A novel two-dimensional (2D) material member in the transition metal dichalcogenides family, few-layered rhenium disulfide (ReS) was prepared by liquid phase method successfully. By using the open-aperture Z-scan method, the saturable absorption properties at 2.8 μm were characterized with a saturable fluence of 22.6 μJ/cm and a modulation depth of 9.7%. A passively Q-switched solid-state laser at 2.8 μm was demonstrated by using the as-prepared ReS saturable absorber successfully. Under an absorbed pump power of 920 mW, a maximum output power of 104 mW was obtained with a pulse width of 324 ns and a repetition rate of 126 kHz. To the best of our knowledge, this is the first demonstration of applying ReS in an all-solid-state laser. Moreover, this represents the shortest pulses in Q-switched MIR lasers based on a 2D material as the saturable absorber, which demonstrated the superiority of ReS acting as an optical modulator for generating short-pulsed lasers. The results well prove that 2D ReS is a reliable optical modulator for MIR solid-state lasers.
1T-titanium selenide (1T-TiSe2), a representative of 1T phase transition metal dichalcogenides (TMDs), exhibits semimetallic behaviour with a nearly zero bandgap structure, which makes it a promising photoelectric material. A high-quality multilayer 1T-TiSe2 saturable absorber (SA) is successfully fabricated by a combination of liquid phase exfoliation and the spin coating method. The broadband nonlinear saturable absorption properties of the prepared 1T-TiSe2 SA are investigated by using the open aperture (OA) Z-scan method. Passively Q-switched (PQS) all-solid-state lasers with different bulk crystals at the wavelengths of 1.0, 1.3, 2.0 and 2.8 μm are realised based on the 1T-TiSe2 SA. To the best of our knowledge, this is the first presentation of the application of a 1T-TiSe2 material to all-solid-state bulk lasers. The results indicate that 1T-TiSe2 could be an alternative broadband SA for solid-state pulsed lasers and exhibits promising potential applications in mode-locked ultrafast lasers.
In this article, a high-power diode-end-pumped passively Q-switched (PQS) Tm:YAP laser is reported with novel two-dimension (2D) molybdenum ditelluride (MoTe) as a saturable absorber (SA). By using the open-aperture Z-scan method, the saturable absorption properties around 2.0 μm was characterized with a saturable fluence of 2.26 μJ∕cm and a modulation depth of 6.0% for the as-prepared MoTe SA. The band structure of MoTe with the introduction of Te vacancies is simulated by the DFT method, and the results indicate that the bandgap can be reduced with the vacancies in a suitable range. The shortest pulse width of 380 ns was obtained with an average output power of 1.21 W at a repetition rate of 144 kHz, corresponding to a maximum single pulse energy of 8.4 µJ and peak power of 22.2 W. It is the first presentation of MoTe as the saturable absorber in 2.0 μm solid-state pulse laser generation and the pulse width is the shortest among 2.0 μm solid-state lasers passive Q-switched with transitional metal dichalcogenides (TMDs) SAs to the best of our knowledge. The results indicated that MoTe should be an excellent optical modulator for high repetition rate and short pulsed laser generation in a broadband spectral range.
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.