Stretchable electroluminescent device is a compliant form of light-emitting device to expand the application areas of conventional optoelectronics on rigid wafers. Currently, practical implementations are impeded by the high operating voltage required to achieve sufficient brightness. In this study, we report the fabrication of an intrinsically stretchable electroluminescent device based on silver nanowire electrodes and high-k thermoplastic elastomers. The device exhibits a bright emission with a low driving voltage by using polar elastomer as a dielectric matrix of the electroluminescent layer. Highly stretchable silver nanowire electrodes contribute to the exceptional elasticity and durability of the device in spite of bending, stretching, twisting, puncturing, and cutting. Stretchable electroluminescent devices developed here may find potential uses in wearable displays, deformable lightings, and soft robotics.
Stretchable alternating current electroluminescent display is an emerging form of light-emitting device by combining elasticity with optoelectronic properties. The practical implementations are currently impeded by the high operating voltages required to achieve sufficient brightness. In this study, we report the development of dielectric nanocomposites by filling surface-modified ceramic nanoparticles into polar elastomers, which exhibit a series of desirable attributes, in terms of high permittivity, mechanical deformability, and solution processability. Dielectric nanocomposite effectively concentrates electric fields onto phosphor to enable low-voltage operation of stretchable electroluminescent display, thereby alleviating safety concerns toward wearable applications. The practical feasibility is demonstrated by an epidermal stopwatch that allows intimate integration with the human body. The high-permittivity nanocomposites reported here represent an attractive building block for stretchable electronic systems, which may find broad range of applications in intrinsically stretchable transistors, sensors, light-emitting devices, and energy-harvesting devices.
Intrinsically stretchable electronics represent an attractive platform for next-generation implantable devices by reducing the mechanical mismatch and the immune responses with biological tissues. Despite extensive efforts, soft implantable electronic devices often exhibit an obvious trade-off between electronic performances and mechanical deformability because of limitations of commonly used compliant electronic materials. Here, we introduce a scalable approach to create intrinsically stretchable and implantable electronic devices featuring the deployment of liquid metal components for ultrahigh stretchability up to 400% tensile strain and excellent durability against repetitive deformations. The device architecture further shows long-term stability under physiological conditions, conformal attachments to internal organs, and low interfacial impedance. Successful electrophysiological mapping on rapidly beating hearts demonstrates the potential of intrinsically stretchable electronics for widespread applications in health monitoring, disease diagnosis, and medical therapies.
Liquid metal confined in the elastomer represents an ideal platform for stretchable electronics with ultimate deformability. To enable facile and scalable patterning of conductive features, bulk liquid metal is typically dispersed into fine particles to formulate printable inks. The presence of native oxide or organic ligands stabilizing these liquid metal particles unfortunately inhibits their direct coalescence to recover the metallic conductivity and liquid-state deformability. Here, we report a chemical sintering process that converts printed liquid metal microparticles into a highly deformable conductor. The process involves the removal of surface passivating oxide by a short exposure to acid fume and subsequent selective wetting of liquid metal microparticles onto copper nanoplates present in the ink formulation. The chemical reaction provides the basis for a facile and scalable procedure to print conductive features over a large area with exceptional conductivity (>104 S cm–1) and ultrahigh stretchability (∼1000% strain). Their practical suitability is demonstrated by the fabrication of an ultrastretchable ribbon cable and an epidermal heater.
A breathable and stretchable form of electronic nanotextile is developed as a platform for epidermal devices.
The rapid expansion of electronic technology and short lifespan of consumer devices create a huge amount of electronic waste. The disposal of discarded devices represents a serious environmental challenge. Biodegradable devices are able to decompose into benign components after a period of stable operation during its service life, which represents a potential solution to reduce the environmental footprint of electronic technology. The widespread applications of biodegradable electronics are still hampered by the lack of facile manufacturing approach for high quality devices. Here, a laser sintering technique to weld naturally oxidized Zn microparticles into biodegradable conductors is reported. The sintering process is carried out under ambient conditions and compatible with various biodegradable substrates. A low‐cost fabrication procedure involving stencil printing and laser treatment is established to create conductive features with excellent conductivity and mechanical durability. The practical suitability of printed Zn conductor is demonstrated by fabricating near‐field communication tags, which are flexible and fully functional with the transient behavior modulated by the choice of packaging materials. The printed biodegradable conductor may find potential applications in eco‐friendly sensors, transient printed circuit boards, and implantable medical devices.
A stretchable alternating current electroluminescent display seamlessly combines the light-emitting capabilities with mechanical compliance, which offers exciting opportunities for applications in wearable gadgets, soft robots, and fashion designs. The widespread adaption to deformable forms of optoelectronics is currently impeded by the tedious and labor-intensive fabrication process. This study reports an efficient and scalable procedure to create a fully screen-printed, multicolor, and stretchable electroluminescent display. The as-prepared device exhibits excellent deformability and low-voltage operation. The practical implementation is demonstrated by creating a wearable sound-synchronized sensing system with an epidermal display responsive to the rhythm of music. The ink formulation and printing procedure developed here pave the way for convenient fabrication of stretchable electronic devices.
In spite of the excellent electrical and electrochemical properties, two-dimensional transition metal carbide (MXene) is often limited by the high stiffness for the direct implementation in next-generation stretchable and wearable energy storage devices. The improved deformability has been achieved in ultrathin composite electrodes utilizing additives that substantially reduce the specific capacitance. Here, we demonstrate an ultrastretchable and highperforming supercapacitor based on MXene electrodes with crumpled textures. After screening on the thickness, the crumpled MXene film of ∼3 μm in thickness is identified as the optimal choice to mitigate the crack formations under large and repetitive mechanical strains. The as-prepared symmetric supercapacitor, therefore, demonstrates a high specific capacitance of ∼470 mF cm −2 , ultrahigh stretchability up to 800% area strain, and >90% retention of the initial capacitance after 1000 stretch−relaxation cycles. The developments offer an attractive avenue to design stretchable electrodes based on various two-dimensional nanomaterials and their composites.
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