This study investigated the influence of membrane property and feed water organic matter quality on the permeate flux and water quality during gravity-driven membrane (GDM) filtration. GDM filtration was continuously carried out over 500 days at hydrostatic pressure of 65 mbar in dead-end mode without any back-flushing or membrane cleaning. Three ultrafiltration (UF) membranes (PES-100 kDa, PVDF-120 kDa, and PVDF-100 kDa) and one microfiltration (MF) membrane (PTFE-0.3 μm) were tested for treating lake water with varied organic matter qualities due to algal growth. The fluxes of the four membranes rapidly decreased to ~8 L/(m × h) within a week of GDM filtration. The flux variations were quite similar for the four membranes during the entire GDM filtration, indicating that membrane property has a little effect on the flux. The flux strongly depends on the feed water organic matter quality. The average flux in treating low organics containing water (7-60 days) was ~5 L/(m × h) and decreased to ~2 L/(m × h) in treating high organics containing water (60-300 days). The accumulation of algal-derived biopolymers was mainly responsible for the flux decline by forming biofilms with high permeation resistance. The average flux in 300-500 days increased to ~3.5 L/(m × h) when the feed water contained lower levels of biopolymers and higher levels of easily biodegradable organics, which created open and heterogeneous biofilms with lower permeation resistance. Removal efficiency for Escherichia coli was more than 5 log, while the removal efficiency for total bacterial cells was 1 log-2 log for the four membranes, indicating some bacterial regrowth after the filtration. Removal efficiency for the MS2 phage was 2.4 log and 1.5 log for the fouled PES-UF and PTFE-MF membranes.
Gravity-driven membrane (GDM) filtration is one of the promising technologies for decentralized water treatment systems due to its low cost, simple operation, and convenient maintenance. The objective of this study was to evaluate the permeability of submerged GDM filtration with three different membranes, i.e., polyethersulfone and polyvinylidene difluoride ultrafiltration (PES-UF and PVDF-UF) and polytetrafluoroethylene microfiltration membrane (PTFE-MF). The GDM system was operated using lake water for about one year. The determined average permeability values were high for PVDF-UF (192.9 L/m2/h/bar (LMH/bar)) and PTFE-MF (80.6 LMH/bar) and relatively lower for PES-UF (46.1 LMH/bar). The observed higher permeability for PVDF-UF and PTFE-MF was thought to be related to the rougher surface of these two membranes compared to PES-UF. The fouling layers of PVDF-UF and PTFE-MF were characterized by high biomass and the presence of a number of nematodes, while PES-UF showed a thin fouling layer with no nematode. The relatively high and fluctuated permeability of PVDF-UF and PTFE-MF could thus be attributed to the high biological activity of nematodes making the fouling layer more loose and porous. This was supported by a good linear relationship among the permeability, biomass concentration, and the number of nematodes in the fouling layers. These results provide important insights into membrane selection as a critical factor affecting the flux performance of the GDM filtration system for a decentralized drinking water supply.
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