+7 9117294724 1. AbstractThis work proposes new chemical and mechanical materials and techniques for III-V semiconductor NW/silicone membrane formation and optoelectronic device fabrication. Molecular beam epitaxy (MBE)-synthesized n-, p-and i-GaP NWs were encapsulated by introduced G-coating method into synthesized polydimethylsiloxane-graft-polystyrene and released from the Si growth substrate. The fabricated membranes were contacted with different materials including single-walled carbon nanotubes or ferrocenyl-containing polymethylhydrosiloxane with and without multi-walled carbon nanotubes doping. The electrical connection of the fabricated membranes was verified by electron beam induced current (EBIC) spectroscopy. The developed methods and materials can be applied for fabrication of high quality flexible inorganic optoelectronic devices.
IntroductionThe appealing properties of organic light emitting diodes (OLEDs), i. e. relatively easy and inexpensive fabrication, and efficient electroluminescence (EL) allowed the OLED-based industry to conquer a significant market share. For instance, modern smartphones are mostly produced with the OLED displays [weblink1, weblink2]. However, organic materials are far behind the inorganic materials in terms of stability and external quantum efficiency (EQE) of EL
Electrically conductive thin-film materials possessing high transparency are essential components for many optoelectronic devices. The advancement in the transparent conductor applications requires a replacement of indium tin oxide (ITO), one of the key materials in electronics. ITO and other transparent conductive metal oxides have several drawbacks, including poor flexibility, high refractive index and haze, limited chemical stability, and depleted raw material supply. Single-walled carbon nanotubes (SWCNTs) are a promising alternative for transparent conducting films (TCFs) because of their unique and excellent chemical and physical properties. Here, the latest achievements in the optoelectronic performance of TCFs based on SWCNTs are analyzed.Various approaches to evaluate the performance of transparent electrodes are briefly reviewed. A roadmap for further research and development of the transparent conductors using "rational design," which breaks the deadlock for obtaining the TCFs with a performance close to the theoretical limit, is also described.
We report here a new feasible approach to produce upconversion luminescent metal oxide aerogels with high textural characteristics. Monolithic aerogels show upconversion luminescence converting near-infra red excitation into visible light emission.
We propose a novel strategy to enhance optoelectrical properties of single-walled carbon nanotube (SWCNT) films for transparent electrode applications by film patterning. First, we theoretically considered the effect of the conducting pattern geometry on the film quality factor and, then, experimentally examined the calculated structures. We extend these results to show that the best characteristics of patterned SWCNT films can be achieved using the combination of initial film properties: low transmittance and high conductivity. The proposed strategy allows the patterned layers of SWCNTs to outperform the widely used indium-tin-oxide electrodes on both flexible and rigid substrates.Recent development of optoelectronic and photonic technologies for compact devices have introduced new challenges in fabrication of flexible, stretchable, transparent and conductive electrodes 1-3 . A wide range of possible applications includes solar cells 4 , light emitting diodes (LEDs) 5-7 , touchscreens 1,8,9 , "smart" devices, and wearable electronics 2,10 . The typical requirement for these applications is high transmittance in the middle of the visible spectral range and low sheet resistance. A few recent works have recently proposed new approaches, which allowed competing with highly efficient, indium-tin-oxide (ITO) coatings, one of the most developed and spread transparent conductive film (TCF) materials 1,11 . However, poor mechanical properties, high refractivity and price 2,12-14 , made researchers and engineers to search for alternative TCFs. Remarkable results were obtained with Cu and Ag nanofibers and nanowires 15 ,
We report a cathode material based on plasma‐treated single‐walled carbon nanotubes decorated by RuOx nanoparticles using atomic layer deposition. We have examined cathode performance towards hydrogen evolution reaction by tailoring material wettability, conductivity yielded by plasma treatment, and the catalyst loading. We discuss that nucleation of particles is facilitated by the appearance of carboxylic and hydroxyl groups triggered by oxygen plasma action. The best performance is associated with samples containing RuOx particles of 4–5 nm, which show hydrogen evolution onset potential to be about −5 mV (vs. RHE) in 0.5 M H2SO4 measured at a current density of −1 mA cm−2 and Tafel slope of 47.5 mV/dec. The material possesses stable performance at −10 mA cm−2 with a potential of about −160 mV.
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