Recent experiments have demonstrated that outdoor ozone reacts with materials inside residential building enclosures, potentially reducing indoor exposures to ozone or altering ozone reaction byproducts. However, test methods to measure ozone penetration factors in residences (P) remain limited. We developed a method to measure ozone penetration factors in residences under infiltration conditions and applied it in an unoccupied apartment unit. Twenty-four repeated measurements were made, and results were explored to (i) evaluate the accuracy and repeatability of the new procedure using multiple solution methods, (ii) compare results from 'interference-free' and conventional UV absorbance ozone monitors, and (iii) compare results against those from a previously published test method requiring artificial depressurization. The mean (±s.d.) estimate of P was 0.54 ± 0.10 across a wide range of conditions using the new method with an interference-free monitor; the conventional monitor was unable to yield meaningful results due to relatively high limits of detection. Estimates of P were not clearly influenced by any indoor or outdoor environmental conditions or changes in indoor decay rate constants. This work represents the first known measurements of ozone penetration factors in a residential building operating under natural infiltration conditions and provides a new method for widespread application in buildings.
Understanding the bioaerosol dynamics of droplets and droplet nuclei emitted during respiratory activities is important for understanding how infectious diseases are transmitted and potentially controlled. To this end, we conducted experiments to quantify the size-resolved dynamics of indoor bioaerosol transport and control in an unoccupied apartment unit operating under four different HVAC particle filtration conditions. Two model organisms (Escherichia coli K12 and bacteriophage T4) were aerosolized under alternating low and high flow rates to roughly represent constant breathing and periodic coughing. Size-resolved aerosol sampling and settle plate swabbing were conducted in multiple locations. Samples were analyzed by DNA extraction and quantitative polymerase chain reaction (qPCR). DNA from both organisms was detected during all test conditions in all air samples up to 7 m away from the source, but decreased in magnitude with the distance from the source. A greater fraction of T4 DNA was recovered from the aerosol size fractions smaller than 1 μm than E. coli K12 at all air sampling locations. Higher efficiency HVAC filtration also reduced the amount of DNA recovered in air samples and on settle plates located 3-7 m from the source.
Much of human exposure to particulate matter of outdoor origin occurs inside buildings, particularly in residences. The particle penetration factor through leaks in a building's exterior enclosure assembly is a key parameter that governs the infiltration of outdoor particles. However, experimental data for size-resolved particle penetration factors in real buildings, as well as penetration factors for fine particles less than 2.5 μm (PM ) and ultrafine particles less than 100 nm (UFPs), remain limited, in part because of previous limitations in instrumentation and experimental methods. Here, we report on the development and application of a modified test method that utilizes portable particle sizing instrumentation to measure size-resolved infiltration factors and envelope penetration factors for 0.01-2.5 μm particles, which are then used to estimate penetration factors for integral measures of UFPs and PM . Eleven replicate measurements were made in an unoccupied apartment unit in Chicago, IL to evaluate the accuracy and repeatability of the test procedure and solution methods. Mean estimates of size-resolved penetration factors ranged from 0.41 ± 0.14 to 0.73 ± 0.05 across the range of measured particle sizes, while mean estimates of penetration factors for integral measures of UFPs and PM were 0.67 ± 0.05 and 0.73 ± 0.05, respectively. Average relative uncertainties for all particle sizes/classes were less than 20%.
Venting range hoods can control indoor air pollutants emitted during residential cooktop and oven cooking. To quantify their potential benefits, it is important to know how frequently and under what conditions range hoods are operated during cooking. We analyzed data from 54 single family houses and 17 low-income apartments in California in which cooking activities, range hood use, and fine particulate matter (PM2.5) were monitored for one week per home. Range hoods were used for 36% of cooking events in houses and 28% in apartments. The frequency of hood use increased with cooking frequency across homes. In both houses and apartments, the likelihood of hood use during a cooking event increased with the duration of cooktop burner use, but not with the duration of oven use. Actual hood use rates were higher in the homes of participants who self-reported more frequent use in a pre-study survey, but actual use was far lower than self-reported frequency. Residents in single family houses used range hoods more often when cooking caused a discernible increase in PM2.5. In apartments, residents used their range hood more often only when high concentrations of PM2.5 were generated during cooking.
Toshifumi Hotchi prepared 23 instrumentation and assisted with data collection at Sites 1-2; Marion Russell supervised preparation and analysis of passive samples; Yuhan Wang assisted with data analysis. We are 25 also deeply appreciative of the building managers and participants.
Much of human exposure to nitrogen oxides (NO x ) of ambient origin occurs indoors. Reactions with materials inside building envelopes are expected to influence the amount of ambient NO x that infiltrates indoors. However, envelope penetration factors for ambient NO x constituents have never been measured. Here, we develop and apply methods to measure the penetration factor and indoor loss rates for ambient NO x constituents using time-resolved measurements in an unoccupied apartment unit. Multiple test methods and parameter estimation approaches were tested, including natural and artificial indoor NO x elevation with and without accounting for indoor oxidation reactions. Twelve of 16 tests yielded successful estimates of penetration factors and indoor loss rates. The penetration factor for NO was confirmed to be ∼1 and the mean (±s.d.) NO 2 penetration factor was 0.72 ± 0.06 with a mean relative uncertainty of ∼15%. The mean (±s.d.) indoor NO 2 loss rate was 0.27 ± 0.12 h −1 , ranging 0.06−0.47 h −1 , with strong correlations with indoor relative and absolute humidity. Indoor NO loss rates were strongly correlated with the estimated ozone concentration in infiltrating air. Results suggest that envelope penetration factors and loss rates for NO x constituents can be reasonably estimated across a wide range of conditions using these approaches.
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