Significant potential of electronic textiles for wearable applications has triggered active studies of luminescent fibers toward smart textile displays. In spite of notable breakthroughs in the lighting fiber technology, a class of information displays with a luminescent fiber network is still underdeveloped due to several formidable challenges such as limited electroluminescence fiber performance, acute vulnerability to chemical and mechanical factors, and lack of decent engineering schemes to form fibers with robust interconnectable pixels for two-dimensional matrix addressing. Here, we present a highly feasible strategy for organic light-emitting diode (OLED) fiber-based textile displays that can overcome these issues by implementing prominent solution options including compatible fabrication method of OLED pixel arrays on adapted fiber configurations and chemically/mechanically sturdy but electrically conductive passivation system. To create solid interconnectable OLED fibers without compromising the high electroluminescence performance, phosphorescence OLED materials are deposited onto process-friendly fibers of rectangular stripes, where periodically patterned OLED pixels are selectively passivated with robust polymer and circumventing metal pads by a stamp-assisted printing method. A woven textile of interlaced interconnectable OLED fibers with perpendicularly arranged conductive fibers serves as a matrix-addressable two-dimensional network that can be operated by the passive matrix scheme. Successful demonstrations of stably working woven OLED textile in the water, as well as under the applied tensile force, support feasibility of the present approach to reify fully addressable, environmentally durable, fiber-based textile displays.
Wearable electronic devices are being developed because of their wide potential applications and user convenience. Among them, wearable organic light emitting diodes (OLEDs) play an important role in visualizing the data signal processed in wearable electronics to humans. In this study, textile-based OLEDs were fabricated and their practical utility was demonstrated. The textile-based OLEDs exhibited a stable operating lifetime under ambient conditions, enough mechanical durability to endure the deformation by the movement of humans, and washability for maintaining its optoelectronic properties even in water condition such as rain, sweat, or washing. In this study, the main technology used to realize this textile-based OLED was multi-functional near-room-temperature encapsulation. The outstanding impermeability of TiO2 film deposited at near-room-temperature was demonstrated. The internal residual stress in the encapsulation layer was controlled, and the device was capped by highly cross-linked hydrophobic polymer film, providing a highly impermeable, mechanically flexible, and waterproof encapsulation.
Organic light-emitting diode (OLED) fibers with favorable electroluminescence properties and interconnectable pixel configurations have represented the potential for wearable electronic textile displays. Nevertheless, the current technology of OLED fiber-based textile displays still leaves to be desired due to several challenges, including limited emission area and lack of encapsulation systems. Here we present a fibrous OLED textile display that can attain a large emission area and long-term stability by implementing addressable networks comprised of integrated phosphorescence OLED fibers and by designing multilayer encapsulations. The integrated fiber configuration offers decoupled functional fiber surfaces for an interconnectable 1-dimensional OLED pixel array and a data-addressing conductor. Tailored triadic metal/ultrathin oxide/polymer multilayer enables not only the oxygen/water permeation inhibition but also the controllable conductive channels of dielectric antifuses. Together with reliable bending stability, the long-term operation of OLED textiles in water manifests the feasibility of the present device concept toward water-resistant full-emitting-area fibrous textile displays.
Smart displays have been integrated into our daily life, providing new concepts of interconnections between humans and interactivity with close collaboration
Increasing demand for real-time healthcare monitoring is leading to advances in thin and flexible optoelectronic device-based wearable pulse oximetry. Most previous studies have used OLEDs for this purpose, but did not consider the side effects of broad full-width half-maximum (FWHM) characteristics and single substrates. In this study, we performed SpO2 measurement using a fiber-based quantum-dot pulse oximetry (FQPO) system capable of mass production with a transferable encapsulation technique, and a narrow FWHM of about 30 nm. Based on analyses we determined that uniform angular narrow FWHM-based light sources are important for accurate SpO2 measurements through multi-layer structures and human skin tissues. The FQPO was shown to have improved photoplethysmogram (PPG) signal sensitivity with no waveguide-mode noise signal, as is typically generated when using a single substrate (30–50%). We successfully demonstrate improved SpO2 measurement accuracy as well as all-in-one clothing-type pulse oximetry with FQPO.
Spectral upconversion systems placed underneath solar cells have the considerable potential for enhancement of the photovoltaic performance as they allow additional absorption for the solar photons with energy below the bandgap of active materials. However, their application to a type of ultrathin solar cells for achieving the meaningful benefit of the efficiency improvement is challenging, because a pre‐existing rear‐side reflector that substantially increases the photon absorption needs to be eliminated for photonic interaction between photovoltaic active layer and upconversion medium, and hence a level of cell efficiency becomes limited. Herein a facile strategy is presented that can circumvent the issue of performance deterioration arising from the expelled reflector for integrating plasmonically enhanced upconversion systems with ultrathin nonfullerene‐based polymer solar cells. By employing a wavelength‐selectively reflective rear electrode of metal/dielectric multilayer that enables the photon penetration only at excitation and emission wavelengths of the upconversion process, the effect of photocurrent improvement with uncompromising efficiency levels can be expected from the plasmonic upconversion backplane comprising NaYF4:Yb3+,Er3+ core‐shell nanoparticles and metallic nanostructure. Systematic studies of optical process and resulting device performance in both experiments and numerical modeling provide the optimal design scheme for high‐performance polymer solar cells assisted with upconversion systems.
Introduction of metallic nanoparticles that can generate the surface plasmon resonance (SPR) has been considered as a prominent option for enhancing the performance of polymer solar cells (PSCs), as the radiative scattering and field confinement by the SPR can extend the effective photon traveling length and manipulate the spatial absorption profile. Despite many successful efforts to favorably exploit metallic nanoparticles, further studies of their effects on the PSC performance have been demanded to achieve the full benefit from them. Here, we systematically investigate the optical and photovoltaic performances of PSCs with disorderly distributed silver nanoprisms embedded in the photoactive material. Due to the superior properties of the plasmonic scattering of this class of nanoparticles, a significant improvement of photon absorption is gained from the devices with silver nanoprisms, particularly in the wavelength range of substandard absorption property including the band-edge wavelengths. While such absorption improvement can be obviously reinforced as an increase in the particle density, its level becomes saturated and decayed eventually because of the concurrently promoted photon loss by plasmonic absorption. At the optimal configurations of silver nanoprisms for the productive light trapping effect, the incorporated PSC devices present a photocurrent of ∼17.76 mA/cm2 and a power conversion efficiency of ∼9.68%, where their net increase ratios are ∼10% and ∼13% compared to the reference PSC devices, respectively. Details of numerical modeling and experiments for both metal nanoprisms and PSC devices offer an optimum route to tailoring metallic nanoparticles for high-performance PSC systems.
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