The Casimir force is the attraction between uncharged metallic surfaces as a result of quantum mechanical vacuum fluctuations of the electromagnetic field. We demonstrate the Casimir effect in microelectromechanical systems using a micromachined torsional device. Attraction between a polysilicon plate and a spherical metallic surface results in a torque that rotates the plate about two thin torsional rods. The dependence of the rotation angle on the separation between the surfaces is in agreement with calculations of the Casimir force. Our results show that quantum electrodynamical effects play a significant role in such microelectromechanical systems when the separation between components is in the nanometer range.
The Casimir force between uncharged metallic surfaces originates from quantum mechanical zero point fluctuations of the electromagnetic field. We demonstrate that this quantum electrodynamical effect has a profound influence on the oscillatory behavior of microstructures when surfaces are in close proximity (≤ 100 nm). Frequency shifts, hysteretic behavior and bistability caused by the Casimir force are observed in the frequency response of a periodically driven micromachined torsional oscillator.
Microelectromechanical systems (MEMS) incorporating active piezoelectric layers offer integrated actuation, sensing, and transduction. The broad implementation of such active MEMS has long been constrained by the inability to integrate materials with giant piezoelectric response, such as Pb(Mg(1/3)Nb(2/3))O(3)-PbTiO(3) (PMN-PT). We synthesized high-quality PMN-PT epitaxial thin films on vicinal (001) Si wafers with the use of an epitaxial (001) SrTiO(3) template layer with superior piezoelectric coefficients (e(31,f) = -27 ± 3 coulombs per square meter) and figures of merit for piezoelectric energy-harvesting systems. We have incorporated these heterostructures into microcantilevers that are actuated with extremely low drive voltage due to thin-film piezoelectric properties that rival bulk PMN-PT single crystals. These epitaxial heterostructures exhibit very large electromechanical coupling for ultrasound medical imaging, microfluidic control, mechanical sensing, and energy harvesting.
The atomic force microscope (AFM) offers a rich observation window on the nanoscale, yet many dynamic phenomena are too fast and too weak for direct AFM detection. Integrated cavity-optomechanics is revolutionizing micromechanical sensing; however, it has not yet impacted AFM. Here, we make a groundbreaking advance by fabricating picogram-scale probes integrated with photonic resonators, to realize functional AFM detection that achieve high temporal resolution (< 10 ns) and picometer vertical displacement uncertainty, simultaneously. The ability to capture fast events with high precision is leveraged to measure the thermal conductivity (η), for the first time, concurrently with chemical composition at the nanoscale in photothermal induced resonance experiments. The intrinsic η of metal-organic-framework individual microcrystals, not measurable by macroscale techniques, is obtained with a small measurement uncertainty (8 %). The improved sensitivity (50×) increases the measurement throughput 2500-fold and enables chemical composition measurement of molecular-monolayer-thin samples. Our paradigm-shifting photonic readout for small probes breaks the common tradeoff between AFM measurement precision and ability to capture transient events, thus transforming the ability to observe nanoscale dynamics in materials.
The collective oscillation of conduction electrons, responsible for the localized surface plasmon resonances, enables engineering nanomaterials by tuning their optical response from the visible to terahertz as a function of nanostructure size, shape, and environment. While theoretical calculations helped tremendously in understanding plasmonic nanomaterials and optimizing their light matter interaction, only a few experimental techniques are available to study these materials with high spatial resolution. In this work, the photothermal-induced resonance (PTIR) technique is applied for the first time to image the dark plasmonic resonance of gold asymmetric split ring resonators (A-SRRs) in the mid-infrared (IR) spectral region with nanoscale resolution. Additionally, the chemically specific PTIR signal is used to map the local absorption enhancement of poly(methyl methacrylate) coated on A-SRRs, revealing hot spots with local enhancement factors up to ≈30 at 100 nm lateral resolution. We argue that PTIR nanoscale characterization will facilitate the engineering and application of plasmonic nanomaterials for mid-IR applications.
We demonstrate optomechanically-mediated electromagnetically-induced transparency and wavelength conversion in silicon nitride (Si3N4) microdisk resonators. Fabricated devices support whispering gallery optical modes with a quality factor (Q) of 10 6 , and radial breathing mechanical modes with a Q=10 4 and a resonance frequency of 625 MHz, so that the system is in the resolved sideband regime. Placing a strong optical control field on the red (blue) detuned sideband of the optical mode produces coherent interference with a resonant probe beam, inducing a transparency (absorption) window for the probe. This is observed for multiple optical modes of the device, all of which couple to the same mechanical mode, and which can be widely separated in wavelength due to the large bandgap of Si3N4. These properties are exploited to demonstrate frequency upconversion and downconversion of optical signals between the 1300 nm and 980 nm bands with a frequency span of 69.4 THz.Recent demonstrations of strong radiation pressure interactions in cavity optomechanics have focused on the resolved sideband regime, where mechanical sidebands of the optical mode lie outside its linewidth [1]. Such systems have been used in laser cooling a mechanical oscillator to its ground state [2,3], coherent interference effects such as electromagnetically-induced transparency (EIT) [4,5], parametrically-driven normal mode splitting [6][7][8], and observing energy exchange between the optical and mechanical systems [8,9]. Here, we study a system consisting of a small diameter silicon nitride (Si 3 N 4 ) microdisk in which multiple high quality factor optical modes couple to a 625 MHz mechanical radial breathing mode. We demonstrate optomechanicallymediated EIT and wavelength conversion [10][11][12][13], upand downconverting signals across the widely separated 1300 nm and 980 nm wavelengths bands. Our results establish Si 3 N 4 as a viable platform for chip-scale cavity optomechanics in the resolved sideband regime. More generally, Si 3 N 4 offers potential integration of cavity optomechanics with numerous classical and quantum photonic elements, including ultra-low-loss passive components [14], microcavity frequency combs [15] and spectrally narrow mode-locked lasers [16], and integrated superconducting single photon detectors [17].In the context of chip-scale guided wave devices, experiments making use of frequency-resolved mechanical sidebands have largely been in two systems exhibiting significantly different parameter regimes: silica microtoroid cavities [4,8] and silicon photonic and phononic crystal resonators (optomechanical crystals) [3,5,18]. Silica microtoroids support ultra-high quality factor optical modes (Q o >10 7 , decay rate κ/2π≈10 MHz) that are coupled to > ∼ 50 MHz frequency mechanical modes with a zero-point optomechanical coupling rate g 0 /2π > ∼ 1 kHz.In contrast, silicon optomechanical crystals have Q o ≈ 10 6 (κ/2π > ∼ 200 MHz) modes that couple to few GHz mechanical modes with g 0 /2π≈1 MHz. Though similar physics has ...
The Casimir force between bodies in vacuum can be understood as arising from their interaction with an infinite number of fluctuating electromagnetic quantum vacuum modes, resulting in a complex dependence on the shape and material of the interacting objects. Becoming dominant at small separations, the force has a significant role in nanomechanics and object manipulation at the nanoscale, leading to a considerable interest in identifying structures where the Casimir interaction behaves significantly different from the well-known attractive force between parallel plates. Here we experimentally demonstrate that by nanostructuring one of the interacting metal surfaces at scales below the plasma wavelength, an unexpected regime in the Casimir force can be observed. Replacing a flat surface with a deep metallic lamellar grating with sub-100 nm features strongly suppresses the Casimir force and for large inter-surfaces separations reduces it beyond what would be expected by any existing theoretical prediction.
Photothermal induced resonance (PTIR), also known as AFM-IR, is a scanning probe technique that provides sample composition information with a lateral resolution down to 20 nm. Interest in PTIR stems from its ability to identify unknown samples at the nanoscale thanks, in first approximation, to the direct comparability of PTIR spectra with far-field infrared databases. The development of rapidly tuning quantum cascade lasers has increased the PTIR throughput considerably, making nanoscale hyperspectral imaging within a reasonable time frame possible. Consequently, a better understanding of PTIR signal generation and of the fine details of PTIR analysis has become of paramount importance for extending complex IR analysis methods developed in the far-field, e.g., for classification and hyperspectral imaging, to nanoscale PTIR spectra. Here we calculate PTIR spectra via thin-film optics, to identify subtle changes (band shifts, deviation from linear approximation, etc.) for common sample parameters in the case of PTIR with total internal reflection illumination. Results show signal intensity linearity and small band shifts as long as the sample is prepared correctly, with band shifts typically smaller than macroscale attenuated total reflection (ATR) spectroscopy. Finally, a generally applicable algorithm to retrieve the pure imaginary component of the refractive index (i.e., the chemically specific information) is provided to overcome the PTIR spectra nonlinearity.
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