Efficient keV X-ray Generation from Irradiation of in-situ Produced Silver Clusters by Ti:sapphire Laser Pulses

In this paper, an experimental study on generation of nanoparticle various sizes using Ti:sapphire laser pulses, is reported. Nanoparticle formation in plasma plumes of metals like silver and copper, expanding in vacuum, has been studied using stretched pulses of 300 ps duration [subnanoseconds (sub-ns)] from a Ti:sapphire laser. It has been compared with the nanoparticle formation (of the same materials) when compressed pulses of 45 fs duration were used under similar focusing conditions. Nanoparticle formation is observed at intensities as high as 2×1016 W/cm2. The structural analysis of the nanoparticle deposition on a silicon substrate showed that, using 45 fs pulses, smaller nanoparticles of average size ∼20 nm were generated, whereas on using the sub-ns pulses, larger particles were produced. Also, the visible light transmission and reflection from the nanoparticle film of Ag on glass substrate showed surface plasmon resonance (SPR). The SPR curves of the films of nanoparticles deposited by femtosecond pulses were always broader and reflection/transmission was always smaller when compared with the films formed using the sub-ns pulses, indicating smaller size particle formation by ultrashort pulses. Thus, it has been demonstrated that variation in the laser pulse duration of laser offers a simple tool for varying the size of the nanoparticles generated in plasma plumes.

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X-ray enhancement in a nanohole target irradiated by intense ultrashort laser pulses

Chakravarty

Arora

Chakera

et al. 2011

Journal of Applied Physics

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In this paper, we present a comparative study of the laser energy absorption, soft x-ray emission (in the water window region: 2.3–4.4 nm) and hard x-ray emission (in the 2–20 keV range) from planar aluminum and nanohole alumina of 40 nm average diameter, when irradiated by Ti:sapphire laser pulses. The laser pulse duration was varied from 45 to 500 fs, and the focused intensity on the target ranged from ∼3 × 1016 W/cm2 to 3×1017 W/cm2. The x-ray yield enhancement from the nanoholes shows an increased coupling of the laser energy to the target. The effect of laser pulse duration on the x-ray emission was also studied, where a resonance like phenomenon was observed. The laser energy absorption measurements in the nanoholes showed a marginal enhancement in absorption as compared to planar Al. The integrated keV x-ray yield, from nanohole alumina and planar Al, at an intensity of 3 × 1017 W/cm2, was 25 and 3.5 μJ, respectively. The results can be explained by considering the hydrodynamic expansion of the laser irradiated structure and field enhancement in the nanoholes.

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Efficient keV X-ray Generation from Irradiation of in-situ Produced Silver Clusters by Ti:sapphire Laser Pulses

Cited by 4 publications

References 29 publications

Enhanced soft X-ray emission from carbon nanofibers irradiated with ultra-short laser pulses

Enhanced soft X-ray emission from carbon nanofibers irradiated with ultra-short laser pulses

Formation of metal nanoparticles of various sizes in plasma plumes produced by Ti:sapphire laser pulses

X-ray enhancement in a nanohole target irradiated by intense ultrashort laser pulses

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