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The Digital Cherenkov Viewing Device (DCVD) [5] is a tool used by nuclear safeguards inspectors to verify irradiated nuclear fuel assemblies in wet storage based on the Cherenkov light produced by the assembly. Verifying that no rods have been substituted in the fuel, so-called partialdefect verification, is done by comparing the intensity measured with a DCVD with a predicted intensity, based on operator fuel declaration. The prediction model currently used by inspectors is based on simulations of Cherenkov light production in a BWR 8x8 geometry. This work investigates prediction models based on simulated Cherenkov light production in a BWR 8x8 and a PWR 17x17 assembly, as well as a simplified model based on a single rod in water. Cherenkov light caused by both fission product gamma and beta decays was considered. The simulations reveal that there are systematic differences between the model used by safeguards inspectors and the models described in this publication, most noticeably with respect to the fuel assembly cooling time. Consequently, if the intensity predictions are based on another fuel type than the fuel type being measured, a systematic bias in intensity with respect to burnup and cooling time is introduced. While a simplified model may be accurate enough for a set of fuel assemblies with nearly identical cooling times, the prediction models may differ systematically by up to 18 % for fuels with more varied cooling times. Accordingly, these investigations indicate that the currently used model may need to be exchanged with a set of more detailed, fuel-type specific models, in order minimize the model dependent systematic deviations.
A project to research the application of nondestructive assay (NDA) to spent fuel assemblies is underway. The research team comprises the European Atomic Energy Community (EURATOM), embodied by the European Commission, DG Energy, Directorate EURATOM Safeguards; the Swedish Nuclear Fuel and Waste Management Company (SKB); two universities; and several United States national laboratories. The Next Generation of Safeguards Initiative-Spent Fuel project team is working to achieve the following technical goals more easily and efficiently than in the past using nondestructive assay measurements of spent fuel assemblies: (1) verify the initial enrichment, burnup, and cooling time of facility declaration; (2) detect the diversion or replacement of pins, (3) estimate the plutonium mass, (4) estimate the decay heat, and (5) determine the reactivity of spent fuel assemblies. This study focuses on spectrally resolved gamma-ray measurements performed on a diverse set of 50 assemblies [25 pressurized water reactor (PWR) assemblies and 25 boiling water reactor (BWR) assemblies]; these same 50 assemblies will be measured with neutron-based NDA instruments and a full-length calorimeter. Given that encapsulation/repository and dry storage safeguards are the primarily intended applications, the analysis focused on the dominant gamma-ray lines of 137 Cs, 154 Eu, and 134 Cs because these isotopes will be the primary gamma-ray emitters during the time frames of interest to these applications. This study addresses the impact on the measured passive gamma-ray signals due to the following factors: burnup, initial enrichment, cooling time, assembly type (eight different PWR and six different BWR fuel designs),
The purpose of the Next Generation Safeguards Initiative (NGSI)-Spent Fuel (SF) project is to strengthen the technical toolkit of safeguards inspectors and/or other interested parties. The NGSI-SF team is working to achieve the following technical goals more easily and efficiently than in the past using nondestructive assay measurements of spent fuel assemblies: (1) verify the initial enrichment, burnup, and cooling time of facility declaration; (2) detect the diversion or replacement of pins; (3) estimate the plutonium mass [which is also a function of the variables in (1)]; (4) estimate the decay heat; and (5) determine the reactivity of spent fuel assemblies. Since August 2013, a set of measurement campaigns has been conducted at the Central Interim Storage Facility for Spent Nuclear Fuel (Clab), in collaboration with Swedish Nuclear Fuel and Waste Management Company (SKB). One purpose of the measurement campaigns was to acquire passive gamma spectra with high-purity germanium and lanthanum bromide scintillation detectors from Pressurized Water Reactor and Boiling Water Reactor spent fuel assemblies. The absolute 137 Cs count rate and the 154 Eu/ 137 Cs, 134 Cs/ 137 Cs, 106 Ru/ 137 Cs, and 144 Ce/ 137 Cs isotopic ratios were extracted; these values were used to construct corresponding model functions (which describe each measured quantity's behavior over various combinations of burnup, cooling time, and initial enrichment) and then were used to determine those same quantities in each measured spent fuel assembly. The results obtained in comparison with the operator declared values, as well as the methodology developed, are discussed in detail in the paper.
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