Magnetic skyrmions are nanosized topologically protected spin textures with particlelike properties. They can form lattices perpendicular to the magnetic field, and the orientation of these skyrmion lattices with respect to the crystallographic lattice is governed by spin-orbit coupling. By performing small-angle neutron scattering measurements, we investigate the coupling between the crystallographic and skyrmion lattices in both Cu 2 OSeO 3 and the archetype chiral magnet MnSi. The results reveal that the orientation of the skyrmion lattice is primarily determined by the magnetic field direction with respect to the crystallographic lattice. In addition, it is also influenced by the magnetic history of the sample, which can induce metastable lattices. Kinetic measurements show that these metastable skyrmion lattices may or may not relax to their equilibrium positions under macroscopic relaxation times. Furthermore, multidomain lattices may form when two or more equivalent crystallographic directions are favored by spin-orbit coupling and oriented perpendicular to the magnetic field.

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The reference chiral helimagnet MnSi is the first system where skyrmion lattice correlations have been reported. At zero magnetic field the transition at TC to the helimagnetic state is of first order. Above TC , in a region dominated by precursor phenomena, neutron scattering shows the build up of strong chiral fluctuating correlations over the surface of a sphere with radius 2π/ , where is the pitch of the helix. It has been suggested that these fluctuating correlations drive the helical transition to first order following a scenario proposed by Brazovskii for liquid crystals. We present a comprehensive neutron scattering study under magnetic fields, which provides evidence that this is not the case. The sharp first order transition persists for magnetic fields up to 0.4 T whereas the fluctuating correlations weaken and start to concentrate along the field direction already above 0.2 T. Our results thus disconnect the first order nature of the transition from the precursor fluctuating correlations. They also show no indication for a tricritical point, where the first order transition crosses over to second order with increasing magnetic field. In this light, the nature of the first order helical transition and the precursor phenomena above TC , both of general relevance to chiral magnetism, remain an open question.

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We present a comprehensive small angle neutron scattering study of the doping dependence of the helimagnetic correlations in Mn1−xFexSi. The long-range helimagnetic order in Mn1−xFexSi is suppressed with increasing Fe content and disappears for x > x * ≈ 0.11, i.e. well before xC ≈ 0.17 where the transition temperature vanishes. For x > x * , only finite isotropic helimagnetic correlations persist which bear similarities with the magnetic correlations found in the precursor phase of MnSi. Magnetic fields gradually suppress and partly align these short-ranged helimagnetic correlations along their direction through a complex magnetization process.

The relative importance of long-and short-ranged forces on the thermal fluctuations at polymer interfaces was investigated with neutron reflection. Polyolefin blends were synthesised to create polymer pairs with a tuned interaction parameter, allowing the exploration of situations from near criticality to strongly immiscible cases in thin-film systems. We have observed for the polymer interfacial width, a transition from a region where long-ranged forces dominate, at higher degree of incompatibility, to a region approaching criticality where short-ranged truncation forces are more relevant.

A time of flight Modulation of Intensity by Zero Effort spectrometer mode has been developed for the Larmor instrument at the ISIS pulsed neutron source. The instrument utilizes resonant neutron spin flippers which employ electromagnets with pole shoes, allowing the flippers to operate at frequencies of up to 3 MHz. Tests were conducted at modulation frequencies of 103 kHz, 413 kHz, 826 kHz and 1.03 MHz, resulting in a Fourier time range of ~0.1 ns to 30 ns using a wavelength band of 4 Å to 11 Å.

Universality of the helimagnetic transition in cubic chiral magnets: Small angle neutron scattering and neutron spin echo spectroscopy studies of FeCoSi CopyrightOther than for strictly personal use, it is not permitted to download, forward or distribute the text or part of it, without the consent of the author(s) and/or copyright holder(s), unless the work is under an open content license such as Creative Commons. Takedown policyPlease contact us and provide details if you believe this document breaches copyrights. We will remove access to the work immediately and investigate your claim. We present a comprehensive small angle neutron scattering and neutron spin echo spectroscopy study of the structural and dynamical aspects of the helimagnetic transition in Fe 1−x Co x Si with x = 0.30. In contrast to the sharp transition observed in the archetype chiral magnet MnSi, the transition in Fe 1−x Co x Si is gradual, and long-range helimagnetic ordering coexists with short-range correlations over a wide temperature range. The dynamics are more complex than in MnSi and involve long relaxation times with a stretched exponential relaxation which persists even under magnetic field. These results in conjunction with an analysis of the hierarchy of the relevant length scales show that the helimagnetic transition in Fe 1−x Co x Si differs substantially from the transition in MnSi and question the validity of a universal approach to the helimagnetic transition in chiral magnets.