a pathway for defect-free electrical contact to 2D semiconductors and open up possibilities for circuits with efficient switching characteristics and higher efficiency optoelectronic devices.Van der Waals (vdW) heterostructures, [21] especially when passivated with hexagonal boron nitride (h-BN), [22,23] present an excellent platform for studying the Schottky-Mott limit. Graphene, [24,25] a semimetal with a gate-tunable work function, [26] is a promising alternative to traditional bulk metal electrical contacts to 2D semiconductors. [16] In lieu of using different metals, we propose a modified Schottky-Mott rule for gate-tunable Schottky junctions in which the gate voltage (V G ) directly modulates the barrier height (Φ B ), When 1901392 (2 of 5) www.advmat.de www.advancedsciencenews.com Conflict of InterestThe authors declare no conflict of interest.
Two-dimensional (2D) materials offer unique opportunities in engineering the ultrafast spatiotemporal response of composite nanomechanical structures. In this work, we report on high frequency, high quality factor (Q) 2D acoustic cavities operating in the 50–600 GHz frequency (f) range with f × Q up to 1 × 1014. Monolayer steps and material interfaces expand cavity functionality, as demonstrated by building adjacent cavities that are isolated or strongly-coupled, as well as a frequency comb generator in MoS2/h-BN systems. Energy dissipation measurements in 2D cavities are compared with attenuation derived from phonon-phonon scattering rates calculated using a fully microscopic ab initio approach. Phonon lifetime calculations extended to low frequencies (<1 THz) and combined with sound propagation analysis in ultrathin plates provide a framework for designing acoustic cavities that approach their fundamental performance limit. These results provide a pathway for developing platforms employing phonon-based signal processing and for exploring the quantum nature of phonons.
We demonstrate the use of a quantum transport model to study heavily graded graphene p-n junctions in the quantum Hall regime. A combination of p-n interface roughness and delta function disorder potential allows us to compare experimental results on different devices from the literature. We find that wide p-n junctions suppress mixing of n = 0 Landau levels. Our simulations spatially resolve carrier transport in the device, for the first time, revealing separation of higher order Landau levels in strongly graded junctions, which suppresses mixing.
We have directly written nanoscale patterns of magnetic ordering in FeRh films using focused helium-ion beam irradiation. By varying the dose, we pattern arrays with metamagnetic transition temperatures that range from the as-grown film temperature to below room temperature. We employ transmission electron microscopy, X-ray diffraction, and temperature-dependent transport measurements to characterize the as-grown film, and magneto-optic Kerr effect imaging to quantify the He+ irradiation-induced changes to the magnetic order. Moreover, we demonstrate temperature-dependent optical microscopy and conductive atomic force microscopy as indirect probes of the metamagnetic transition that are sensitive to the differences in dielectric properties and electrical conductivity, respectively, of FeRh in the antiferromagnetic (AF) and ferromagnetic (FM) states. Using density functional theory, we quantify strain- and defect-induced changes in spin-flip energy to understand their influence on the metamagnetic transition temperature. This work holds promise for in-plane AF–FM spintronic devices, by reducing the need for multiple patterning steps or different materials, and potentially eliminating interfacial polarization losses due to cross material interfacial spin scattering.
We present a quantum model which provides enhanced understanding of recent transverse magnetic focusing experiments on graphene p-n junctions. Spatially resolved flow maps of local particle current density show quantum interference and p-n junction filtering effects, which are crucial to explaining the device operation. The Landauer-Büttiker formula is used alongside dephasing edge contacts to give exceptional agreement between simulated nonlocal resistance and the recent experiment by Chen et al. [Science 353, 1522[Science 353, (2016]. The origin of positive and negative focusing resonances and off-resonance characteristics are explained in terms of quantum transmission functions. Our model also captures subtle features from experiment, such as the p-p − to p-p + transition and the second p-n focusing resonance.
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