of applications, such as flexible displays, image sensors, biomedical actuators, and touch panels, due to their good mechanical robustness properties and excellent compatibility of high integration processes. [1][2][3][4][5][6] Over the years, specifically p-type based FETs such as organic, oxide, and 2D semiconductor materials, extensive studies have been investigated to develop good electrical performance such as high carrier mobility and excellent on-off current ratio with chemically and physically stable material properties but are still limited in exploring on a larger scale with expandable applications, micro-scale fabrication, low-temperature processing, and flexibility. [7][8][9][10][11][12] To fully explore the largescale flexible platform-oriented FETs, the p-type semiconductor requires easy and effective processing techniques with temperature independency and expandable applicability in the field of electronics.Tellurium (Te), as a semiconductor material, has recently gained substantial interest due to its favorable properties such as excellent photoconductivity, good piezoelectricity, and high transport properties. [13][14][15][16][17][18][19] Concerning the Te structural properties, it has a strong anisotropic property which endows it to form 1D nanostructure (i.e., nanowires, nanorods, and nanotubes) along its c-axis. [20][21][22][23][24][25][26][27][28] Moreover, Te endures a trigonal atomic structure with strong van der Waals bonding to its neighboring atoms and forms a helical chain of atoms. [29][30][31][32] In recent, based on the 1D nanostructure of Te semiconductor, various studies have been reported to obtain high electrical properties but are limited in terms of stabilization and uniformity of the film synthesis and scalable fabrication. [33][34][35][36] Due to the curly shape of atomic chains of 1D Te nanostructure, the large-scale synthesis with high uniformity and stability is quite sensitive for fieldeffect transistors (FETs) fabrication with extensive applicability. In this regard, various strategies have successfully been demonstrated to enhance the electrical performance of atomic helical chain-type Te nanostructures-based FET devices through encapsulation methods of CNTs and boron nitride nanotubes (BNNTs), [33][34][35]37] but are still limited in terms of expanding Here, a novel method is introduced to synthesize the uniform hybrid structure of tellurium nanowires (TeNWs) and tellurium-film (Te-film) for flexible fieldeffect transistor (FET) array device to exhibit excellent electrical, mechanical, and optical performance. To fabricate such a device, all the processes are performed at low temperatures (< 100 °C) with easy processing methods. The uniformity of the hybrid structure of TeNWs/Te-film is confirmed using scanning electron microscopy (SEM) and Raman spectroscopy with a comparison of the bare TeNWs-film. Electrical properties of the TeNWs/ Te-based FET device exhibits high mobility of 5.35 cm 2 V −1 s −1 and on/off ratio of >10 4 along with stable and uniform results of th...