2021
DOI: 10.1016/j.carbon.2020.12.031
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Optical properties of silicon-implanted polycrystalline diamond membranes

Abstract: We investigate the optical properties of polycrystalline diamond membranes containing silicon-vacancy (SiV) color centers in combination with other nano-analytical techniques. We analyze the correlation between the Raman signal, the SiV emission, and the background luminescence in the crystalline grains and in the grain boundaries, identifying conditions for the addressability of single SiV centers. Moreover, we perform a scanning transmission electron microscopy (STEM) analysis, which associates the microscop… Show more

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Cited by 10 publications
(5 citation statements)
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“…After annealing, the PL signal of the formed emitters is acquired using a confocal scanning setup described in detail in ref. [22]. Figure 1d shows an exemplary result, reproducing the implanted matrix except for the spots with 10 3 Si ions or less.…”
Section: Methods and Preparationmentioning
confidence: 91%
“…After annealing, the PL signal of the formed emitters is acquired using a confocal scanning setup described in detail in ref. [22]. Figure 1d shows an exemplary result, reproducing the implanted matrix except for the spots with 10 3 Si ions or less.…”
Section: Methods and Preparationmentioning
confidence: 91%
“…PCD membrane is a good platform for photostable quantum emitters; for example, SiV color centers can be easily implanted in the first few nanometer layers for near‐field plasmon coupling. [ 30,46 ]…”
Section: Methodsmentioning
confidence: 99%
“…PCD membrane is a good platform for photostable quantum emitters; for example, SiV color centers can be easily implanted in the first few nanometer layers for near-field plasmon coupling. [30,46] The AFM head facilitated three directional degrees of freedom to control the probe. Besides, the sample was mounted on an XY piezo stage, and thus in total, we had five directional degrees of freedom.…”
Section: Methodsmentioning
confidence: 99%
“…In other words, it is questionable whether polycrystalline diamond defects (grain surface and sp 2 -related defects) might act as traps for the excited carriers of SiV centers, hence decreasing their internal PL quantum efficiency. The latter is relatively unimportant in a relatively thick (few microns) film where the surface to volume ratio is low; 14 however, in thin layers of 100–300 nm, the grain surface and sp 2 -defects may play an important role in the light emission efficiency of SiV centers. Diamond thin films prepared on a low-index substrate could be considered a promising material for diamond photonic structures provided the coupling of SiV centers to defects can manifest itself as inefficient.…”
Section: Introductionmentioning
confidence: 99%