In 1963 Glauber introduced the modern theory of quantum coherence 1 , which extended the concept of first-order (onebody) correlations, describing phase coherence of classical waves, to include higher-order (n-body) quantum correlations characterizing the interference of multiple particles. Whereas the quantum coherence of photons is a mature cornerstone of quantum optics, the quantum coherence properties of massive particles remain largely unexplored. To investigate these properties, here we use a uniquely correlated 2 source of atoms that allows us to observe n-body correlations up to the sixthorder at the ideal theoretical limit (n!). Our measurements constitute a direct demonstration of the validity of one of the most widely used theorems in quantum many-body theory-Wick's theorem 3 -for a thermal ensemble of massive particles. Measurements involving n-body correlations may play an important role in the understanding of thermalization of isolated quantum systems 4 and the thermodynamics of exotic many-body systems, such as Efimov trimers 5 .Glauber's modern theory of optical coherence and the famous Hanbury Brown-Twiss effect 6 were pivotal in the establishment of the field of quantum optics. Importantly, the definition of a coherent state required coherence to all orders, which for example distinguishes a monochromatic but incoherent thermal source of light from a truly coherent source such as a laser. Higher-order correlation functions therefore provide a more rigorous test of coherence.Higher-order correlations, characterized by an n-body correlation function g (n) , are of general interest and have been investigated in many fields of physics including astronomy 6 , particle physics 7 , quantum optics 8 , and quantum atom optics 9 . In particular they have been a fruitful area of research in the field of quantum optics, where they have been used to investigate the properties of laser light, including heralded single photons 10 , and the statistics of parametric down-conversion sources 11 . State-of-the-art quantum optics experiments have measured photon correlation functions up to sixth order for quasi-thermal sources 8 , allowing the possibility of performing full quantum state tomography 12 .Higher-order correlations experiments with massive particles are currently approaching the same level of maturity as with photons. So far, experiments have directly observed correlations up to fourth order with single-atom-sensitive detection techniques for ultracold atomic bosons 9,13,14 , and second-order correlations for an atomic source of fermions 15 demonstrating the uniquely quantum mechanical property of atom-atom antibunching. Alternative, indirect techniques have also been employed to investigate higher-order correlations, including the measurements of twobody (photoassociation 16 ) and three-body 17 loss rates that are sensitive, respectively, to second-and third-order correlation functions. Interestingly, fermionic atom pairs 18 and fermionic antibunching 19 have also been observed in the atomic shot no...
The coherence properties of amplified matter waves generated by four-wave mixing (FWM) are studied using the Hanbury-Brown-Twiss method. We examine two limits. In the first case stimulated processes lead to the selective excitation of a pair of spatially separated modes, which we show to be second order coherent, while the second occurs when the FWM process is multimode, due to spontaneous scattering events which leads to incoherent matter waves. Amplified FWM is a promising candidate for fundamental tests of quantum mechanics where correlated modes with large occupations are required.
A fundamental property of a three-dimensional Bose-Einstein condensate is long-range coherence; however, in systems of lower dimensionality, not only is the long-range coherence destroyed but additional states of matter are predicted to exist. One such state is a "transverse condensate," first predicted by van Druten and Ketterle [Phys. Rev. Lett. 79, 549 (1997)], in which the gas condenses in the transverse dimensions of a highly anisotropic trap while remaining thermal in the longitudinal dimension. Here, we detect the transition from a three-dimensional thermal gas to a gas undergoing transverse condensation by probing Hanbury Brown-Twiss correlations.
We consider laser-pumped one-dimensional two-component bosons in a parabolic trap embedded in a high-finesse optical cavity. Above a threshold pump power, the photons that populate the cavity modify the effective atom trap and mediate a coupling between the two components of the Bose-Einstein condensate. We calculate the ground state of the laser-pumped system and find different stages of selforganization depending on the power of the laser. The modified potential and the laser-mediated coupling between the atomic components give rise to rich many-body physics: an increase of the pump power triggers a self-organization of the atoms while an even larger pump power causes correlations between the self-organized atoms-the BEC becomes fragmented and the reduced density matrix acquires multiple macroscopic eigenvalues. In this fragmented superradiant state, the atoms can no longer be described as two-level systems and the mapping of the system to the Dicke model breaks down.
We present here the first measurement of the third-order spatial correlation function for atoms, made possible by cooling a metastable helium cloud to create an ultracold thermal ensemble just above the Bose-Einstein condensation point. The resulting large correlation length well exceeds the spatial resolution limit of the single-atom detection system, and enables extension of our earlier temporal measurements to evaluate the third-order correlation function in the spatial plane of the detector. The enhancement of the spatial third-order correlation function above a value of unity demonstrates the presence of spatial three-atom bunching, as expected for an incoherent source. Contents
We study the effects of strong inter-particle interaction on diffraction of a Bose-Einstein condensate of ^6\mathrm{Li}_26Li2 molecules from a periodic potential created by pulses of a far detuned optical standing wave. For short pulses we observe the standard Kapitza-Dirac diffraction, with the contrast of the diffraction pattern strongly reduced for very large interactions due to interaction-dependent loss processes. For longer pulses diffraction shows the characteristic for matter waves impinging on an array of tubes and coherent channeling transport. We observe a slowing down of the time evolution governing the population of the momentum modes caused by the strong atom interaction. A simple physical explanation of that slowing down is the phase shift caused by the self-interaction of the forming matter wave patterns inside the standing light wave. Simple 1D mean field simulations qualitatively capture the phenomenon, however to quantitatively reproduce the experimental results the molecular scattering length has to be multiplied by factor of 4.2. In addition, two contributions to interaction-dependent degradation of the coherent diffraction patterns were identified: (i) in-trap loss of molecules during the lattice pulse, which involves dissociation of Feshbach molecules into free atoms, as confirmed by radio-frequency spectroscopy and (ii) collisions between different momentum modes during separation. This was confirmed by interferometrically recombining the diffracted momenta into the zero-momentum peak, which consequently removed the scattering background.
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