Conventional energy-integration black-white X-ray imaging lacks spectral information of X-ray photons. Although X-ray spectra (energy) can be distinguished by photon-counting technique typically with CdZnTe detectors, it is very challenging to be applied to large-area flat-panel X-ray imaging (FPXI). Herein, we design multi-layer stacked scintillators of different X-ray absorption capabilities and scintillation spectrums, in this scenario, the X-ray energy can be discriminated by detecting the emission spectra of each scintillator, therefore the multispectral X-ray imaging can be easily obtained by color or multispectral visible-light camera in one single shot of Xray. To verify this idea, stacked multilayer scintillators based on several emerging metal halides were fabricated in the cost-effective and scalable solution process, and proofof-concept multi-energy FPXI were experimentally demonstrated. The dual-energy Xray image of a "bone-muscle" model clearly showed the details that were invisible in conventional energy-integration FPXI. By stacking four layers of specifically designed multilayer scintillators with appropriate thicknesses, a prototype FPXI with four energy channels was realized, proving its extendibility to multispectral or even hyperspectral X-ray imaging. This study provides a facile and effective strategy to realize energyresolved flat-panel X-ray imaging.
Lead-free copper halide scintillators have shown tremendous potential applications in X-ray detection and imaging. However, the imaging resolution is still rather limited due to the lack of a scintillation waveguide, especially for the solution-processed nanocrystal scintillators. Here, we report a solution synthesis route for Cs3Cu2I5 nanowire (NW) arrays via an anodized aluminum oxide (AAO) template-assisted in situ growth. As the NWs grow, the precursor concentration directly affects the length and uniformity of the Cs3Cu2I5 NWs among the various factors. The as-synthesized Cs3Cu2I5 NW array scintillators achieve a high spatial resolution of 20 lp mm–1, which is so far the highest value for this emerging copper halide scintillators. The present study provides a convenient and facile method to synthesize Cs3Cu2I5 NW arrays for high-resolution X-ray imaging.
Conventional energy-integration black-white X-ray imaging lacks spectral information of X-ray photons. Although X-ray spectra (energy) can be distinguished by photon-counting technique typically with CdZnTe detectors, it is very challenging to be applied to large-area flat-panel X-ray imaging (FPXI). Herein, we design multi-layer stacked scintillators of different X-ray absorption capabilities and scintillation spectrums, in this scenario, the X-ray energy can be discriminated by detecting the emission spectra of each scintillator, therefore the spectral-resolving X-ray imaging can be easily obtained by color or multispectral visible-light camera in one single shot of X-ray. To verify this idea, stacked multilayer scintillators based on several emerging metal halides were fabricated in the cost-effective and scalable solution process, and proof-of-concept multi-energy FPXI was experimentally demonstrated. The energy-resolving X-ray image of a “bone-muscle” model clearly showed the details that were invisible in conventional energy-integration FPXI. By stacking four layers of specifically designed multilayer scintillators with appropriate thicknesses, a prototype FPXI with four energy channels was realized, proving its extendibility to multispectral or even hyperspectral X-ray imaging. This study provides a facile and effective strategy to realize energy-resolved flat-panel X-ray imaging.
Thin film transistor (TFT) has been a key device for planal drive display technology, and operating the TFT device in a saturation regime is particularly important for driving the light emission at a stable current. Considering the light emission reaches the TFT planal, it is thereby meaningful to understand the effect of illumination on TFT saturation behavior in order to improve the stability of light emission. Through experiments and simulations, our study shows that the drift current of photogenerated carriers can follow a saturation behavior when the channel conductance is dominated by charges induced by gate bias rather than the charges generated by photons, and vice versa. The obtained device physics insights are beneficial for developing TFT technologies that can drive light emission at a stable current.
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