Organic-inorganic halide perovskite quantum dots (PQDs) constitute an attractive class of materials for many optoelectronic applications. However, their charge transport properties are inferior to materials like graphene. On the other hand, the charge generation efficiency of graphene is too low to be used in many optoelectronic applications. Here, we demonstrate the development of ultrathin phototransistors and photonic synapses using a graphene-PQD (G-PQD) superstructure prepared by growing PQDs directly from a graphene lattice. We show that the G-PQDs superstructure synchronizes efficient charge generation and transport on a single platform. G-PQD phototransistors exhibit excellent responsivity of 1.4 × 108 AW–1 and specific detectivity of 4.72 × 1015 Jones at 430 nm. Moreover, the light-assisted memory effect of these superstructures enables photonic synaptic behavior, where neuromorphic computing is demonstrated by facial recognition with the assistance of machine learning. We anticipate that the G-PQD superstructures will bolster new directions in the development of highly efficient optoelectronic devices.
Reduced graphene oxide has certain unique qualities that make them versatile for a myriad of applications. Unlike graphene oxide, reduced graphene oxide is a conductive material and well suited for use in electrically conductive materials, such as solar cell devices. In this study, we report on the synthesis of graphene oxide as well as the fabrication and characterization of dye-sensitized solar cells with a photoanode which is an amalgam of reduced graphene oxide and titanium dioxide. The synthesized reduced graphene oxide and the corresponding photoanode were fully characterized using Ultraviolet-visible, Fourier transform infrared (FTIR), and Raman Spectrometry. The morphology of the sample was assessed using Atomic Force Microscopy, Field Emission Scanning Electron Microscopy, Transmission Electron Microscopy, and Energy Dispersive X-ray Spectroscopy. The photovoltaic characteristics were determined by photocurrent and photo-voltage measurements of the fabricated solar cells. The electrical impedances of both sets of devices were also evaluated. Overall, the solar to electric power efficiency of the device with reduced graphene oxide was observed to be higher (2.02%) than the device without the reduced graphene oxide (1.61%).
This work deals with the synthesis, characterization, and application of carbon nanoparticles (CNP) adorned graphene oxide (GO) nanocomposite materials. Here we mainly focus on an emerging topic in modern research field presenting GO-CNP nanocomposite as a infrared (IR) radiation detector device. GO-CNP thin film devices were fabricated from liquid phase at ambient condition where no modifying treatments were necessary. It works with no cooling treatment and also for stationary objects. A sharp response of human body IR radiation was detected with time constants of 3 and 36 sec and radiation responsivity was 3 mAW−1. The current also rises for quite a long time before saturation. This work discusses state-of-the-art material developing technique based on near-infrared photon absorption and their use in field deployable instrument for real-world applications. GO-CNP-based thin solid composite films also offer its potentiality to be utilized as p-type absorber material in thin film solar cell, as well.
Downloaded by [University of Nebraska, Lincoln] at 03:05 10 October 2015 ACCEPTED MANUSCRIPT ACCEPTED MANUSCRIPT 2 We studied the elemental analysis, structural morphology, mechanical, and electrical properties of carbon nanoparticles synthesised from diesel. The spherical carbon particles size in the range of about 10 to 80 nm in diameter was observed in SEM studies which were identified by AFM study as an aggregation of carbon particles of average size 2.5 nm. The surface rms of carbon nanoparticle thin film (CNTF) was measured directly by AFM and found 0.22 nm. The DMT elastic modulus of carbon nanoparticles (CNP) was measured by PeakForce QNM mode of AFM. The minimum and maximum elastic modulus was measured of 0.40 GPa and 43.89 GPa respectively. The resistivity, conductivity, magneto resistance, mobility and average Hall coefficient were measured by 'Ecopia Hall-effect measurement system' by 4-point Van der Pauw approach at ambient condition. We demonstrated I-V characteristic at the Indium/CNTF thin film interface which is accompanied by rectifying behavior.
We report an efficient infrared (IR) detector comprising reduced graphene oxide (RGO) and carbon nanoparticles (CNPs) for detecting human body IR radiation under ambient conditions.
Graphene oxide (GO) thin films were prepared by solution-casting of non-reduced suspension on glass substrates at ambient conditions. Films were rendered to conductive both with hydrazine treatment and annealing and the results were compared. Annealed films treated without hydrazine revealed superiority over the others. Surface morphology of these films showed very smooth film texture as seen by scanning electron microscope and atomic force microscope. Different optical and electrical parameters were analyzed. Band gap enhanced from 1.25 to 2.4 eV as the solution concentration was decreased where the transmittance increased. This work, in particular represents a straight forward approach compared to other studies to achieve device-quality GO thin films and the findings are important for various optoelectronic applications.
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