emission, α-particle emission, 3D reactions, sequential reaction §1. IntroductionIn a series of experiments on bombardments of low energy deuterons on deuterated Ti for a study of the low energy D + D reaction in metal, we have observed energetic charged particles which cannot be explained as emitted in usual nuclear reactions. They are protons with energies up to ~17 MeV and α particles with energies up to ~6.5 MeV. In this paper, we point out how the observed energy spectra indicate that a reaction involving three deuterons occurs in the bombardment; a bump seen in the proton spectra can be well understood, whereas the mechanism of emitting the continuous protons and α particles is not completely clear at present time.
§2. ExperimentTargets were prepared as follows. D 2 gas was absorbed by various Ti rods (99.5% Ti; 10, 8, and 6 mm in diameter and 30 mm in length) and plates (10 mm × 30 mm × 2 mm), which were manufactured by Nippon Mining Co., Ltd. A cylindrical vessel (16 mm in inner diameter and 10 cm in length) made of inconel metal was used for the gas absorption, and was set in an electric oven. Typical contaminants in Ti are listed in Table I. The vacuum line was made of stainless steel and was evacuated by a turbo molecular pump. Before admitting D 2 gas, a Ti rod or plate was loaded into a vessel and degassed by heating the vessel at around 800°C in vacuum of 10 -5 Pa for at least 20 hours. After that, the vessel was cooled down to about 600°C and then was filled with the D 2 gas. The system was refilled with the gas again and again until the