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Lidar (light detection and ranging) depolarization measurements were performed simultaneously at three wavelengths using a coherent white light continuum. The white light continuum ranging from the ultraviolet to the infrared region was generated by a focused 0.5 TW/100 fs pulse in a krypton gas cell at the atmospheric pressure. The lidar system consisted of three depolarization channels at 450, 550, and 800 nm. The observed depolarization ratios for each wavelength showed differences for clouds. These depolarization features in wavelength are discussed in terms of particle size and shape using T-matrix computations. The depolarization ratios at three wavelengths can be used to infer information on the size of the particles in clouds, assuming an ice crystal shape a priori. Also, the obtained size distributions from the three-wavelength depolarization ratios correspond with the changes in particle size indicated by changes in the Angstrom coefficient obtained by multiwavelength lidar techniques. This study demonstrated that the three-wavelength depolarization ratios provided additional information about the size and shape of clouds and aerosols.

A white light continuum was generated by a self-trapped intense femtosecond laser pulse in atmospheric-pressure rare gas, krypton. The measured broad spectrum of the generated white light ranged from 300 nm to more than 950 nm. This new light source was utilized for the first time to perform three-wavelength backscatter measurement of aerosols and clouds. The time-resolved backscattered light was separated into three channels, 350 nm, 550 nm and 700 nm. Each channel showed strong backscattering from aerosols and clouds up to 2.5 km. Experimental measurement indicates that this novel light source can be used for multiwavelength lidar studies.

Poor air quality has been identified as one of the main risks to human health, especially in developing regions, where the information on physical chemical properties of air pollutants is lacking. To bridge this gap, we conducted an intensive measurement campaign in Manila, Philippines to determine the emission factors (EFs) of particle number (PN) and equivalent black carbon (BC). The focus was on public utility jeepneys (PUJ), equipped with old technology diesel engines, widely used for public transportation. The EFs were determined by aerosol physical measurements, fleet information, and modeled dilution using the Operational Street Pollution Model (OSPM). The results show that average vehicle EFs of PN and BC in Manila is up to two orders of magnitude higher than European emission standards. Furthermore, a PUJ emits up to seven times more than a light-duty vehicles (LDVs) and contribute to more than 60% of BC emission in Manila. Unfortunately, traffic restrictions for heavy-duty vehicles do not apply to PUJs. The results presented in this work provide a framework to help support targeted traffic interventions to improve urban air quality not only in Manila, but also in other countries with a similar fleet composed of old-technology vehicles.