Optical transmission of a two-dimensional array of subwavelength holes in a metal film has been numerically studied using a differential method. Transmission spectra have been calculated showing a significant increase of the transmission in certain spectral ranges corresponding to the excitation of the surface polariton Bloch waves on a metal surface with a periodic hole structure. Under the enhanced transmission conditions, the near-field distribution of the transmitted light reveals an intensity enhancement greater than 2 orders of magnitude in localized ( approximately 40 nm) spots resulting from the interference of the surface polaritons Bragg scattered by the holes in an array.

A new surface wave is introduced, the cosine-Gauss beam, which does not diffract while it propagates in a straight line and tightly bound to the metallic surface for distances up to 80 μm. The generation of this highly localized wave is shown to be straightforward and highly controllable, with varying degrees of transverse confinement and directionality, by fabricating a plasmon launcher consisting of intersecting metallic gratings. Cosine-Gauss beams have potential for applications in plasmonics, notably for efficient coupling to nanophotonic devices, opening up new design possibilities for next-generation optical interconnects.

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We employ nonlinear autocorrelation measurements to investigate plasmon-assisted hot carrier dynamics generated in optical gold antennas. We demonstrate that surface plasmons enable a nonlinear formation of hot carriers, providing thus a unique lever to optimize the energy distribution and generation efficiency of the photo-excited charges. The temporal response of the carriers' relaxation can be controlled within a range extending from 500 fs to 2.5 ps. By conducting a quantitative analysis of the dynamics, we determine the nonlinear absorption cross-section of individual optical antennas. As such, this work provides strong insights on the understanding of plasmon-induced hot carrier generation, especially in the view of applications where the time response plays a preponderant role.

The fundamentals of the near-field interaction between a subwavelength metallic tip and a photonic-crystal nanocavity are investigated experimentally and theoretically. It is shown experimentally that the cavity resonance is tuned without any degradation by the presence of the tip and that the reported near-field interaction is strongly related to the field distribution within the nanostructure. Then, in light of a perturbation theory, we show that this interaction is selectively related to the electric field or magnetic field distribution within the cavity, depending on the tip properties. © 2007 The American Physical Society

The membrane surface of polarized renal epithelial cells (MDCK cells) grown as a monolayer was imaged with the atomic force microscope. The surface topography of dried cells determined by this approach was consistent with electron microscopy images previously reported. Fixed and living cells in aqueous medium gave more fuzzy images, likely because of the presence of the cell glycocalix. Treatment of living cells with neuraminidase, an enzyme that partly degrades the glycocalix, allowed sub-micrometer imaging. Protruding particles, 10 to 60 nm xy size, occupy most of the membrane surface. Protease treatment markedly reduced the size of these particles, indicating that they corresponded to proteins. Tip structure effects were probably involved in the exaggerated size of imaged membrane proteins. Although further improvements in the imaging conditions, including tip sharpness, are required, atomic force microscope already offers the unique possibility to image proteins at the membrane surface of living cells.

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In near-field optics the very concept of dipole is often used to represent either an elementary source or a scattering center. The most simple and widely used example is that of a small spherical particle whose polarizability is assumed to conform to the Clausius-Mossotti relation. While in conventional, far-field optics this approximation is known to be valid provided that the object is much smaller than the wavelength, its extension to near-field optics requires some precautions. Indeed, in the case of the scattering, by a spherical object, of an evanescent field generated, for instance, by total internal reflection or by a surface polariton, the strong-field gradient may increase the contribution to the polarizability of multipoles higher than the dipole. Such high-order multipoles are seldom considered in near-field optics because they complicate considerably any scattering calculation. In this paper we derive, for a spherical particle, the contributions of multipole orders up to the hexadecapole. This serves to illustrate the relative importance of each order. Moreover, within the framework of the coupled dipole method, we study, self-consistently, the problem of the scattering of an evanescent field by the sphere. We show that, with an initial field decreasing exponentially, the dipole approximation can be misleading.