2022
DOI: 10.1038/s41563-021-01172-3
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Suspension electrolyte with modified Li+ solvation environment for lithium metal batteries

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Cited by 241 publications
(162 citation statements)
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“…57,58 Inorganic components are believed to be beneficial to the improvement of SEI/CEI performance, as verified by experiments. Adding Li 2 S nanoparticles in SEI and Li 2 O nanoparticles in electrolytes could boost the cycling stability, 24,59 and Li 3 N and LiF also exhibited positive impacts on Li battery performance. 21,60 In addition, Li + could diffuse quickly in the grain boundary among Li 2 S, Li 3 N, Li 2 O, and LiF.…”
Section: Anion Regulationmentioning
confidence: 99%
“…57,58 Inorganic components are believed to be beneficial to the improvement of SEI/CEI performance, as verified by experiments. Adding Li 2 S nanoparticles in SEI and Li 2 O nanoparticles in electrolytes could boost the cycling stability, 24,59 and Li 3 N and LiF also exhibited positive impacts on Li battery performance. 21,60 In addition, Li + could diffuse quickly in the grain boundary among Li 2 S, Li 3 N, Li 2 O, and LiF.…”
Section: Anion Regulationmentioning
confidence: 99%
“…Over the past few years, several strategies including optimization of electrolyte, modification of current collector, and adjustment of testing parameters have been devoted to improving the electrochemical performance of Li metal batteries by constructing favorable solid electrolyte interphase (SEI) and optimization of delithiation process [ 10 13 ]. The development of dual-salt electrolyte, local high-concentration electrolyte or novel electrolyte chemistry could enhance the Coulombic efficiency (CE) of plated Li metal on bare Cu up to 99.5%, which could fulfill the critical requirement of realistic anode-free Li metal batteries [ 14 18 ]. However, the volume fluctuation derived from continuous Li plating/stripping on planar current collector should be also took into account, especially in the practical pouch cells [ 19 ].…”
Section: Introductionmentioning
confidence: 99%
“…[ 2–4 ] However, the sluggish ion diffusion and high charge‐transfer resistance in metallic lithium anodes especially at high rates dramatically aggravate lithium dendrite growth and intensify volume change, leading to rapid electrolyte consumption, low Coulombic efficiency (CE), and capacity decay of LMBs. [ 5–7 ]…”
Section: Introductionmentioning
confidence: 99%