We present results from light scattering experiments on tetragonal FeS with the focus placed on lattice dynamics. We identify the Raman active A1g and B1g phonon modes, a second order scattering process involving two acoustic phonons, and contributions from potentially defect-induced scattering. The temperature dependence between 300 and 20 K of all observed phonon energies is governed by the lattice contraction. Below 20 K the phonon energies increase by 0.5-1 cm −1 thus indicating putative short range magnetic order. Along with the experiments we performed latticedynamical simulations and a symmetry analysis for the phonons and potential overtones and find good agreement with the experiments. In particular, we argue that the two-phonon excitation observed in a gap between the optical branches becomes observable due to significant electronphonon interaction.
We report the evolution of the electronic correlation strength across the nematic critical point in FeySe1−xSx (0.10≦x≦0.24; y≧0.9), inferred from the measurements of the slope of the upper critical field Hc2. Superconducting transition Tc and quasiparticle mass m* exhibit similar reduction with sulfur content x. Our results indicate that electronic correlations from all Fermi surface pockets show strong interconnection with pairing strength and are not governed by the change of nematic fluctuations. The upper critical field anisotropy γH = Hc2
ab/Hc2
c exhibits a minimum in the critical region and stronger temperature dependence away from it.
Symmetries, quantum geometries and electronic correlations are among the most important ingredients of condensed matters, and lead to nontrivial phenomena in experiments, for example, non-reciprocal charge transport. Of particular interest is whether the non-reciprocal transport can be manipulated. Here, we report the controllable large non-reciprocal charge transport in the intrinsic magnetic topological insulator MnBi2Te4. The current direction relevant resistance is observed at chiral edges, which is magnetically switchable, edge position sensitive and stacking sequence controllable. Applying gate voltage can also effectively manipulate the non-reciprocal response. The observation and manipulation of non-reciprocal charge transport reveals the fundamental role of chirality in charge transport of MnBi2Te4, and pave ways to develop van der Waals spintronic devices by chirality engineering.
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