The Global Warming Potential (GWP) is used within the Kyoto Protocol to the United Nations Framework Convention on Climate Change as a metric for weighting the climatic impact of emissions of different greenhouse gases. The GWP has been subjected to many criticisms because of its formulation, but nevertheless it has retained some favour because of the simplicity of its design and application, and its transparency compared to proposed alternatives. Here, two new metrics are proposed, which are based on a simple analytical climate model. The first metric is called the Global Temperature Change Potential and represents the temperature change at a given time due to a pulse emission of a gas (GTP P ); the second is similar but represents the effect of a sustained emission change (hence GTP S ). Both GTP P and GTP S are presented as relative to the temperature change due to a similar emission change of a reference gas, here taken to be carbon dioxide. Both metrics are compared against an upwelling-diffusion energy balance model that resolves land and ocean and the hemispheres. The GTP P does not perform well, compared to the energy balance model, except for long-lived gases. By contrast, the GTP S is shown to perform well relative to the energy balance model, for gases with a wide variety of lifetimes. It is also shown that for time horizons in excess of about 100 years, the GTP S and GWP produce very similar results, indicating an alternative interpretation for the GWP. The GTP S retains the advantage of the GWP in terms of transparency, and the relatively small number of input parameters required for calculation. However, it has an enhanced relevance, as it is further down the cause-effect chain of the impacts of greenhouse gases emissions and has an unambiguous interpretation. It appears to be robust to key uncertainties and simplifications in its derivation and may be an attractive alternative to the GWP.

Multi-gas climate agreements require a metric by which emissions of gases with different lifetimes and radiative properties can be placed on a common scale. The Kyoto Protocol to the United Nations Framework Convention on Climate Change uses the global warming potential (GWP) as such a metric. The GWP has attracted particular criticism as being inappropriate in the context of climate policy which seeks to restrict warming below a given target, because it gives equal weight to emissions irrespective of the target and the proximity to the target. The use of an alternative metric, the time-dependent global temperature change potential (GTP), is examined for its suitability and the prospects for it including very short-lived species. It retains the transparency and relative ease of use, which are attractive features of the GWP, but explicitly includes a dependence on the target of climate policy. The weighting of emissions using the GTP is found to be significantly dependent on the scenarios offuture emissions and the sensitivity of the climate system. This may indicate that the use of any GTP-based weighting in future policymaking would necessitate regular revisions, as the global-mean temperature moves towards a specified target.

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Spatial patterns of local climate feedback and equilibrium partial temperature responses are produced from eight general circulation models with slab oceans forced by doubling carbon dioxide (CO2). The analysis is extended to other forcing mechanisms with the Met Office Hadley Centre slab ocean climate model version 3 (HadSM3). In agreement with previous studies, the greatest intermodel differences are in the tropical cloud feedbacks. However, the greatest intermodel spread in the equilibrium temperature response comes from the water vapor plus lapse rate feedback, not clouds, disagreeing with a previous study. Although the surface albedo feedback contributes most in the annual mean to the greater warming of high latitudes, compared to the tropics (polar amplification), its effect is significantly ameliorated by shortwave cloud feedback. In different seasons the relative importance of the contributions varies considerably, with longwave cloudy-sky feedback and horizontal heat transport plus ocean heat release playing a major role during winter and autumn when polar amplification is greatest. The greatest intermodel spread in annual mean polar amplification is due to variations in horizontal heat transport and shortwave cloud feedback. Spatial patterns of local climate feedback for HadSM3 forced with 2 × CO2, +2% solar, low-level scattering aerosol and high-level absorbing aerosol are more similar than those for different models forced with 2 × CO2. However, the equilibrium temperature response to high-level absorbing aerosol shows considerably enhanced polar amplification compared to the other forcing mechanisms, largely due to differences in horizontal heat transport and water vapor plus lapse rate feedback, with the forcing itself acting to reduce amplification. Such variations in high-latitude response between models and forcing mechanisms make it difficult to infer specific causes of recent Arctic temperature change.

The response of climate to ozone perturbations caused by regional emissions of NOx or CO has been studied through a sequence of model simulations. Changes in O 3 and OH concentrations due to emission perturbations in Europe and southeast Asia have been calculated with two global 3-D chemical tracer models(CTMs; LMDzINCA and Oslo-CTM2). The radiative transfer codes of three general circulation models (GCMs; ECHAM4, UREAD and LMD) have been used to calculate the radiative forcing of the O 3 perturbations, and for a subset of the cases full GCM simulations have been performed with ECHAM4 and UREAD. The results have been aggregated to a global number in two ways: first, through integrating the global-mean radiative forcing of a sustained step change in emissions, and second through a modified concept (SGWP * ) which includes possible differences in the climate sensitivity of O 3 , CH 4 and CO 2 changes. In terms of change in global tropospheric O 3 burden the two CTMs differ by less than 30%. Both CTMs show a higher north/south gradient in the sensitivity to changes in NOx emission than for CO. We are not able to conclude whether real O 3 perturbations in general have a different climate sensitivity from CO 2 . However, in both GCMs high-latitude emission perturbations lead to climate perturbations with higher (10-30%) climate sensitivities. The calculated SGWP * , for a 100 yr time horizon, are negative for three of the four CTM/GCM combinations for European emissions (−9.6 to +6.9), while for the Asian emissions the SGWP * (H = 100) is always positive (+2.9 to +25) indicating a warming. For CO the SGWP * values (3.8 and 4.4 for European and Asian emissions respectively, with only the Oslo-CTM2/ECHAM4 model combination) are less regionally dependent. Our results support the view that for NOx, regionally different weighting factors for the emissions are necessary. For CO the results are more robust and one global number may be acceptable.

The response of climate to ozone perturbations caused by regional emissions of NOx or CO has been studied through a sequence of model simulations. Changes in O3 and OH concentrations due to emission perturbations in Europe and southeast Asia have been calculated with two global 3‐D chemical tracer models(CTMs; LMDzINCA and Oslo‐CTM2). The radiative transfer codes of three general circulation models (GCMs; ECHAM4, UREAD and LMD) have been used to calculate the radiative forcing of the O3 perturbations, and for a subset of the cases full GCM simulations have been performed with ECHAM4 and UREAD. The results have been aggregated to a global number in two ways: first, through integrating the global‐mean radiative forcing of a sustained step change in emissions, and second through a modified concept (SGWP*) which includes possible differences in the climate sensitivity of O3, CH4 and CO2 changes. In terms of change in global tropospheric O3 burden the two CTMs differ by less than 30%. Both CTMs show a higher north/south gradient in the sensitivity to changes in NOx emission than for CO. We are not able to conclude whether real O3 perturbations in general have a different climate sensitivity from CO2. However, in both GCMs high‐latitude emission perturbations lead to climate perturbations with higher (10–30%) climate sensitivities. The calculated SGWP*, for a 100 yr time horizon, are negative for three of the four CTM/GCM combinations for European emissions (−9.6 to +6.9), while for the Asian emissions the SGWP* (H= 100) is always positive (+2.9 to +25) indicating a warming. For CO the SGWP* values (3.8 and 4.4 for European and Asian emissions respectively, with only the Oslo‐CTM2/ECHAM4 model combination) are less regionally dependent. Our results support the view that for NOx, regionally different weighting factors for the emissions are necessary. For CO the results are more robust and one global number may be acceptable.

Abstract. We combined high resolution aircraft flight data from the EU Fifth Framework Programme project AERO2k with analysis data from the ECMWF's integrated forecast system to calculate diurnally resolved 3-D contrail cover. We scaled the contrail cover in order to match observational data for the Bakan area (eastern-Atlantic/western-Europe).We found that less than 40% of the global distance travelled by aircraft is due to flights during local night time. Yet, due to the cancellation of shortwave and longwave effects during daytime, night time flights contribute a disproportional 60% to the global annual mean forcing. Under clear sky conditions the night flights contribute even more disproportionally at 76%. There are pronounced regional variations in night flying and the associated radiative forcing. Over parts of the North Atlantic flight corridor 75% of air traffic and 84% of the forcing occurs during local night, whereas only 35% of flights are during local night in South-East Asia, yet these contribute 68% of the radiative forcing. In general, regions with a significant local contrail radiative forcing are also regions for which night time flights amount to less than half of the daily total of flights. Therefore, neglecting diurnal variations in air traffic/contrail cover by assuming a diurnal mean contrail cover can over-estimate the global mean radiative forcing by up to 30%.

Air traffic condensation trails, or contrails, are believed to have a net atmospheric warming effect, although one that is currently small compared to that induced by other sources of human emissions. However, the comparably large growth rate of air traffic requires an improved understanding of the resulting impact of aircraft radiative forcing on climate. Contrails have an effect on the Earth's energy balance similar to that of high thin ice clouds. Their trapping of outgoing longwave radiation emitted by the Earth and atmosphere (positive radiative forcing) is partly compensated by their reflection of incoming solar radiation (negative radiative forcing). On average, the longwave effect dominates and the net contrail radiative forcing is believed to be positive. Over daily and annual timescales, varying levels of air traffic, meteorological conditions, and solar insolation influence the net forcing effect of contrails. Here we determine the factors most important for contrail climate forcing using a sophisticated radiative transfer model for a site in southeast England, located in the entrance to the North Atlantic flight corridor. We find that night-time flights during winter (December to February) are responsible for most of the contrail radiative forcing. Night flights account for only 25 per cent of daily air traffic, but contribute 60 to 80 per cent of the contrail forcing. Further, winter flights account for only 22 per cent of annual air traffic, but contribute half of the annual mean forcing. These results suggest that flight rescheduling could help to minimize the climate impact of aviation.