The resistivity of thin $La_{0.7}A_{0.3}MnO_{3}$ films ($A=Ca, Sr$) is
investigated in a wide temperature range. The comparison of the resistivities
is made among films grown by different techniques and on several substrates
allowing to analyze samples with different amounts of disorder. In the
low-temperature nearly half-metallic ferromagnetic state the prominent
contribution to the resistivity scales as $T^{\alpha}$ with $\alpha \simeq 2.5$
for intermediate strengths of disorder supporting the theoretical proposal of
single magnon scattering in presence of minority spin states localized by the
disorder. For large values of disorder the low-temperature behavior of the
resistivity is well described by the law $T^{3}$ characteristic of anomalous
single magnon scattering processes, while in the regime of low disorder the
$\alpha$ exponent tends to a value near 2. In the high temperature insulating
paramagnetic phase the resistivity shows the activated behavior characteristic
of polaronic carriers. Finally in the whole range of temperatures the
experimental data are found to be consistent with a phase separation scenario
also in films doped with strontium ($A=Sr$).Comment: 5 figure
We report on the role of oxygen content alone on structural and transport properties of La0.65Sr0.35MnO3−δ (LSMO) thin films. Identical films were deposited side-by-side during a single deposition run and subsequently post-annealed separately in vacuum to systematically vary the oxygen content. All films remained coherently strained to the SrTiO3 substrate, with no broadening of rocking curve widths after post-anneal. As oxygen content decreases, the LSMO unit cell expands while the metal-insulator transition temperature TMI decreases. A linear correlation between the out-of-plane lattice parameter and the metal-insulator transition temperature was observed.
We report resistance versus magnetic field measurements for a La0.65Sr0.35MnO3/SrTiO3/La0.65Sr0.35MnO3 tunnel junction grown by molecular-beam epitaxy, that show a large field window of extremely high tunneling magnetoresistance (TMR) at low temperature. Scanning the in-plane applied field orientation through 360 • , the TMR shows 4-fold symmetry, i.e. biaxial anisotropy, aligned with the crystalline axes but not the junction geometrical long axis. The TMR reaches ∼ 1900 % at 4 K, corresponding to an interfacial spin polarization of > 95 % assuming identical interfaces. These results show that uniaxial anisotropy is not necessary for large TMR, and lay the groundwork for future improvements in TMR in manganite junctions.
The performance of manganite-based magnetic tunnel junctions (MTJs) has suffered from reduced magnetization present at the junction interfaces that is ultimately responsible for the spin polarization of injected currents; this behavior has been attributed to a magnetic "dead layer" that typically extends a few unit cells into the manganite. X-ray magnetic scattering in resonant conditions (XRMS) is one of the most innovative and effective techniques to extract surface or interfacial magnetization profiles with subnanometer resolution, and has only recently been applied to oxide heterostructures. Here we present our approach to characterizing the surface and interfacial magnetization of such heterostructures using the XRMS technique, conducted at the BEAR beamline (Elettra synchrotron, Trieste). Measurements were carried out in specular reflectivity geometry, switching the left/right elliptical polarization of light as well the magnetization direction in the scattering plane. Spectra were collected across the Mn L 2,3 edge for at least four different grazing angles in order to better analyse the interference phenomena. The resulting reflectivity spectra have been carefully fit to obtain the magnetization profiles, minimizing the number of free parameters as much as possible. Optical constants of the samples (real and imaginary part of the refractive index) in the interested frequency range are obtained through absorption measurements in two magnetization states and subsequent Kramers-Kronig transformation, allowing quantitative fits of the magnetization profile at different temperatures. We apply this method to the study of air-
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