A doctoral thesis is often described as a solitary endeavour; however, the long list that follows definitely proves the opposite. First and foremost, I would like to express my sincere and profound gratitude to my supervisor and promotor Arjen, whose support was crucial in shaping my thesis with his immense knowledge, critical reviews and patience. Thank you, Arjen, for giving me the opportunity to do my PhD research with you and for providing me with comfortable research conditions. I learned a lot from you Arjen and without your support, I certainly could not have finished my dissertation successfully. I'm also indebted to Maarten who has been my daily supervisor and whose contribution to the completion of this thesis is indispensable. Maarten, I have been extremely lucky to have a supervisor who cared so much about my work, and who responded to my questions and queries so promptly. Your knowledge of good scientific and mathematical practices has shaped this dissertation in numerous ways. Meetings with you were always very encouraging and inspiring. My special thanks go to Joke, our enthusiastic and very helpful office manager. Your administrative and personal support has provided another very necessary part of PhD life. The help from you alongside with Anke and Monique has made my life at the UT easier. I would like to thank all my current and former colleagues at the WEM department and friends of current and former WFN for all lunch talks, coffee times, WEM uitje, Chrismas lunch, EGU conference time and all great conversations. Special thanks to