We experimentally investigate the process of intramolecular quantum interference in high-order harmonic generation in impulsively aligned CO2 molecules. The recombination interference effect is clearly seen through the order dependence of the harmonic yield in an aligned sample. The experimental results can be well modeled assuming that the effective de Broglie wavelength of the returning electron wave is not significantly altered by the Coulomb field of the molecular ion. We demonstrate that such interference effects can be effectively controlled by changing the ellipticity of the driving laser field.
Wavelength scaling of high harmonic generation efficiencyUsing longer wavelength laser drivers for high harmonic generation is desirable because the highest extreme ultraviolet frequency scales as the square of the wavelength. Recent numerical studies predict that high harmonic efficiency falls dramatically with increasing wavelength, with a very unfavorable Àð5À6Þ scaling. We performed an experimental study of the high harmonic yield over a wavelength range of 800-1850 nm. A thin gas jet was employed to minimize phase matching effects, and the laser intensity and focal spot size were kept constant as the wavelength was changed. Ion yield was simultaneously measured so that the total number of emitting atoms was known. We found that the scaling at constant laser intensity is À6:3AE1:1 in Xe and À6:5AE1:1 in Kr over the wavelength range of 800-1850 nm, somewhat worse than the theoretical predictions.
Using quadrupole scan measurements we show laser-wakefield accelerated electrons to have a normalized transverse emittance of 0:21 þ0:01 À0:02 mm mrad at 245 MeV. We demonstrate a multishot and a single-shot method, the mean emittance values for both methods agree well. A simple model of the beam dynamics in the plasma density downramp at the accelerator exit matches the source size and divergence values inferred from the measurement. In the energy range of 245 to 300 MeV the normalized emittance remains constant.Laser-wakefield acceleration (LWFA) [1,2] can deliver ultrarelativistic electron beams in a compact setup with unique features [3][4][5][6]. It is receiving particular attention as a source or driver for ultrashort x-ray beams [7,8] and for its potential for realizing a tabletop free-electron laser (FEL) [9]. The electron bunch duration has recently been measured to be only a few femtoseconds long [10,11] which results in peak beam currents on the order of kiloamperes. An essential parameter for the performance of x-ray sources, FELs, or linear colliders is the transverse electron beam emittance. Previous emittance measurements of LWFA electron beams have used the pepperpot method [12][13][14] giving normalized emittances of $2:2 mm mrad with single shots down to the resolution limit of 1:1 mm mrad. As these measurements are not spectrally resolved, they rely on a low energy spread to give a meaningful normalized emittance. For LWFA beams which fluctuate in energy and energy spread, a simultaneous measurement of the spectrum is required. This technique is also limited to electron energies that can be sufficiently scattered by the pepper-pot mask; to date, measurements of a 508 MeV beam have been carried out [15]. Experiments characterizing the betatron radiation emitted by the electron beam while it is in the plasma suggest the beam size there to be & 1 m [16,17], which in combination with a divergence measurement give an estimated emittance of <0:5 mm mrad [18]. However, inferring the emittance from the electron beam size in the plasma and its downstream divergence in the vacuum can be unreliable as this neglects the plasma-vacuum density transition at the accelerator exit; here the decreasing strength of the plasma focusing forces result in an increase in beam size and decrease in divergence [13]. This publication reports on direct measurements of the emittance of LWFA electrons that are both energy resolved and that include the beam transport of the density downramp at the accelerator exit. This is achieved by analyzing their beam size around a focus using a quadrupole lens scan method [19].The transverse phase space of an electron beam is often specified using the Twiss parameters , , , and the natural emittance ". These parameters describe the volume and orientation of the particle distribution in phase space. The beam size at a particular position ðs 1 Þ is related to the Twiss parameters at s 0 by [20] ðs 1 Þ 2 ¼ M 2 11 ðs 0 Þ À2M 11 M 12 ðs 0 Þþ M 2 12 ðs 0 Þ: (1)Here M ij refers to the ij eleme...
Understanding the role of coherent electronic motion is expected to resolve general questions of importance in macromolecular energy transfer. We demonstrate a novel nonlinear optical method, angle-resolved coherent wave mixing, that separates out coherently coupled electronic transitions and energy transfers in an instantaneous two-dimensional mapping. Angular resolution of the signal is achieved by using millimeter laser beam waists at the sample and by signal relay to the far field; for this we use a high energy, ultrabroadband hollow fiber laser source. We reveal quantum electronic beating with a time-ordered selection of transition energies in a photosynthetic complex.
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.
customersupport@researchsolutions.com
10624 S. Eastern Ave., Ste. A-614
Henderson, NV 89052, USA
This site is protected by reCAPTCHA and the Google Privacy Policy and Terms of Service apply.
Copyright © 2024 scite LLC. All rights reserved.
Made with 💙 for researchers
Part of the Research Solutions Family.