Anomalous thermal transition and crystallization behaviors of three room temperature ionic liquids (RTILs) in graphene multilayers (GMLs), in a different manner to bulk RTILs, occurred due to the molecular orientation of the confined system triggered by the complex π-π stacking and hydrogen bonding interactions.
The reduced graphene oxides (RGOs) functionalized by pyridinium-based ionic liquids (ILs) with SCN anions revealed 6-fold higher capacitance compared to that of RGOs due to the redox behavior of ILs as well as good rate capability and cycle stability despite the appearance of pseudo-capacitance.
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