A facile water-based one-pot reaction protocol for obtaining 20 nm thick uniform silica coatings on cellulose nanofibrils (CNFs) are herein presented for the first time. The fully covering silica shells result in a thermal stability of the CNFs improved by ca. 70 °C and 50 °C under nitrogen and oxygen atmosphere, respectively. Heating of the core-shell hybrid fibres to 400 °C results in complete degradation/removal of the CNF cores, and demonstrates an inexpensive route to large-scale preparation of silica nanotubes with the CNFs used as templates. The key to a uniform condensation of the silica (from tetraethyl orthosilicate) to the cellulose is a reaction medium that permits in-situ nucleation and growth of the silica phase on the fibrils, while simultaneously matching the quantity of the condensed silica with specific surface area of the CNFs. Most coatings were applied to bundles of 2-3 associated CNFs, which could be discerned from their negative imprint that remained inside the silica nanotubes. Finally, it is demonstrated how the coated nanofibrils can be freeze-dried into highly porous associated silica/cellulose aerogels with a density of 0.005 g/cm 3 and how these hybrid aerogels preserve their shape when extensively exposed to 400 °C under air (>6 h). The resulting material is the first reported silica nanotube aerogel obtained by using cellulose nanofibrils as templates.