Abstract. On April 15 and 19, 1998, two intense dust storms were generated over the Gobi desert by springtime low-pressure systems descending from the northwest. The windblown dust was detected and its evolution followed by its yellow color on SeaWiFS satellite images, routine surface-based monitoring, and through serendipitous observations. The April 15 dust cloud was recirculating, and it was removed by a precipitating weather system over east Asia

Natural dust is often associated with hot, subtropical deserts, but significant dust events have been reported from cold, high latitudes. This review synthesizes current understanding of high‐latitude (≥50°N and ≥40°S) dust source geography and dynamics and provides a prospectus for future research on the topic. Although the fundamental processes controlling aeolian dust emissions in high latitudes are essentially the same as in temperate regions, there are additional processes specific to or enhanced in cold regions. These include low temperatures, humidity, strong winds, permafrost and niveo‐aeolian processes all of which can affect the efficiency of dust emission and distribution of sediments. Dust deposition at high latitudes can provide nutrients to the marine system, specifically by contributing iron to high‐nutrient, low‐chlorophyll oceans; it also affects ice albedo and melt rates. There have been no attempts to quantify systematically the expanse, characteristics, or dynamics of high‐latitude dust sources. To address this, we identify and compare the main sources and drivers of dust emissions in the Northern (Alaska, Canada, Greenland, and Iceland) and Southern (Antarctica, New Zealand, and Patagonia) Hemispheres. The scarcity of year‐round observations and limitations of satellite remote sensing data at high latitudes are discussed. It is estimated that under contemporary conditions high‐latitude sources cover >500,000 km2 and contribute at least 80–100 Tg yr−1 of dust to the Earth system (~5% of the global dust budget); both are projected to increase under future climate change scenarios.

Iron is an essential micronutrient that limits primary productivity in much of the ocean, including the Gulf of Alaska (GoA). However, the processes that transport iron to the ocean surface are poorly quantified. We combine satellite and meteorological data to provide the first description of widespread dust transport from coastal Alaska into the GoA. Dust is frequently transported from glacially‐derived sediment at the mouths of several rivers, the most prominent of which is the Copper River. These dust events occur most frequently in autumn, when coastal river levels are low and riverbed sediments are exposed. The dust plumes are transported several hundred kilometers beyond the continental shelf into iron‐limited waters. We estimate the mass of dust transported from the Copper River valley during one 2006 dust event to be between 25–80 ktons. Based on conservative estimates, this equates to a soluble iron loading of 30–200 tons. We suggest the soluble Fe flux from dust originating in glaciofluvial sediment deposits from the entire GoA coastline is two to three times larger, and is comparable to the annual Fe flux to GoA surface waters from eddies of coastal origin. Given that glaciers are retreating in the coastal GoA region and in other locations, it is important to examine whether fluxes of dust are increasing from glacierized landscapes to the ocean, and to assess the impact of associated Fe on marine ecosystems.

of monthly means of satellite-derived chlorophyll (CHL) and cloud condensation nuclei (CCN), as well as model outputs of hydroxyl radical (OH), rainfall amount (RAIN), and wind speed (WIND) for the Southern Ocean (SO, 40°S-60°S) is analyzed in order to explain CCN seasonality. Chlorophyll is used as a proxy for oceanic dimethylsulfide (DMS) emissions since both climatological aqueous DMS and atmospheric methanesulfonate (MSA) concentrations are tightly coupled with chlorophyll seasonality over the Southern Ocean. OH is included as the main atmospheric oxidant of DMS to produce CCN, and rainfall amount as the main loss factor for CCN through aerosol scavenging. Wind speed is used as a proxy for sea salt (SS) particles production. The CCN concentration seasonality is characterized by a clear pattern of higher values during austral summer and lower values during austral winter. Linear and multiple regression analyses reveal high significant correlations between CCN and the product of chlorophyll and OH (in phase) and rainfall amount (in antiphase). Also, CCN concentrations are anticorrelated with wind speed, which shows very little variability and a slight wintertime increase, in agreement with the sea salt seasonality reported in the literature. Finally, the fraction of the total aerosol optical depth contributed by small particles (ETA) exhibits a seasonality with a 3.5-fold increase from austral winter to austral summer. The biogenic contribution to CCN is estimated to vary between 35% (winter) and 80% (summer). Sea salt particles, although contributing an important fraction of the CCN burden, do not play a role in controlling CCN seasonality over the SO. These findings support the central role of biogenic DMS emissions in controlling not only the number but also the variability of CCN over the remote ocean.Citation: Vallina, S. M., R. Simó, and S. Gassó (2006), What controls CCN seasonality in the Southern Ocean? A statistical analysis based on satellite-derived chlorophyll and CCN and model-estimated OH radical and rainfall, Global Biogeochem. Cycles, 20, GB1014,

Aerosol-cloud interaction is the most uncertain mechanism of anthropogenic radiative forcing of Earth's climate, and aerosol-induced cloud water changes are particularly poorly constrained in climate models. By combining satellite retrievals of volcano and ship tracks in stratocumulus clouds, we compile a unique observational data set and confirm that liquid water path (LWP) responses to aerosols are bidirectional, and on average the increases in LWP are closely compensated by the decreases. Moreover, the meteorological parameters controlling the LWP responses are strikingly similar between the volcano and ship tracks. In stark contrast to observations, there are substantial unidirectional increases in LWP in the Hadley Centre climate model, because the model accounts only for the decreased precipitation efficiency and not for the enhanced entrainment drying. If the LWP increases in the model were compensated by the decreases as the observations suggest, its indirect aerosol radiative forcing in stratocumulus regions would decrease by 45%. Plain Language Summary It remains unclear how much of the global warming induced by greenhouse gases is offset by aerosols because the effect of aerosol particles on clouds is the most uncertain mechanism of forcing of Earth's climate by human activities. Cloud water responses to aerosols are especially uncertain. Here we compare the properties of low marine clouds impacted by volcanic and ship emissions with the properties of the nearby unpolluted clouds in order to increase the understanding of aerosol impacts on clouds. Clouds impacted by emissions from volcanoes and ships lose or gain water depending on meteorological conditions, but on average the amount of water does not change much in the polluted clouds. These observations disagree with the systematic increases in cloud water in response to aerosols simulated by the Hadley Centre climate model. This model, like other contemporary climate models, only accounts for cloud water increases that result from decreased precipitation efficiency and does not account for the enhanced drying in polluted clouds. Our results suggest that the ability of aerosols to offset global warming might be overestimated. The observational constraints derived here on aerosol-induced cloud water changes would ultimately translate into reduced uncertainties in projections of the future climate.

Peer ReviewedPostprint (author’s final draft

[1] The global chemical transport model GEOS-Chem, implemented with a dust-iron dissolution scheme, was used to analyze the magnitude and spatial distribution of mineral dust and soluble-iron (sol-Fe) deposition to the South Atlantic Ocean (SAO). The comparison of model results with remotely sensed data shows that GEOS-Chem can capture dust source regions in Patagonia and characterize the temporal variability of dust outflow. For a year-long model simulation, 22 Tg of mineral dust and 4 Gg of sol-Fe were deposited to the surface waters of the entire SAO region, with roughly 30% of this dust and sol-Fe predicted to be deposited to possible high nitrate low chlorophyll oceanic regions. Model-predicted dissolved iron fraction of mineral dust over the SAO was small, on average only accounting for 0.57% of total iron. Simulations suggest that the primary reason for such a small fraction of sol-Fe is the low ambient concentrations of acidic trace gases available for mixing with dust plumes. Overall, the amount of acid added to the deliquesced aerosol solution was not enough to overcome the alkalinity buffer of Patagonian dust and initiate considerable acid dissolution of mineral-iron. Sensitivity studies show that the amount of sol-Fe deposited to the SAO was largely controlled by the initial amount of sol-Fe at the source region, with limited contribution from the spatial variability of Patagonian-desert topsoil mineralogy and natural sources of acidic trace gases. Simulations suggest that Patagonian dust should have a minor effect on biological productivity in the SAO.

Although emission of dust from the Patagonia desert is shown by global aerosol models, there is conflicting observational evidence of dust activity in the region. Because dust from Patagonia into the Southern Ocean (SO) may play a role in regulating phytoplankton activity, it is necessary to confirm whether there is dust activity and if so, how far the dust travels into the SO. We used a combination of surface visibility, satellite measurements (MODIS and OMI) and transport model (HYSPLIT) to track and report for the first time a dust event originating in Patagonia. We show that the dust reached the free troposphere in the Sub‐Antarctic Atlantic Ocean. Although the dust emission was significant, cloudiness and dilution of the plume resulted in difficult conditions to track dust in the SW Atlantic. We show that the use of any single tool (i.e., MODIS or OMI) is not enough to track the dust and only an integrated approach of satellite and modeling tools can achieve a consistent description. As a result, current platforms used for dust detection are probably underestimating aerosol loading in the area