Lead-free (Na 0:5 K 0:5 )NbO 3 (NKN) powders and thin films were fabricated from stoichiometric (Na/K ¼ 50=50), 4 mol % excess (52/52, 53/51, and 55/49), and 10 mol % excess (55/55, 56/54, 58/52, and 60/50) precursor solutions by the sol-gel process. The NKN55/55 powder heat-treated at 800 C showed an orthorhombic phase and rectangular grains whose size was estimated to be about 300 nm. With increasing Na/K ratio, grain size increased to about 1 mm and the cubic-tetragonal (T c ) phase transition peak emerged at 392 C in a differential thermal analysis (DTA) curve. On the other hand, single-phase NKN thin films were fabricated at 600 C from the (Na,K)-excess precursor solutions (58/52 and 60/50). In particular, the NKN58/ 52 thin film showed a low leakage current density (10 À7 A/cm 2 at 40 kV/cm), and the maximum polarization P max and dielectric constant " r at 1 kHz were 9.1 mC/cm 2 and 725, respectively.
A tracer-encapsulated solid pellet (TESPEL) injection system for the TJ-II stellarator was recently developed. In order to reduce the time and cost for the development, we combined a TESPEL injector provided by National Institute for Fusion Science with an existing TJ-II cryogenic pellet injection system. Consequently, the TESPEL injection into the TJ-II plasma was successfully achieved, which was confirmed by several pellet diagnostics including a normal-incidence spectrometer for monitoring a tracer impurity behavior.
A 20 barrel solid hydrogen pellet injector, which is able to inject 20 cylindrical pellets with a diameter and length of between 3.0 and 3.8 mm at the velocity of 1200 m/s, has been developed for the purpose of direct core fueling in LHD (Large Helical Device). The in situ pipe gun concept with the use of compact cryo-coolers enables stable operation as a fundamental facility in plasma experiments. The combination of the two types of pellet injection timing control modes, i.e., pre-programing mode and real-time control mode, allows the build-up and sustainment of high density plasma around the density limit. The pellet injector has demonstrated stable operation characteristics during the past three years of LHD experiments.
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