We introduce a femtosecond-laser-based technique for selective opening of airholes in photonic crystal fibers (PCFs). With this technique, selective filling and inflation of the airholes in the PCF cladding are demonstrated. The technique may find important applications in tailoring or altering PCF characteristics and make it possible to seamlessly integrate various components/functions into PCFs. © 2010 Optical Society of America OCIS codes: 060.2310, 060.2340, 060.2400.The photonic crystal fiber (PCF) with a periodic array of airholes running along its length has attracted significant interest recently [1,2]. The precise arrangement of airholes and their index profiles throughout the cladding region allow various types of PCFs with novel properties to be designed. Endlessly single-mode operation, lightguidance in hollow air-core, and very high nonlinearity and birefringence are a few of the novel properties of PCFs that may not be achieved with conventional singlemode fibers (SMFs) [3,4]. Apart from the high level of flexibility in the PCF fabrication process, novel functionality may be added to PCFs by postprocessing [5][6][7][8].Techniques for postprocessing PCFs include tapering and inscription of periodic structures that are widely adopted for conventional fibers and selective filling or pressurization of airholes, which is unique to PCFs. Examples of PCF postprocessing include selective filling of airholes with an index tunable polymer to realize birefringence tunability [5], inflating/deflating airholes to reduce splice loss and to achieve in-fiber mode conversion [6,7], and infiltrating submicrometer gold into a selected hole of a polarization maintaining PCF to achieve polarizationand wavelength-dependent transmission [8]. All these examples rely on the selective opening or closing of airholes within the cladding region. We previously demonstrated selective filling of PCFs by using a conventional fusion splicer [9], but it lacks the freedom to choose arbitrary airholes for filling. In this Letter, we report a technique for selective opening of airholes and demonstrate the selective filling and inflation of arbitrary holes in the PCF cladding. Our approach starts by sealing all the airholes of a PCF by a thin layer of silica and then drilling individual holes through the layer by a femtosecond IR laser (fs-laser). With reference to Fig. 1(a), the PCF is first spliced to a conventional SMF by a fusion splicer. The SMF is then cleaved at a location about 30 μm from the splicing point. The splicing parameters are adjusted so that airhole deformation during splicing is minimized, while the splice is reasonably strong to survive the cleaving [10]. The thin layer of SMF seals all the airholes, but the end facet of the PCF beneath the thin silica layer can be clearly viewed under a microscope, allowing an individual airhole to be selected and located. Figure 1(b) shows the microscopic view of the end facet of a large-mode-area PCF [LMA-10, NKT Photonics A/S, scanning electron micrograph (SEM) photograph is sho...