38 pages, 15 figuresPeripheral collisions with radioactive heavy-ion beams at relativistic energies are discussed as an innovative approach for probing the transient regime experienced by fissile systems evolving towards quasi-equilibrium. A dedicated experiment using the advanced technical installations of GSI, Darmstadt, permitted to realize ideal conditions for the investigation of relaxation effects in the meta-stable well. Combined with a highly sensitive experimental signature, it provides a measure of the transient effects with respect to the flux over the fission barrier. Within a two-step reaction process, 45 proton-rich unstable spherical isotopes produced by projectile-fragmentation of a stable 238U beam have been used as secondary projectiles. The fragmentation of the radioactive projectiles on lead results in nearly spherical compound nuclei which span a wide range in excitation energy and fissility. The decay of these excited systems by fission is studied with a dedicated set-up which permits the detection of both fission products in coincidence and the determination of their atomic numbers with high resolution. The width of the fission-fragment nuclear charge distribution is shown to be specifically sensitive to pre-saddle transient effects and is used to establish a clock for the passage of the saddle point. The comparison of the experimental results with model calculations points to a fission delay of (3.3+/-0.7).10-21s for initially spherical compound nuclei, independent of excitation energy and fissility. This value suggests a nuclear dissipation strength at small deformation of (4.5+/-0.5).1021s-1. The very specific combination of the physics and technical equipment exploited in this work sheds light on previous controversial conclusions
The nuclide cross sections and the longitudinal velocity distributions of residues produced in the reactions of 136 Xe and 124 Xe at 1 A GeV in a lead target were measured at the highresolution magnetic spectrometer, the Fragment Separator (FRS) of GSI. The data cover a broad range of isotopes of the elements between Z = 3 and Z = 56 for 136 Xe and between Z = 5 and Z = 55 for 124 Xe, reaching down to cross sections of a few microbarns. The velocity distributions exhibit a Gaussian shape for masses above A = 20, while more complex behaviour is observed for lighter masses. The isotopic distributions for both reactions preserve a memory on the projectile N/Z ratio over the whole residue mass range.
Production cross sections of medium-mass neutron-rich nuclei obtained in the fragmentation of 136 Xe projectiles at 1 A GeV have been measured with the FRagment Separator (FRS) at GSI. 125 Pd was identified for the first time. The measured cross sections are compared to 238 U fission yields and model calculations in order to determine the optimum reaction mechanism to extend the limits of the chart of the nuclides around the r-process waiting point at N=82.
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