Jute cellulose nanocrystal/poly(N,N-dimethylacrylamide-co-3-methacryloxypropyltrimethoxysilane) hybrid hydrogels for removing methylene blue dye from aqueous solution

Hossain, Shafiul; Shahruzzaman, Md.; Kabir, Sumaya F.; Rahman, Md. Shirajur; Sultana, Sabrina; Mallik, Abul K.; Haque, Papia; Takafuji, Makoto; Rahman, Mohammed Mizanur

doi:10.1016/j.jsamd.2021.02.005

Cited by 18 publications

(4 citation statements)

References 27 publications

Supporting

Mentioning

Contrasting

Order By: Relevance

“…The preparation of jute fiber from cellulose nanocrystal was followed as per our previous report [ 16 ]. At first, the jute fibers were washed to remove impurities.…”

Section: Methodsmentioning

confidence: 99%

Advanced CNC/PEG/PDMAA Semi-IPN Hydrogel for Drug Delivery Management in Wound Healing

Afrin

Shahruzzaman

Haque

et al. 2022

Gels

Self Cite

View full text Add to dashboard Cite

A Semi Interpenetrating Polymer Network (semi-IPN) hydrogel was prepared and loaded with an antibiotic drug, gentamicin, to investigate the wound healing activity of this system. The semi-IPN hydrogel was synthesized by combining natural polymer cellulose nanocrystal (CNC) and synthetic polymer polyethylene glycol (PEG) and poly (N,N′-dimethyl acrylamide) (PDMAA), which was initially added as a monomer dimethyl acrylamide (DMAA). CNC was prepared from locally obtained jute fibers, dispersed in a PEG-NaOH solvent system and then mixed with monomer DMAA, where polymerization was initiated by an initiator potassium persulphate (KPS) and cross-linked by N,N′-methylenebisacrylamide (NMBA). The size, morphology, biocompatibility, antimicrobial activity, thermal and swelling properties of the hydrogel were investigated by different characterization techniques. The biocompatibility of the hydrogel was confirmed by cytotoxicity analysis, which showed >95% survival of the BHK-21, Vero cell line. The drug loaded hydrogel showed antimicrobial property by forming 25 and 23 mm zone of inhibition against Staphylococcus aureus (gram-positive) and Escherichia coli (gram-negative) bacteria, respectively, in antimicrobial analysis. At pH 5.5, 76% of the drug was released from the hydrogel within 72 h, as observed in an in vitro drug release profile. In an in vivo test, the healing efficiency of the drug loaded hydrogel was examined on a mice model with dorsal wounds. Complete healing of the wound without any scar formation was achieved in 12 days, which revealed excellent wound healing properties of the prepared drug loaded semi-IPN hydrogel. These results showed the relevance of such a system in the rapid healing of acute wounds.

show abstract

“…The preparation of jute fiber from cellulose nanocrystal was followed as per our previous report [ 16 ]. At first, the jute fibers were washed to remove impurities.…”

Section: Methodsmentioning

confidence: 99%

Advanced CNC/PEG/PDMAA Semi-IPN Hydrogel for Drug Delivery Management in Wound Healing

Afrin

Shahruzzaman

Haque

et al. 2022

Gels

Self Cite

View full text Add to dashboard Cite

show abstract

“…Hossain et al proved this theory when they synthesized DMAA-based 3-methacryloxypropyltrimethoxysilane hydrogels and used them for removing methylene blue cationic dye from waste water. The maximum adsorption value of the DMAA-based hydrogel was 131.58 mg/g [ 31 ]. Since DMAA acts as a hydrogen bond acceptor, it could help to enhance the material’s adsorption properties.…”

Section: Nn-dimethylacrylamide-based Hydrogels For Dye Removalmentioning

confidence: 99%

“…The adsorption capacity of DMAA hydrogels augments with the increasing of pH of the solution due to the hydrolysis and protonation. Mechanisms of adsorption have been noticed on the works of Hossain et al ( Figure 1 ) [ 31 , 33 ]. At low value of pH, dimethyl acrylamide groups are protonated, and a positively charged NH(CH 3 ) 2 + surface leads to electrostatic interaction with the negatively charged dye molecules, thus improving the negatively charged dye removal [ 34 , 35 ].…”

Section: Nn-dimethylacrylamide-based Hydrogels For Dye Removalmentioning

confidence: 99%

A Short Review on the N,N-Dimethylacrylamide-Based Hydrogels

Akhmetzhan

Myrzakhmetova

Amangeldi

et al. 2021

Gels

View full text Add to dashboard Cite

Scientists have been encouraged to find different methods for removing harmful heavy metal ions and dyes from bodies of water. The adsorption technique offers promising outcomes for heavy metal ion removal and is simple to run on a large scale, making it appropriate for practical applications. Many adsorbent hydrogels have been developed and reported, comprising N,N-dimethylacrylamide (DMAA)-based hydrogels, which have attracted a lot of interest due to their reusability, simplicity of synthesis, and processing. DMAA hydrogels are also a suitable choice for self-healing materials and materials with good mechanical properties. This review work discusses the recent studies of DMAA-based hydrogels such as hydrogels for dye removal and the removal of hazardous heavy metal ions from water. Furthermore, there are also references about their conduct for self-healing materials and for enhancing mechanical properties.

show abstract

“…In addition, jute is the golden fiber of Bangladesh which has been grasped attention as a potential reinforcement of polymer composites 17 . So far, millimeter-scale jute fiber based hydrogels are rarely reported except few on submicrometer scale such as jute cellulose 18 and carboxymethylated cellulose nanofiber 19 hydrogels.…”

Section: Introductionmentioning

confidence: 99%

Jute Fiber Reinforced Hydrogel Composite for Removal of Methylene Blue Dye from Water

Shakil

Begum

Shaikh

et al. 2022

Dhaka Univ. J. Sci.

View full text Add to dashboard Cite

In this study, a hydrogel composite based on natural jute fiber (JF) has been prepared and employed for the removal of methylene blue (MB) dye from aqueous solution. Polyacrylamide (PAAm) hydrogel was synthesized by thermal polymerization in presence of N,N□-methylene bisacrylamide (MBAA) as the cross-linker and potassium per sulfate (KPS) as the initiator. JF reinforced hydrogel (JFRH) composite was prepared by incorporating JF into PAAm matrix prior to the polymerization. The prepared JFRH was characterized by FTIR spectroscopy and scanning electron microscope. It was found that, JFRH composite demonstrated strong mechanical properties with a compressive strength of 1.5 MPa at a deformation of above 80%. The prepared JFRH composite can remove more than 90% of MB from an aqueous solution and be separated easily from the solution after the adsorption process. Therefore, the synthesized JF based hydrogel composite could significantly expand the use of our natural golden fiber for reinforcement of composite materials and removal of dyes from water bodies. Dhaka Univ. J. Sci. 70(2): 59-64, 2022 (July)

show abstract

Jute cellulose nanocrystal/poly(N,N-dimethylacrylamide-co-3-methacryloxypropyltrimethoxysilane) hybrid hydrogels for removing methylene blue dye from aqueous solution

Cited by 18 publications

References 27 publications

Advanced CNC/PEG/PDMAA Semi-IPN Hydrogel for Drug Delivery Management in Wound Healing

Advanced CNC/PEG/PDMAA Semi-IPN Hydrogel for Drug Delivery Management in Wound Healing

A Short Review on the N,N-Dimethylacrylamide-Based Hydrogels

Jute Fiber Reinforced Hydrogel Composite for Removal of Methylene Blue Dye from Water

Contact Info

Product

Resources

About