Silicon nanowire (SiNW)-based solar cells on glass substrates have been fabricated by wet electroless chemical etching (using silver nitrate and hydrofluoric acid) of 2.7 microm multicrystalline p(+)nn(+) doped silicon layers thereby creating the nanowire structure. Low reflectance (<10%, at 300-800 nm) and a strong broadband optical absorption (>90% at 500 nm) have been measured. The highest open-circuit voltage (V(oc)) and short-circuit current density (J(sc)) for AM1.5 illumination were 450 mV and 40 mA/cm(2), respectively at a maximum power conversion efficiency of 4.4%.
Building upon the success and relevance of the 2014 Magnetism Roadmap, this 2017 Magnetism Roadmap edition follows a similar general layout, even if its focus is naturally shifted, and a different group of experts and, thus, viewpoints are being collected and presented. More importantly, key developments have changed the research landscape in very relevant ways, so that a novel view onto some of the most crucial developments is warranted, and thus, this 2017 Magnetism Roadmap article is a timely endeavour. The change in landscape is hereby not exclusively scientific, but also reflects the magnetism related industrial application portfolio. Specifically, Hard Disk Drive technology, which still dominates digital storage and will continue to do so for many years, if not decades, has now limited its footprint in the scientific Topical ReviewOriginal content from this work may be used under the terms of the Creative Commons Attribution 3.0 licence. Any further distribution of this work must maintain attribution to the author(s) and the title of the work, journal citation and DOI. and research community, whereas significantly growing interest in magnetism and magnetic materials in relation to energy applications is noticeable, and other technological fields are emerging as well. Also, more and more work is occurring in which complex topologies of magnetically ordered states are being explored, hereby aiming at a technological utilization of the very theoretical concepts that were recognised by the 2016 Nobel Prize in Physics.Given this somewhat shifted scenario, it seemed appropriate to select topics for this Roadmap article that represent the three core pillars of magnetism, namely magnetic materials, magnetic phenomena and associated characterization techniques, as well as applications of magnetism. While many of the contributions in this Roadmap have clearly overlapping relevance in all three fields, their relative focus is mostly associated to one of the three pillars. In this way, the interconnecting roles of having suitable magnetic materials, understanding (and being able to characterize) the underlying physics of their behaviour and utilizing them for applications and devices is well illustrated, thus giving an accurate snapshot of the world of magnetism in 2017.The article consists of 14 sections, each written by an expert in the field and addressing a specific subject on two pages. Evidently, the depth at which each contribution can describe the subject matter is limited and a full review of their statuses, advances, challenges and perspectives cannot be fully accomplished. Also, magnetism, as a vibrant research field, is too diverse, so that a number of areas will not be adequately represented here, leaving space for further Roadmap editions in the future. However, this 2017 Magnetism Roadmap article can provide a frame that will enable the reader to judge where each subject and magnetism research field stands overall today and which directions it might take in the foreseeable future.The first mater...
Various nanostructures are directly written by electron-beam-induced deposition using dimethyl-gold(III)-acetylacetonate as the precursor gas. After purification, their potential applications include plasmonic devices and metamaterials. Carbon contamination of the as-written structures can be completely removed by low-temperature ozone treatment, leaving polycrystalline pure gold structures (see figure). This treatment reduces the size of the nanostructures but does not substantially alter their functional shape
Magnetic multilayer films provide convenient model systems for studying the physics of antiferromagnetic films and surfaces. Here we report on the magnetic reversal and domain structure in antiferromagnetically coupled Co/Pt multilayers that are isomorphic to layered antiferromagnetic films with perpendicular magnetic anisotropy. We observe two distinct remanent states and reversal modes of the system. In mode 1 the magnetization in each layer reverses independently, producing an antiferromagnetic remanent state that shows full lateral correlation and vertical anticorrelation across the interlayers. In mode 2 the reversal in adjacent layers is locally synchronized with a remanent state that is vertically correlated but laterally anticorrelated in ferromagnetic stripe domains. Theoretical energy calculations of the two ground states identify a new phase boundary that is in good agreement with our experimental results.
Large thermal changes driven by a magnetic field have been proposed for environmentally friendly energy-efficient refrigeration 1 , but only a few materials which suffer hysteresis show these giant magnetocaloric effects 2-11 . Here we create giant and reversible extrinsic magnetocaloric effects in epitaxial films of the ferromagnetic manganite La 0.7 Ca 0.3 MnO 3 using strain-mediated feedback from BaTiO 3 substrates near a first-order structural phase transition. Our findings should inspire the discovery of giant magnetocaloric effects in a wide range of magnetic materials, and the parallel development of nanostructured bulk samples for practical applications.2 Magnetocaloric (MC) effects may be parameterized as adiabatic changes of temperature, or isothermal changes of entropy or heat, and have long been used to achieve millikelvin temperatures in the laboratory 12 . More recently, the discovery of giant MC effects near room temperature has led to suggestions for household and industrial cooling applications 1 . However, these giant MC effects arise in only a few materials [2][3][4][5][6][7][8][9][10][11] (Table 1), where strongly coupled magnetic and structural degrees of freedom produce magnetic phase transitions that are accompanied by changes in crystal symmetry 2-10 or volume 11 . It is therefore interesting to explore whether giant MC effects in magnetic materials can be created-rather than merely tuned 16 -via strain. (Table 1). By exploiting a first-order structural phase transition in BaTiO 3 (BTO) substrates, we create giant and reversible MC effects in epitaxial films of LCMO via the entropic interconversion of ferromagnetic and paramagnetic phases, whose coexistence 17,18 we reveal using photoemission electron microscopy (with magnetic contrast from x-ray magnetic circular dichroism) and ferromagnetic resonance.These extrinsic MC effects arise due to a strain-mediated feedback mechanism near the rhombohedral-orthorhombic transition in BTO at ~200 K, i.e. well away from LCMO C T at which the small intrinsic MC effects are seen. 3At temperature T, the isothermal entropy change ) (H S of a magnetic material due to applied magnetic field H may be obtained via the Maxwell relationprovided that thermally driven changes in measured magnetization M arise due to changes in the magnitude and not the direction of the local magnetization (μ 0 is the permeability of free space, the prime indicates the dummy variable of integration). The Clausius-Clapeyron equation:represents a nominally equivalent indirect method for evaluating S across first-order phase transitions in terms of the corresponding change in spontaneous magnetization 0 M and the field-induced shift in transition temperature T 0 . Equations 1 and 2 follow from thermodynamics and do not depend on microscopic details. X-ray diffraction (XRD) of room-temperature LCMO//BTO reveals that the film reflections are weak and broad, and confirms the presence of 90° BTO domains (Fig. 1).The relative population of BTO twins varies between substrates, wi...
Andreas Berger CICnanoGUNE BRTA Following the success and relevance of the 2014 and 2017 Magnetism Roadmap articles, this 2020 Magnetism Roadmap edition takes yet another timely look at newly relevant and highly active areas in magnetism research. The overall layout of this article is unchanged, given that it has proved the most appropriate way to convey the most relevant aspects of today’s magnetism research in a wide variety of sub-fields to a broad readership. A different group of experts has again been selected for this article, representing both the breadth of new research areas, and the desire to incorporate different voices and viewpoints. The latter is especially relevant for thistype of article, in which one’s field of expertise has to be accommodated on two printed pages only, so that personal selection preferences are naturally rather more visible than in other types of articles. Most importantly, the very relevant advances in the field of magnetism research in recent years make the publication of yet another Magnetism Roadmap a very sensible and timely endeavour, allowing its authors and readers to take another broad-based, but concise look at the most significant developments in magnetism, their precise status, their challenges, and their anticipated future developments. While many of the contributions in this 2020 Magnetism Roadmap edition have significant associations with different aspects of magnetism, the general layout can nonetheless be classified in terms of three main themes: (i) phenomena, (ii) materials and characterization, and (iii) applications and devices. While these categories are unsurprisingly rather similar to the 2017 Roadmap, the order is different, in that the 2020 Roadmap considers phenomena first, even if their occurrences are naturally very difficult to separate from the materials exhibiting such phenomena. Nonetheless, the specifically selected topics seemed to be best displayed in the order presented here, in particular, because many of the phenomena or geometries discussed in (i) can be found or designed into a large variety of materials, so that the progression of the article embarks from more general concepts to more specific classes of materials in the selected order. Given that applications and devices are based on both phenomena and materials, it seemed most appropriate to close the article with the application and devices section (iii) once again. The 2020 Magnetism Roadmap article contains 14 sections, all of which were written by individual authors and experts, specifically addressing a subject in terms of its status, advances, challenges and perspectives in just two pages. Evidently, this two-page format limits the depth to which each subject can be described. Nonetheless, the most relevant and key aspects of each field are touched upon, which enables the Roadmap as whole to give its readership an initial overview of and outlook into a wide variety of topics and fields in a fairly condensed format. Correspondingly, the Roadmap pursues the goal of giving each reader a brief reference frame of relevant and current topics in modern applied magnetism research, even if not all sub-fields can be represented here. The first block of this 2020 Magnetism Roadmap, which is focussed on (i) phenomena, contains five contributions, which address the areas of interfacial Dzyaloshinskii–Moriya interactions, and two-dimensional and curvilinear magnetism, as well as spin-orbit torque phenomena and all optical magnetization reversal. All of these contributions describe cutting edge aspects of rather fundamental physical processes and properties, associated with new and improved magnetic materials’ properties, together with potential developments in terms of future devices and technology. As such, they form part of a widening magnetism ‘phenomena reservoir’ for utilization in applied magnetism and related device technology. The final block (iii) of this article focuses on such applications and device-related fields in four contributions relating to currently active areas of research, which are of course utilizing magnetic phenomena to enable specific functions. These contributions highlight the role of magnetism or spintronics in the field of neuromorphic and reservoir computing, terahertz technology, and domain wall-based logic. One aspect common to all of these application-related contributions is that they are not yet being utilized in commercially available technology; it is currently still an open question, whether or not such technological applications will be magnetism-based at all in the future, or if other types of materials and phenomena will yet outperform magnetism. This last point is actually a very good indication of the vibrancy of applied magnetism research today, given that it demonstrates that magnetism research is able to venture into novel application fields, based upon its portfolio of phenomena, effects and materials. This materials portfolio in particular defines the central block (ii) of this article, with its five contributions interconnecting phenomena with devices, for which materials and the characterization of their properties is the decisive discriminator between purely academically interesting aspects and the true viability of real-life devices, because only available materials and their associated fabrication and characterization methods permit reliable technological implementation. These five contributions specifically address magnetic films and multiferroic heterostructures for the purpose of spin electronic utilization, multi-scale materials modelling, and magnetic materials design based upon machine-learning, as well as materials characterization via polarized neutron measurements. As such, these contributions illustrate the balanced relevance of research into experimental and modelling magnetic materials, as well the importance of sophisticated characterization methods that allow for an ever-more refined understanding of materials. As a combined and integrated article, this 2020 Magnetism Roadmap is intended to be a reference point for current, novel and emerging research directions in modern magnetism, just as its 2014 and 2017 predecessors have been in previous years.
A critical requirement for bit patterned media applications is the control and minimization of the switching field distribution (SFD). Here, we use the ΔH(M,ΔM) method to separate dipolar interactions due to neighbor islands from the intrinsic SFD by measuring a series of partial reversal curves of perpendicular anisotropy Co∕Pd based multilayer films deposited onto prepatterned Si substrates. For a 100-nm-period island array the dipolar broadening contributes 22% to the observed SFD. For a 45-nm-period array this value increases to 31%. These results highlight the importance of quantifying long-range dipolar interactions for determining the intrinsic SFD of patterned media.
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