requires 58, 70, and 129 mV in alkaline, acid, and neutral media, respectively, to reach 10 mA cm -2 , which also presents fast reaction kinetics and high long-term stability. The experimental and density functional theory (DFT) results verify that the abundant active heterostructure in Super-Co 3 S 4 /P-WS 2 /Co 9 S 8 can not only provide Pt-like H*-adsorption Gibbs free energy (ΔG H* ) but also promote the H 2 O adsorption and dissociation kinetics for all-pH HER. Moreover, the collaboration of favorable metallic components and special nanoarray morphology can also strengthen the electric conductivity for electron transfer and promote the maximum exposure of active heterointerfaces for mass transport in electrocatalysis. The interesting strategy herein is expected to inspire the future design of advanced metal sulfide-based heterostructures for energy storage and conversion.
Rock glaciers represent typical periglacial landscapes and are distributed widely in alpine mountain environments. Rock glacier activity represents a critical indicator of water reserves state, permafrost distribution, and landslide disaster susceptibility. The dynamics of rock glacier activity in alpine periglacial environments are poorly quantified, especially in the central Himalayas. Multi-temporal Interferometric Synthetic Aperture Radar (MT-InSAR) has been shown to be a useful technique for rock glacier deformation detection. In this study, we developed a multi-baseline persistent scatterer (PS) and distributed scatterer (DS) combined MT-InSAR method to monitor the activity of rock glaciers in the central Himalayas. In periglacial landforms, the application of the PS interferometry (PSI) method is restricted by insufficient PS due to large temporal baseline intervals and temporal decorrelation, which hinder comprehensive measurements of rock glaciers. Thus, we first evaluated the rock glacier interferometric coherence of all possible interferometric combinations and determined a multi-baseline network based on rock glacier coherence; then, we constructed a Delaunay triangulation network (DTN) by exploiting both PS and DS points. To improve the robustness of deformation parameters estimation in the DTN, we combined the Nelder–Mead algorithm with the M-estimator method to estimate the deformation rate variation at the arcs of the DTN and introduced a ridge-estimator-based weighted least square (WLR) method for the inversion of the deformation rate from the deformation rate variation. We applied our method to Sentinel-1A ascending and descending geometry data (May 2018 to January 2019) and obtained measurements of rock glacier deformation for 4327 rock glaciers over the central Himalayas, at least more than 15% detecting with single geometry data. The line-of-sight (LOS) deformation of rock glaciers in the central Himalayas ranged from −150 mm to 150 mm. We classified the active deformation area (ADA) of all individual rock glaciers with the threshold determined by the standard deviation of the deformation map. The results show that 49% of the detected rock glaciers (monitoring rate greater than 30%) are highly active, with an ADA ratio greater than 10%. After projecting the LOS deformation to the steep slope direction and classifying the rock glacier activity following the IPA Action Group guideline, 12% of the identified rock glaciers were classified as active and 86% were classified as transitional. This research is the first multi-baseline, PS, and DS network-based MT-InSAR method applied to detecting large-scale rock glaciers activity.
Maintaining
the human body’s comfort is a predominant requirement
of functional textiles, but there are still considerable drawbacks
to design an intelligent textile with proper moisture absorption and
evaporation properties. Herein, we develop moisture-wicking and solar-heated
coaxial fibers with a bark-like appearance for fabric comfort management.
The cortex layer of coaxial fibers can absorb moisture via the synergistic
effect of the hierarchical roughness and the hydrophilic polymeric
matrix. The core layer containing zirconium carbide nanoparticles
can assimilate energy from the body and sunlight, which raises the
surface temperature of the material and accelerates moisture evaporation.
The resulting coaxial fiber-based membrane exhibits an excellent droplet
diffusion radius of 2.73 cm, an excellent wicking height of 6.97 cm,
and a high surface temperature of 61.7 °C which is radiated by
simulated sunlight. Moreover, the designed fabric also exhibits a
significant UV protection factor of 2000. Overall, the successful
synthesis of such fascinating fibrous membranes enables the rapid
removal of sweat from the human body textile, providing a suitable
and comfortable microenvironment for the human body.
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