Antiferromagnets are hard to control by external magnetic fields because of the alternating directions of magnetic moments on individual atoms and the resulting zero net magnetization. However, relativistic quantum mechanics allows for generating current-induced internal fields whose sign alternates with the periodicity of the antiferromagnetic lattice. Using these fields, which couple strongly to the antiferromagnetic order, we demonstrate room-temperature electrical switching between stable configurations in antiferromagnetic CuMnAs thin-film devices by applied current with magnitudes of order 10(6) ampere per square centimeter. Electrical writing is combined in our solid-state memory with electrical readout and the stored magnetic state is insensitive to and produces no external magnetic field perturbations, which illustrates the unique merits of antiferromagnets for spintronics.
Magnetic frustration effects in artificial kagome arrays of nanomagnets are investigated using x-ray photoemission electron microscopy and Monte Carlo simulations. Spin configurations of demagnetized networks reveal unambiguous signatures of long range, dipolar interaction between the nanomagnets. As soon as the system enters the spin ice manifold, the kagome dipolar spin ice model captures the observed physics, while the short range kagome spin ice model fails.
Large thermal changes driven by a magnetic field have been proposed for environmentally friendly energy-efficient refrigeration 1 , but only a few materials which suffer hysteresis show these giant magnetocaloric effects 2-11 . Here we create giant and reversible extrinsic magnetocaloric effects in epitaxial films of the ferromagnetic manganite La 0.7 Ca 0.3 MnO 3 using strain-mediated feedback from BaTiO 3 substrates near a first-order structural phase transition. Our findings should inspire the discovery of giant magnetocaloric effects in a wide range of magnetic materials, and the parallel development of nanostructured bulk samples for practical applications.2 Magnetocaloric (MC) effects may be parameterized as adiabatic changes of temperature, or isothermal changes of entropy or heat, and have long been used to achieve millikelvin temperatures in the laboratory 12 . More recently, the discovery of giant MC effects near room temperature has led to suggestions for household and industrial cooling applications 1 . However, these giant MC effects arise in only a few materials [2][3][4][5][6][7][8][9][10][11] (Table 1), where strongly coupled magnetic and structural degrees of freedom produce magnetic phase transitions that are accompanied by changes in crystal symmetry 2-10 or volume 11 . It is therefore interesting to explore whether giant MC effects in magnetic materials can be created-rather than merely tuned 16 -via strain. (Table 1). By exploiting a first-order structural phase transition in BaTiO 3 (BTO) substrates, we create giant and reversible MC effects in epitaxial films of LCMO via the entropic interconversion of ferromagnetic and paramagnetic phases, whose coexistence 17,18 we reveal using photoemission electron microscopy (with magnetic contrast from x-ray magnetic circular dichroism) and ferromagnetic resonance.These extrinsic MC effects arise due to a strain-mediated feedback mechanism near the rhombohedral-orthorhombic transition in BTO at ~200 K, i.e. well away from LCMO C T at which the small intrinsic MC effects are seen. 3At temperature T, the isothermal entropy change ) (H S of a magnetic material due to applied magnetic field H may be obtained via the Maxwell relationprovided that thermally driven changes in measured magnetization M arise due to changes in the magnitude and not the direction of the local magnetization (μ 0 is the permeability of free space, the prime indicates the dummy variable of integration). The Clausius-Clapeyron equation:represents a nominally equivalent indirect method for evaluating S across first-order phase transitions in terms of the corresponding change in spontaneous magnetization 0 M and the field-induced shift in transition temperature T 0 . Equations 1 and 2 follow from thermodynamics and do not depend on microscopic details. X-ray diffraction (XRD) of room-temperature LCMO//BTO reveals that the film reflections are weak and broad, and confirms the presence of 90° BTO domains (Fig. 1).The relative population of BTO twins varies between substrates, wi...
We report x-ray magnetic circular dichroism and superconducting quantum interference device magnetometry experiments to study magnetic order and coupling in thin Fe/(Ga, Mn)As(100) films. We observe induced magnetic order in the (Ga, Mn)As layer that extends over more than 2 nm, even at room temperature. We find spectroscopic evidences of a hybridized d configuration of Mn atoms in Fe/(Ga, Mn)As, with negligible Mn diffusion and/or MnFe intermixing. We show by experiment as well as by theory that the magnetic moment of the Mn ions couples antiparallel to the moment of the Fe overlayer.
Nucleation processes of mixed-phase states are an intrinsic characteristic of first-order phase transitions, typically related to local symmetry breaking. Direct observation of emerging mixed-phase regions in materials showing a first-order metal–insulator transition (MIT) offers unique opportunities to uncover their driving mechanism. Using photoemission electron microscopy, we image the nanoscale formation and growth of insulating domains across the temperature-driven MIT in NdNiO3 epitaxial thin films. Heteroepitaxy is found to strongly determine the nanoscale nature of the phase transition, inducing preferential formation of striped domains along the terraces of atomically flat stepped surfaces. We show that the distribution of transition temperatures is a local property, set by surface morphology and stable across multiple temperature cycles. Our data provide new insights into the MIT of heteroepitaxial nickelates and point to a rich, nanoscale phenomenology in this strongly correlated material.
International audienceVery large average velocities, up to 600 m/s, have been found for domain-wall motion driven by 3-ns-long pulses of electric current in zero magnetic field in the NiFe layer of 200-nm-wide NiFe/Cu/Co nanowires. For longer pulses, the domain-wall motion is strongly hindered by pinning potentials. Dipolar interactions between the NiFe and Co layers caused by anisotropy inhomogeneities have been identified as the most important among the different potential sources of DW pinning. The domain-wall velocities increase with current density, but a substantial drop is observed at current densities above 4×10^11 A/m
Large changes in the magnetization of ferromagnetic films can be electrically driven by non-180 ferroelectric domain switching in underlying substrates, but the shear components of the strains that mediate these magnetoelectric effects have not been considered so far. Here we reveal the presence of these shear strains in a polycrystalline film of Ni on a 0.68Pb(Mg 1/3 Nb 2/3)O 3-0.32PbTiO 3 substrate in the pseudo-cubic (011) pc orientation. Although vibrating sample magnetometry records giant magnetoelectric effects that are consistent with the hitherto expected 90 rotations of a global magnetic easy axis, high-resolution vector maps of magnetization (constructed from photoemission electron microscopy data, with contrast from x-ray magnetic circular dichroism) reveal that the local magnetization typically rotates through smaller angles of 62-84. This shortfall with respect to 90 is a consequence of the shear strain associated with ferroelectric domain switching. The non-orthogonality represents both a challenge and an opportunity for the development and miniaturization of magnetoelectric devices. Wisconsin-Madison (J.-M. H.). D. P. acknowledges funding from the Agència de Gestió d'Ajuts Universitaris i de Recercaa-Generalitat de Catalunya (Grant 2014 BP-A 00079). We thank Diamond Light Source for time on beamline I06 (proposal SI-8876), and we thank Sen Zhang for discussions. Author contributions M.G. initiated the study. M.G. and N.D.M. led the project with S.S.D. R.M., R.P.C. and C.H.W.B. were responsible for the growth of thin film Ni. The collection and preliminary analysis of PEEM data were performed by M.G., with assistance from X.M., L.C.P and W.Y. All other experimental work was performed by M.G. F.M. and S.S.D. were responsible for constructing PEEM vector maps, and the subsequent pixel by pixel analysis. D.P. performed image and data processing. N.D.M. proposed the pixel-by-pixel analysis of PEEM vector maps that led to the key finding of sub 90° magnetization rotation. J. M.H. identified and calculated the shear strain that accompanies ferroelectric domain switching in PMN-PT. M.G. identified the resulting principal axes of strain and hence magnetic easy axes. M.G. and N.D.M. interpreted the observed magnetoelectric effects.
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