2008
DOI: 10.1021/nl802160z
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A High-Temperature Single-Photon Source from Nanowire Quantum Dots

Abstract: We present a high-temperature single-photon source based on a quantum dot inside a nanowire. The nanowires were grown by molecular beam epitaxy in the vapor-liquid-solid growth mode. We utilize a two-step process that allows a thin, defect-free ZnSe nanowire to grow on top of a broader, cone-shaped nanowire. Quantum dots are formed by incorporating a narrow zone of CdSe into the nanowire. We observe intense and highly polarized photoluminescence even from a single emitter. Efficient photon antibunching is obse… Show more

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Cited by 114 publications
(99 citation statements)
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“…A central goal in the active field of fundamental and applied research are semiconductor nanowires (NW). Here, the transfer of these concepts on this one-dimensional platform using axial [4,5] or radial approaches [6,7,8] are of crucial importance. For axial NW based QDs key experiments including ultra-bright single photon emission [9], quasi-static charge state control [10] and optical initialization of spin states [11] clearly underpinned the large potential of these systems.…”
Section: Introductionmentioning
confidence: 99%
“…A central goal in the active field of fundamental and applied research are semiconductor nanowires (NW). Here, the transfer of these concepts on this one-dimensional platform using axial [4,5] or radial approaches [6,7,8] are of crucial importance. For axial NW based QDs key experiments including ultra-bright single photon emission [9], quasi-static charge state control [10] and optical initialization of spin states [11] clearly underpinned the large potential of these systems.…”
Section: Introductionmentioning
confidence: 99%
“…14 Interestingly enough, II-VI QDs defined in thin nanowire display a fast decay dynamics. 27 This behavior could be explained by a longitudinal optical dipole component associated with a-at least partial-light hole character of the exciton.…”
mentioning
confidence: 99%
“…[1][2][3][4][5][6][7][8][9] The integration of QDs in one-dimensional crystals (nanowires, NWs) has increasingly gained interest because of the improvement in the photon extraction efficiency and overall functionality. [10][11][12][13][14][15][16][17][18][19] Recently, it has been shown that self-segregation processes in ternary Al x Ga 1Àx As shells lead to the observation of luminescence stemming from 3D confined excitons. Several high-resolution imaging methods have demonstrated that the Al x Ga 1Àx As shells are indeed not homogeneous and contain nanoscale Ga-rich islands.…”
mentioning
confidence: 99%