A novel polymeric biomaterial platform with tunable functionalizability for extrusion-based 3D printing.

With the objective of generating photo-responsive polymers, carbonate monomers with pendant cinnamoyl or coumarin moieties, which are capable of photo-reversible dimerization, were synthesized.

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Triethylamine hydrochloride and triethylamine catalyze the melt polymerization of carbonate monomers faster than stannous octoate.

A novel allenyl-containing 1,3-spiro-amido alcohol auxiliary has been prepared and used in a variety of diastereoselective Diels-Alder reactions providing exclusively endo adducts with diastereomeric ratios ranging from 2:1 to >99:1.

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